We report large Lande g-factors observed in PbTe-Pb hybrid nanowires. The g-factor can reach 83, significantly larger than those in bare PbTe nanowires (typically below 20). We attribute this enhancement to orbital effects in the superconducting film, particularly when the magnetic field is nearly perpendicular to the Pb film. This enhancement is beneficial for the search for topological superconductivity by reducing the critical magnetic field required for the phase transition.
We investigate the anisotropic behaviors in PbTe and PbTe-Pb hybrid nanowires. In previous studies on PbTe, wire-to-wire variations in anisotropy indicate significant device disorder, posing a serious challenge for applications. Here, we achieve reproducible anisotropy in PbTe nanowires through a substantial reduction of disorder. We then couple PbTe to a superconductor Pb, and observe a pronounced deviation in the anisotropy behavior compared to bare PbTe nanowires. This deviation is gate tunable and attributed to the spin-orbit interaction and orbital effect, controlled by charge transfer between Pb and PbTe. These results provide guidance for the controlled engineering of exotic quantum states in this hybrid material platform.
Material challenges are the key issue in Majorana research, where surface disorder constrains device performance. Here, we tackle this challenge by embedding PbTe nanowires within a lattice-constant-matched crystal. The wire edges are shaped by self-organized growth instead of lithography, resulting in nearly atomically flat facets along both cross-sectional and longitudinal directions. Quantized conductance is observed at zero magnetic field with channel lengths maximally reaching 1.7 μm, significantly surpassing the state-of-the-art III-V nanowires (an order-of-magnitude improvement compared to InSb). Coupling PbTe to a Pb film unveils a flat interface spanning micrometers and a large superconducting gap of 1 meV. Our result not only represents a stride toward meeting the stringent low-disorder requirement for Majoranas, but may also open the door to various hybrid quantum devices requiring a low level of disorder.
Clean one-dimensional electron systems can exhibit quantized conductance. The plateau conductance doubles if the transport is dominated by Andreev reflection. Here, we report quantized conductance observed in both Andreev and normal-state transports in PbTe-Pb and PbTe-In hybrid nanowires. The Andreev plateau is observed at 4e^2/h, twice of the normal plateau value of 2e^2/h. In comparison, Andreev conductance in the best-optimized III-V nanowires is non-quantized due to mode-mixing induced dips (a disorder effect), despite the quantization of normal-state transport. The negligible mode mixing in PbTe hybrids indicates an unprecedented low-disorder transport regime for nanowire devices, beneficial for Majorana researches.
We report the realization of epitaxial indium thin films on PbTe nanowires. The film is continuous and forms an atomically sharp interface with PbTe. Tunneling devices reveal a hard superconducting gap. The gap size, 1.08- 1.18 meV, is twice as large as bulk indium's ('0.5 meV), due to the presence of PbTe. A similar enhancement is also observed in the critical temperature of In on a PbTe substrate. Subgap peaks appear at finite magnetic fields. The effective g factor (15-45) is notably enhanced compared to bare PbTe wires (<10) due to the presence of In, differing from Al hybrids. Josephson devices exhibit gate-tunable supercurrents. The PbTe-In hybrid enhances the properties of both the superconductivity of In and g factors of PbTe, and thus may enable exotic phases of matter such as topological superconductivity.
Semiconductor nanowires coupled to a superconductor provide a powerful testbed for quantum device physics such as Majorana zero modes and gate-tunable hybrid qubits. The performance of these quantum devices heavily relies on the quality of the induced superconducting gap. A hard gap, evident as vanishing subgap conductance in tunneling spectroscopy, is both necessary and desired. Previously, a hard gap has been achieved and extensively studied in III-V semiconductor nanowires (InAs and InSb). In this study, we present the observation of a hard superconducting gap in PbTe nanowires coupled to a superconductor Pb. The gap size ($\Delta$) is $\sim$ 1 meV (maximally 1.3 meV in one device). Additionally, subgap Andreev bound states can also be created and controlled through gate tuning. Tuning a device into the open regime can reveal Andreev enhancement of the subgap conductance, suggesting a remarkable transparent superconductor-semiconductor interface, with a transparency of $\sim$ 0.96. These results pave the way for diverse superconducting quantum devices based on PbTe nanowires.
Degeneracy and symmetry have a profound relation in quantum systems. Here, we report gate-tunable subband degeneracy in PbTe nanowires with a nearly symmetric cross-sectional shape. The degeneracy is revealed in electron transport by the absence of a quantized plateau. Utilizing a dual gate design, we can apply an electric field to lift the degeneracy, reflected as emergence of the plateau. This degeneracy and its tunable lifting were challenging to observe in previous nanowire experiments, possibly due to disorder. Numerical simulations can qualitatively capture our observation, shedding light on device parameters for future applications.
Network structures by semiconductor nanowires hold great promise for advanced quantum devices, especially for applications in topological quantum computing. In this study, we created networks of PbTe nanowires arranged in loop configurations. Using shadow-wall epitaxy, we defined superconducting quantum interference devices (SQUIDs) using the superconductor Pb. These SQUIDs exhibit oscillations in supercurrent upon the scanning of a magnetic field. Most of the oscillations can be fitted assuming a sinusoidal current-phase relation for each Josephson junction. Under certain conditions, the oscillations are found to be skewed, suggesting possible deviation from a sinusoidal behavior. Our results highlight the potential of PbTe nanowires for building complex quantum devices in the form of networks.
Planar Josephson junctions are predicted to host Majorana zero modes. The material platforms in previous studies are two dimensional electron gases (InAs, InSb, InAsSb and HgTe) coupled to a superconductor such as Al or Nb. Here, we introduce a new material platform for planar JJs, the PbTe-Pb hybrid. The semiconductor, PbTe, was grown as a thin film via selective area epitaxy. The Josephson junction was defined by a shadow wall during the deposition of the superconductor Pb. Scanning transmission electron microscopy reveals a sharp semiconductor-superconductor interface. Gate-tunable supercurrent and multiple Andreev reflections are observed. A perpendicular magnetic field causes interference patterns of the switching current, exhibiting Fraunhofer-like and SQUID-like behaviors. We further demonstrate a prototype device for Majorana detection, wherein phase bias and tunneling spectroscopy are applicable.
We study a gate-tunable superconducting qubit (gatemon) based on a thin InAs-Al hybrid nanowire. Using a gate voltage to control its Josephson energy, the gatemon can reach the strong coupling regime to a microwave cavity. In the dispersive regime, we extract the energy relaxation time T 1 ∼ 0.56 μs and the dephasing time T 2 * ∼ 0.38 μs. Since thin InAs-Al nanowires can have fewer or single sub-band occupation and recent transport experiment shows the existence of nearly quantized zero-bias conductance peaks, our result holds relevancy for detecting Majorana zero modes in thin InAs-Al nanowires using circuit quantum electrodynamics.
Electron interactions in quantum devices can exhibit intriguing phenomena. One example is assembling an electronic device in series with an on-chip resistor. The quantum laws of electricity of the device are modified at low energies and temperatures by dissipative interactions induced by the resistor, a phenomenon known as the dynamical Coulomb blockade (DCB). The DCB strength is usually nonadjustable in a fixed environment defined by the resistor. Here, we design an on-chip circuit for InAs-Al hybrid nanowires where the DCB strength can be gate-tuned in situ. InAs-Al nanowires could host Andreev or Majorana zero-energy states. This technique enables tracking the evolution of the same state while tuning the DCB strength from weak to strong. We observe the transition from a zero-bias conductance peak to split peaks for Andreev zero-energy states. Our technique opens the door to in situ tuning interaction strength on zero-energy states.
This repository contains the raw data and processing Python scripts corresponding to the paper "Conductance Quantization in PbTe Nanowires"
Semiconductor-superconductor hybrid nanowires are a leading material platform for the realization of Majorana zero modes. The semiconductors in previous studies are dominantly InAs or InSb. In this work, we show the induced superconductivity in a PbTe nanowire epitaxially coupled to a superconductor Pb. The Josephson junction device based on this hybrid reveals a gate-tunable supercurrent in the open regime and a hard superconducting gap in the tunneling regime. By demonstrating the superconducting proximity effect, our result can enable Majorana searches and other applications like gate-tunable qubits in a new semiconductor system.
This repository contains the raw data and processing code of the paper "Hard superconducting gap in PbTe nanowires".
Disorder is the primary obstacle in the current Majorana nanowire experiments. Reducing disorder or achieving ballistic transport is thus of paramount importance. In clean and ballistic nanowire devices, quantized conductance is expected, with plateau quality serving as a benchmark for disorder assessment. Here, we introduce ballistic PbTe nanowire devices grown by using the selective-area-growth (SAG) technique. Quantized conductance plateaus in units of 2e2/h are observed at zero magnetic field. This observation represents an advancement in diminishing disorder within SAG nanowires as most of the previously studied SAG nanowires (InSb or InAs) have not exhibited zero-field ballistic transport. Notably, the plateau values indicate that the ubiquitous valley degeneracy in PbTe is lifted in nanowire devices. This degeneracy lifting addresses an additional concern in the pursuit of Majorana realization. Moreover, these ballistic PbTe nanowires may enable the search for clean signatures of the spin-orbit helical gap in future devices.
Topological quantum computing is based on braiding of Majorana zero modes encoding topological qubits. A promising candidate platform for Majorana zero modes is semiconductor-superconductor hybrid nanowires. The realization of topological qubits and braiding operations requires scalable and disorder-free nanowire networks. Selective area growth of in-plane InAs and InSb nanowires, together with shadow-wall growth of superconductor structures, have demonstrated this scalability by achieving various network structures. However, the noticeable lattice mismatch at the nanowire-substrate interface, acting as a disorder source, imposes a serious obstacle along with this roadmap. Here, combining selective area and shadow-wall growth, we demonstrate the fabrication of PbTe-Pb hybrid nanowires - another potentially promising Majorana system - on a nearly perfectly lattice-matched substrate CdTe, all done in one molecular beam epitaxy chamber. Transmission electron microscopy shows the single-crystal nature of the PbTe nanowire and its atomically sharp and clean interfaces to the CdTe substrate and the Pb overlayer, without noticeable inter-diffusion or strain. The nearly ideal interface condition, together with the strong screening of charge impurities due to the large dielectric constant of PbTe, hold promise towards a clean nanowire system to study Majorana zero modes and topological quantum computing.
Electron interactions in quantum devices can exhibit intriguing phenomena. One example is assembling an electronic device in series with an on-chip resistor. The quantum laws of electricity of the device is modified at low energies and temperatures by dissipative interactions from the resistor, a phenomenon known as dynamical Coulomb blockade (DCB). The DCB strength is usually non-adjustable in a fixed environment defined by the resistor. Here, we design an on-chip circuit for InAs-Al hybrid nanowires where the DCB strength can be gate-tuned in situ. InAs-Al nanowires could host Andreev or Majorana zero-energy states. This technique enables tracking the evolution of the same state while tuning the DCB strength from weak to strong. We observe the transition from a zero-bias conductance peak to split peaks for Andreev zero-energy states. Our technique opens the door to in situ tuning interaction strength on zero-energy states.
We report phase coherent electron transport in PbTe nanowire networks with a loop geometry. Magnetoconductance shows Aharonov-Bohm (AB) oscillations with periods of h/e and h/2e in flux. The amplitudes of h/2e oscillations are enhanced near zero magnetic field, possibly due to interference between time-reversal paths. Temperature dependence of the AB amplitudes suggests a phase coherence length similar to 8-12 mu m at 50 mK. This length scale is larger than the typical geometry of PbTe-based hybrid semiconductor-superconductor nanowire devices.
Inspired by a recent experiment [Phys. Rev. Lett. 122 253201(2019)] that an unprecedented quantum interference was observed in the way of stimulated Raman adiabatic passage (STIRAP) due to the coexisting resonant- and detuned-STIRAPs, we comprehensively study this effect. Our results uncover the scheme robustness towards any external-field fluctuations coming from laser intensity noise and imperfect resonance condition, as well as the persistence of high-contrast interference pattern even when more nearby excited levels are involved. We verify that an auxiliary dynamical phase accumulated in hold time caused by the presence of the quasi-dark state in detuned-STIRAP can sensitively manipulate the visibility and frequency of the interference pattern, representing a new hallmark to measure the hyperfine energy accurately. The robust stability of the scheme comes from the intrinsic superiority embedded in the STIRAP mechanism that preserves the coherence of population transfer, which promises a remarkable performance of quantum interference in a practical implementation.
Inspired by a recent experiment [Phys. Rev. Letts. \textbf{122}, 253201(2019)] that an unprecedented quantum interference was observed in the way of Stimulated Raman adiabatic passage (STIRAP) due to the coexisting resonant- and detuned-STIRAPs, we comprehensively study this effect for uncovering its robustness towards the external-field fluctuations of laser noise, imperfect resonance condition as well as the excited-state decaying. We verify that, an auxiliary dynamical phase accumulated in hold time caused by the quasi-dark state can sensitively manipulate the visibility and frequency of the interference fringe, representing a new hallmark to measure the hyperfine energy accurately. The robust stability of scheme comes from the intrinsic superiority embedded in STIRAP itself, which promises a remarkable preservation of the quantum interference quality in a practical implementation.