Summary We present results of the second experiment on the chemical identification of element 112. Similar to the first test in 2000, we aimed at the production of the spontaneously fissioning 283112 nuclei with T 1/2≈3min. A natU3O8 (with some Nd) target, 2mg of U/cm2 thick, was bombarded with 233-MeV 48Ca ions (the energy in the middle of the target layer). The nuclei recoiling from the target were thermalized in flowing helium. The target chamber was connected through a 25m long capillary to detectors of α-particles and fission fragments. All the equipment and detectors were kept at ambient temperature. According to the test experiments, of all the heavy elements produced in the bombardment, only Hg, Rn and At could be transported to the detectors. The first detecting device was similar to that used earlier – an assembly of 8 pairs of PIPS detectors coated with gold. Here one would observe the decay of element 112 atoms if they like Hg adsorbed on gold. The atoms which were not retained and freely passed through the PIPS detectors entered a new, flow-through ionization chamber, 5000 cm3 in volume, optimized for detecting fission fragments. The PIPS detectors and the ionization chamber were placed inside a large assembly of 3He – filled neutron counters to detect prompt neutrons from the fission events. In 22.5 days, a beam dose of 2.8×1018 ions was accumulated. More than 95 of the simultaneously produced α-active 185Hg (T 1/2=49 s) were found deposited already on the first pair of PIPS detectors; meanwhile, all the PIPSs did not detect any fission event. In the ionization chamber, eight fission events were observed in coincidence with neutron counts while the expected background was insignificant. Hence, the spontaneous fissions of the volatile activity can be conclusively attributed to the decay of element 112 produced in the fusion reaction 48Ca+ 238U, and formerly observed in Dubna physical experiments. Evaluation of the experimental data in terms of the adsorption enthalpies indicates much weaker interaction of element 112 with Au than that of Hg. One can conclude that in the given chemical environment, element 112 behaves like Rn rather than like Hg. The formation cross section of 283112 estimated from the data amounts to several pb. The experiments were carried out at the Flerov Laboratory of Nuclear Reactions at JINR in November–December 2001.
The first attempt to chemically identify one of the recently discovered long-lived isotopes of superheavy elements, namely 283112 (3 min, SF), made at FLNR, Dubna is reported. The nuclide was produced by fusion of accelerated 48Ca with a target of natural U, which contained some Nd to simultaneously produce also short-lived Hg nuclides. According to test experiments with Hg, the expected lighter homologue of element 112, both elements can be isolated from the products of the bombardment in metallic state, and transported from the target in flowing He gas to a detection system, where spontaneous fission and alpha decays 49-s 185Hg) were registered using PIPS detectors. The surface of the detectors was covered with a thin layer of Au or Pd which ensured the detection of Hg with high efficiency due to its chemisorption on these surfaces. While about three SF events could be expected, not a single one was detected at an upper limit for the production cross section of about one picobarn. This may point to a "Rn-like" rather than "Hg-like" behavior of element 112. A new experiment is planned, in which both a "Rn-like" and a "Hg-like" species could be detected.
The 4π-fragment-spectrometer FOBOS developed for heavy-ion research at beam energies of 10–100 AMeV has been commissioned for physical experiments at the Flerov Laboratory of Nuclear Reactions of the Joint Institute for Nuclear Research in Dubna. Based on the logarithmic detector principle, it is able to register charged fragments from protons up to heavy residual nuclei in a large dynamical range. Position-sensitive avalanche counters, axial ionization chambers and CsI(Tl) scintillation detectors are arranged in three concentric detector shells. An array of phoswich detectors is used as a more granular forward detector at narrow polar angles. The modular concept of FOBOS allows for different experimental application in the field of exclusive fragment spectroscopy at medium multiplicities. For illustration, the fragment spectroscopy studies concerning the spontaneous fission process and the fragmentation of hot nuclei by means of the FOBOS set-up are considered.
The 4π-fragment-spectrometer FOBOS developed for heavy-ion research at beam energies of 10–100 AMeV has been commissioned for physical experiments at the Flerov Laboratory of Nuclear Reactions of the Joint Institute for Nuclear Research in Dubna. Based on the logarithmic detector principle, it is able to register charged fragments from protons up to heavy residual nuclei in a large dynamical range. Position-sensitive avalanche counters, axial ionization chambers and CsI(Tl) scintillation detectors are arranged in three concentric detector shells. An array of phoswich detectors is used as a more granular forward detector at narrow polar angles. The modular concept of FOBOS allows for different experimental application in the field of exclusive fragment spectroscopy at medium multiplicities. For illustration, the fragment spectroscopy studies concerning the spontaneous fission process and the fragmentation of hot nuclei by means of the FOBOS set-up are considered.
The projectile-like fragment Separator COMBAS is being designed at the Flerov Laboratory of Nuclear Reactions, JiNR Dubna, for providing radioactive nuclear beams. COMBAS is a compact achromatic beam line with a high resolving power of 4360. It accepts fragments within 6.4 msr solid angle and with a momentum spread of 10%. The method of isotopic Separation is based on a combination of magnetic rigidity and energy loss analysis. The sepürated radioactive bearn is planned to be transported either into a time-projection charnber in the regime gas target - gas detector or to a secondary target positioned in the centre of the FOBOS 4n-array or to another Set-up. The FOBOS detector is intended for heavy ion reaction studies in the bombarding energy range of 10-100 AMeV at the cyclotron U-400M of the FLNR. Presently, only pnmary cyclotron beams are used because COMBAS is not yet complete. FOBOS consists of a gas-detector bali of 30 position-sensitive avalanche counters and 30 axial ionization chambers behind them and an outer scintillator shell of 210 CsI(T1) counters surrounding the gas detectors. An array of 96 phoswich counters Covers the very forward angles. All charged reaction products can be measured in a wide dynamic range and in a geometq covering a substantial part of 4n. First data have ben taken concerning kission and emission 0f intermediate-mass fragmenis in the reactions 'Li (43 AMeV) on 232~11 and 14~ (34 AMeV) Ig7~u.