Electron beam shaping allows the control of the temporal properties of x-ray free-electron laser pulses from femtosecond to attosecond timescales. Here we demonstrate the use of a laser heater to shape electron bunches and enable the generation of attosecond x-ray pulses. We demonstrate that this method can be applied in a selective way, shaping a targeted subset of bunches while leaving the remaining bunches unchanged. This experiment enables the delivery of shaped x-ray pulses to multiple undulator beamlines, with pulse properties tailored to specialized scientific applications.

X-ray Free Electron Lasers provide femtosecond x-ray pulses with narrow bandwidth and unprecedented peak brightness. Special modes of operation have been developed to deliver double pulses for x-ray pump, x-ray probe experiments. However, the longest delay between the two pulses achieved with existing single bucket methods is less than 1 picosecond, thus preventing the exploration of longer time-scale dynamics. We present a novel two-bucket scheme covering delays from 350 picoseconds to hundreds of nanoseconds in discrete steps of 350 picoseconds. Performance for each pulse can be similar to the one in a single pulse operation. The method has been experimentally tested with the Linac Coherent Light Source (LCLS-I) and the copper linac with LCLS-II hard x-ray undulators.

Mesoscale imperfections, such as pores and voids, can strongly modify the properties and the mechanical response of materials under extreme conditions. Tracking the material response and microstructure evolution during void collapse is crucial for understanding its performance. In particular, imperfections in the ablator materials, such as voids, can limit the efficiency of the fusion reaction and ultimately hinder ignition. To characterize how voids influence the response of materials during dynamic loading and seed hydrodynamic instabilities, we have developed a tailored fabrication procedure for designer targets with voids at specific locations. Our procedure uses SU-8 as a proxy for the ablator materials and hollow silica microspheres as a proxy for voids and pores. By using photolithography to design the targets' geometry, we demonstrate precise and highly reproducible placement of a single void within the sample, which is key for a detailed understanding of its behavior under shock compression. This fabrication technique will benefit high-repetition rate experiments at x-ray and laser facilities. Insight from shock compression experiments will provide benchmarks for the next generation of microphysics modeling.

Inertial confinement fusion (ICF) holds increasing promise as a potential source of abundant, clean energy, but has been impeded by defects such as micro-voids in the ablator layer of the fuel capsules. It is critical to understand how these micro-voids interact with the laser-driven shock waves that compress the fuel pellet. At the Matter in Extreme Conditions (MEC) instrument at the Linac Coherent Light Source (LCLS), we utilized an x-ray pulse train with ns separation, an x-ray microscope, and an ultrafast x-ray imaging (UXI) detector to image shock wave interactions with micro-voids. To minimize the high- and low-frequency variations of the captured images, we incorporated principal component analysis (PCA) and image alignment for flat-field correction. After applying these techniques we generated phase and attenuation maps from a 2D hydrodynamic radiation code (xRAGE), which were used to simulate XPCI images that we qualitatively compare with experimental images, providing a one-to-one comparison for benchmarking material performance. Moreover, we implement a transport-of-intensity (TIE) based method to obtain the average projected mass density (areal density) of our experimental images, yielding insight into how defect-bearing ablator materials alter microstructural feature evolution, material compression, and shock wave propagation on ICF-relevant time scales.

Many questions regarding dynamic materials could be answered by using time-resolved ultra-fast imaging techniques to characterize the physical and chemical behavior of materials in extreme conditions and their evolution on the nanosecond scale. In this work, we perform multi-frame phase-contrast imaging (PCI) of micro-voids in low density polymers under laser-driven shock compression. At the Matter in Extreme Conditions (MEC) Instrument at the Linac Coherent Light Source (LCLS), we used a train of four x-ray free electron laser (XFEL) pulses to probe the evolution of the samples. To visualize the void and shock wave interaction, we deployed the Icarus V2 detector to record up to four XFEL pulses, separated by 1-3 nanoseconds. In this work, we image elastic waves interacting with the micro-voids at a pressure of several GPa. Monitoring how the material’s heterogeneities, like micro-voids, dictate its response to a compressive wave is important for benchmarking the performances of inertial confinement fusion energy materials. For the first time in a single sample, we have combined an ultrafast x-ray framing camera and four XFEL pulse train to create an ultrafast movie of micro-void evolution under laser-driven shock compression. Eventually, we hope this technique will resolve the material density as it evolves dynamically under laser shock compression.

X-ray Free Electron Lasers provide femtosecond X-ray pulses with narrow bandwidth and unprecedented peak brightness. Special modes of operation have been developed to deliver double pulses for X-ray pump, X-ray probe experiments. However, the longest delay between the two pulses achieved with existing single bucket methods is less than 1 picosecond, thus preventing exploration of longer timescales dynamics. We present a novel Two-bucket scheme covering delays from 350 picoseconds to hundreds of nanoseconds in discrete steps of 350 picoseconds. Performance for each pulse can be similar to the one in single pulse operation. The method has been experimentally tested with LCLS-I and LCLS-II hard x-ray undulators.

X-ray free-electron lasers (XFELs) enable obtaining novel insights in structural biology. The recently available MHz repetition rate XFELs allow full data sets to be collected in shorter time and can also decrease sample consumption. However, the microsecond spacing of MHz XFEL pulses raises new challenges, including possible sample damage induced by shock waves that are launched by preceding pulses in the sample-carrying jet. We explored this matter with an X-ray-pump/X-ray-probe experiment employing haemoglobin microcrystals transported via a liquid jet into the XFEL beam. Diffraction data were collected using a shock-wave-free single-pulse scheme as well as the dual-pulse pump-probe scheme. The latter, relative to the former, reveals significant degradation of crystal hit rate, diffraction resolution and data quality. Crystal structures extracted from the two data sets also differ. Since our pump-probe attributes were chosen to emulate EuXFEL operation at its 4.5 MHz maximum pulse rate, this prompts concern about such data collection.

Shock waves launched by x-ray pulses in sample-carrying liquid jets may affect protein crystallography data collected at MHz repetition rate x-ray free-electron laser (XFEL) facilities, by damaging the crystals before they are probed. We investigated the shock damage in lysozyme microcrystals using a double-pulse operation mode at a low repetition rate x-ray laser facility. The double-pulse mode generated shock waves with pressures that covered and exceeded the shock pressures expected at MHz pulse rate experiments at the European XFEL (EuXFEL) x-ray laser. The quality of the x-ray diffraction data from the crystals was degraded after the shock passed. A decrease in the number of peaks and in the resolution occurred above an estimated shock pressure threshold on the order of tens of MPa. Based on the scaling of the shock pressure with the sample injection parameters and the pulse rates, this threshold was not reached in initial EuXFEL experiments performed at pulse rates of 1.1 MHz but may be exceeded at the maximum pulse rate of 4.5 MHz. The observation of shock damage in lysozyme crystals indicates how experiments can be designed to rapidly detect, and eventually avoid, shock damage in other crystals. Our analysis of shock pressures in liquid jets can also be used to estimate the effect of the shocks in other types of experiments at MHz repetition rate XFELs.

We report the demonstration of optical compression of an electron beam and the production of controllable trains of femtosecond, soft x-ray pulses with the Linac Coherent Light Source (LCLS) free-electron laser (FEL). This is achieved by enhanced self-amplified spontaneous emission with a 2  μm laser and a dechirper device. Optical compression was achieved by modulating the energy of an electron beam with the laser and then compressing with a chicane, resulting in high current spikes on the beam which we observe to lase. A dechirper was then used to selectively control the lasing region of the electron beam. Field autocorrelation measurements indicate a train of pulses, and we find that the number of pulses within the train can be controlled (from 1 to 5 pulses) by varying the dechirper position and undulator taper. These results are a step toward attosecond spectroscopy with x-ray FELs as well as future FEL schemes relying on optical compression of an electron beam.

With an ultrafast framing camera, we image the propagation of a shock wave on the nanosecond time-scale. Four frame x-ray phase-contrast radiographs are acquired using the pulse train from an x-ray free electron laser.

we will review spatio-temporally tailored laser-electron interactions that enhance linear accelerator and free electron laser brightness to advance ultrafast X-ray spectroscopies.

we will review recent advances exploiting laser-particle interactions to enhance the performance of accelerators and X-ray free electron lasers and their applications in ultrafast science.

We present the new drive laser system for the photo-injector of the LCLS-II XFEL at SLAC, including the first commissioning results and challenges encountered due to high power, high repetition rate ultraviolet laser operation.

We present two laser heater shaping solutions based on Laguerre-Gaussian and discrete beamlet array distributions that significantly outperform current microbunching instability suppression approaches in free-electron lasers.

We report on the use of a Laguerre-Gaussian transverse mode in the LCLS laser heater resulting in better suppression of microbunching instability. We discuss the impact on FEL performance. © 2019 The Author(s)

The microbunching instability is known to be detrimental to x-ray free electron laser performance. At the Linear Coherent Light Source, the microbunching instability is suppressed with a laser heater, which increases the uncorrelated energy spread of e-beam in the injector. While the current system has been shown to improve x-ray brightness, other laser architectures could further enhance performance. In this study, we model the interaction between a laser and e-beam with arbitrary transverse profiles and examine the effect of various laser designs on the energy distribution of the electrons after the injector and laser heater, as well as their ability to suppress microbunching instability. This simulation incorporates random transverse jitter in order to reproduce physically representative operation of the Linac Coherent Light Source. We compare Gaussian and Laguerre-Gaussian modes, and explore composite beams in the form of an array of Gaussian beamlets. We conclude that the Gaussian laser profile is highly susceptible to e-beam ellipticity and random transverse jitter. The Laguerre-Gaussian profile, a mathematically ideal solution to suppressing microbunching, is less susceptible to these effects and can provide effective suppression even with a distorted e-beam, though performance can be improved by increasing stabilization. The array of beamlets presents a solution that produces consistent and smooth energy distributions with significantly less variance in heating than the Laguerre-Gaussian profile.