Nonrelativistic magnon chiral splitting in altermagnets has garnered significant recent attention. In this Letter, we demonstrate that nonlinear three-wave mixing-where magnons split or coalesce-extends this phenomenon into unprecedented relativistic regimes. Employing a bilayer antiferromagnet with Dzyaloshinskii-Moriya interactions, we identify three distinct classes of chiral splitting, each dictated by specific symmetries, such as C_{4}T, σ_{v}T, or their combination. This reveals a novel bosonic mechanism for symmetry-protected chiral splitting, capitalizing on the unique ability of magnons to violate particle-number conservation, a feature absent in low-energy fermionic systems. Our findings pave the way for engineering altermagnetic splitting, with potential applications in advanced magnonic devices and deeper insights into magnon dynamics in complex magnetic systems.
Van der Waals magnetic materials have shown fascinating natural ferromagnetic properties at the atomic level, which has great potential in fields of low power spintronics, quantum computing and optical communication. Herein, we verify perpendicular magnetic anisotropy at room temperature in Fe3GaTe2 (FGT) nanosheet and a robust anomalous Hall effect (AHE) over a wide temperature range (3 K similar to 380 K) and across magnetic field angles of 0 degrees similar to 90 degrees using a standard Hall bar device. Particularly, we realize the reversible magnetic-domain switching and observe the nucleation and expansion of the labyrinth domains in approximately 128.8 nm-thick FGT by polar magneto-optical Kerr effect (MOKE) measurements. The above-mentioned experimental results suggest the strong tunability of the AHE and the thickness-dependent evolution of magnetic domains, establishing a fundamental basis for the design of non-volatile magnetic domain memory devices based on FGT.
Breaking the intrinsic chiral symmetry of massless Dirac fermions in graphene at the two inequivalent valleys gives rise to rich intriguing phenomena. A prototypical example of this is the Kekulé order. Here, we use STM to directly visualize the bond texture associated with Kekulé spiral order in graphene. The Kekulé order originates from the intervalley scattering at 1D grain boundaries, and its strength can be significantly suppressed when a periodic potential is applied. By mapping atomic-scale electronic wave functions, we uncover that the bond texture localized near the 1D boundaries exhibits a complex spatial dependence indicative of phase winding, and it evolves dramatically with electronic energy. Our local-probe measurements thus establish the emergence of Kekulé spiral order in graphene, highlighting topological defects as versatile building blocks for engineering valley-ordered phases.
We propose to realize the quantum nonlinear Hall effect and the inverse Faraday effect through the acoustic wave in a time-reversal invariant but inversion broken Dirac insulator. We focus on the acoustic frequency much lower than the Dirac gap such that the interband transition is suppressed and these effects arise solely from the intrinsic valley-contrasting band topology. The corresponding acoustoelectric conductivity and magnetoacoustic susceptibility are both proportional to the quantized valley Chern number and independent of the quasiparticle lifetime. The linear and nonlinear components of the longitudinal and transverse topological currents can be tuned by adjusting the polarization and propagation directions of the surface acoustic wave. The static magnetization generated by a circularly polarized acoustic wave scales linearly with the acoustic frequency as well as the strain-induced charge density. Our results unveil a quantized nonlinear topological acoustoelectric response of gapped Dirac materials, like hexagonal boron nitride and transition-metal dichalcogenide, paving the way toward room-temperature acoustoelectric devices due to their large band gaps.
We develop a quantitative theory of phonon magnetic moment in doped Dirac semimetals. Our theory is based on an emergent gauge field approach to the electron-phonon coupling, applicable to gapless systems. We find that the magnetic moment is directly proportional to the electrical Hall conductivity through the phonon Hall viscosity. Our theory is combined with the first-principles calculations, allowing us to quantitatively implement it to realistic materials. Magnetic moments are found to be of the order of a Bohr magneton for Raman-active phonon modes in graphene and Cd3As2. Our results provide practical guidance for the dynamical generation of large magnetization in quantum materials.
The recent experimental discovery of the zero-field fractional Chern insulator (FCI) in twisted $\mathrm{MoTe_2}$ moir\'e superlattices has sparked immense interest in this exotic topological quantum state. The FCI has also been observed in previous experiments in magic angle twisted bilayer graphene (TBG) under a finite magnetic field of about 5 Tesla. Generally, the stabilization of FCI requires fine-tuning the topological band to satisfy certain conditions. It would still be helpful to have an intuitive picture to understand the different behaviors in twisted $\mathrm{MoTe_2}$ and TBG. Here, we compare them through the lens of emergent gauge fields. In TBG, the system can be mapped to two Dirac fermions coupled to emergent gauge fields with opposite signs. In contrast, the twisted $\mathrm{MoTe_2}$ reduces to a hole with parabolic dispersion coupled to an emergent gauge field. This contrasting gauge structure provides a new perspective on the observed difference: the zero-field FCI is stable in $\mathrm{MoTe_2}$ but absent in TBG. Based on this understanding, we will explore potential strategies for stabilizing FCI in both moir\'e superlattices.
Understanding the interplay of interaction and disorder in quantum transport poses long-standing scientific challenges for theory and experiment. While highly controlled ultracold atomic platforms combining atomic interactions with spatially disordered lattices have led to remarkable advances, the extension of such controlled studies to phenomena in high-dimensional disordered systems, such as the three-dimensional Anderson metal-insulator transition has been limited. Kicked quantum gases provide an alternate experimental platform that captures the Anderson model in momentum space and features dynamical localization as the analog of Anderson localization. Here, we utilize a momentum space lattice platform using quasiperiodically kicked ultracold atomic gases to experimentally investigate interaction effects on the three-dimensional dynamical Anderson metal-insulator transition. We observe interaction-driven subdiffusion and a divergence of delocalization onset time on approaching the phase boundary. Mean-field numerical simulations show qualitative agreement with experimental observations, but with significant quantitative deviations.
Understanding the interplay of interactions and disorder in quantum transport poses long-standing scientific challenges, with many-body quantum transport phenomena in high-dimensional disordered systems remaining largely unexplored experimentally. We utilize a momentum space lattice platform using quasi-periodically kicked ultracold atomic gases to experimentally investigate many-body effects on the three-dimensional Anderson metal-insulator transition. We observe interaction-driven sub-diffusion and a divergence of delocalization onset time on approaching the many-body phase boundary. Mean-field numerical simulations are in qualitative agreement with experimental observations.
Transition metal dichalcogenide (TMDC) moiré superlattices, owing to the moiré flatbands and strong correlation, can host periodic electron crystals and fascinating correlated physics. The TMDC heterojunctions in the type-II alignment also enable long-lived interlayer excitons that are promising for correlated bosonic states, while the interaction is dictated by the asymmetry of the heterojunction. Here we demonstrate a new excitonic state, quadrupolar exciton, in a symmetric WSe2-WS2-WSe2 trilayer moiré superlattice. The quadrupolar excitons exhibit a quadratic dependence on the electric field, distinctively different from the linear Stark shift of the dipolar excitons in heterobilayers. This quadrupolar exciton stems from the hybridization of WSe2 valence moiré flatbands. The same mechanism also gives rise to an interlayer Mott insulator state, in which the two WSe2 layers share one hole laterally confined in one moiré unit cell. In contrast, the hole occupation probability in each layer can be continuously tuned via an out-of-plane electric field, reaching 100% in the top or bottom WSe2 under a large electric field, accompanying the transition from quadrupolar excitons to dipolar excitons. Our work demonstrates a trilayer moiré system as a new exciting playground for realizing novel correlated states and engineering quantum phase transitions.
Spin Hall effect (SHE), a fundamental transport phenomenon with non-zero spin current but vanishing charge current, has important applications in spintronics for the electrical control of spins. Owing to the half-spin nature of electrons, the rank of spin current (determined by the rank of spin tensors) has been restricted to 0 and 1 for charge and spin Hall effects. Motivated by recent studies of pseudospin-1 fermions in solid state and cold atomic systems, here we introduce and characterize higher-rank ($\geq 2$) SHEs in large spin ($\geq 1$) systems. We find a universal rank-2 spin Hall conductivity $e/{8}\pi $, with zero rank-0 and 1 conductivities, for a spin-1 model with intrinsic spin-orbit coupling. Similar rank-2 SHEs can also be found in a spin-3/2 system. An experimental scheme is proposed to realize and measure rank-2 SHEs with pseudospin-1 ultracold fermionic atoms. Our results reveal novel spin transport phenomena in large spin systems and may find important applications in designing innovative spintronic devices.
Moiré superlattices of semiconducting transition metal dichalcogenides enable unprecedented spatial control of electron wavefunctions, leading to emerging quantum states. The breaking of translational symmetry further introduces a new degree of freedom: high symmetry moiré sites of energy minima behaving as spatially separated quantum dots. We demonstrate the superposition between two moiré sites by constructing a trilayer WSe2/monolayer WS2 moiré heterojunction. The two moiré sites in the first layer WSe2 interfacing WS2 allow the formation of two different interlayer excitons, with the hole residing in either moiré site of the first layer WSe2 and the electron in the third layer WSe2. An electric field can drive the hybridization of either of the interlayer excitons with the intralayer excitons in the third WSe2 layer, realizing the continuous tuning of interlayer exciton hopping between two moiré sites and a superposition of the two interlayer excitons, distinctively different from the natural trilayer WSe2.
Moiré coupling in transition metal dichalcogenides (TMDCs) superlattices introduces flat minibands that enable strong electronic correlation and fascinating correlated states, and it also modifies the strong Coulomb-interaction-driven excitons and gives rise to moiré excitons. Here, we introduce the layer degree of freedom to the WSe2/WS2 moiré superlattice by changing WSe2 from monolayer to bilayer and trilayer. We observe systematic changes of optical spectra of the moiré excitons, which directly confirm the highly interfacial nature of moiré coupling at the WSe2/WS2 interface. In addition, the energy resonances of moiré excitons are strongly modified, with their separation significantly increased in multilayer WSe2/monolayer WS2 moiré superlattice. The additional WSe2 layers also modulate the strong electronic correlation strength, evidenced by the reduced Mott transition temperature with added WSe2 layer(s). The layer dependence of both moiré excitons and correlated electronic states can be well described by our theoretical model. Our study presents a new method to tune the strong electronic correlation and moiré exciton bands in the TMDCs moiré superlattices, ushering in an exciting platform to engineer quantum phenomena stemming from strong correlation and Coulomb interaction.
We demonstrate a generic mechanism to realize topological flat minibands by confining massive Dirac fermions in a periodic moir\'e potential, which can be achieved in a heterobilayer of transition metal dichalcogenides. We show that the topological phase can be protected by the symmetry of moir\'e potential and survive to arbitrarily large Dirac band gap. We take the MoTe$_2$/WSe$_2$ heterobilayer as an example and find that the topological phase can be driven by a vertical electric field. By projecting the Coulomb interaction onto the topological fat minibands, we identify a correlated Chern insulator at half filling and a quantum valley-spin Hall insulator at full filling which explains the topological states observed in the MoTe$_2$/WSe$_2$ in experiment. Our work clarifies the importance of Dirac structure for the topological minibands and unveils a general strategy to design topological moir\'e materials.
Contrary to a driven classical system that exhibits chaotic behaviour and diffusive energy growth, a kicked quantum system can exhibit the emergence of dynamical localization, which limits energy absorption and leads to the breakdown of ergodicity 1 – 4 . The evolution of dynamically localized states in the presence of many-body interactions has long remained an open question 5 – 7 . Here we experimentally study an interacting one-dimensional ultracold gas periodically kicked by a pulsed optical lattice and observe the interaction-driven emergence of dynamical delocalization and many-body quantum chaos. The observed dynamics feature sub-diffusive energy growth over a broad parameter range of interaction and kick strengths. These results shed light on interaction-driven transport phenomena in quantum many-body systems, in a regime where theoretical approaches are extremely challenging and provide conflicting predictions.
Two-dimensional moiré superlattices provide a highly tunable platform to study strongly correlated physics. In particular, the moiré superlattices of two-dimensional semiconductor heterojunctions have been shown to host tunable correlated electronic states such as a Mott insulator and generalized Wigner crystals 1 – 4 . Here we report the observation of an excitonic insulator 5 – 7 , a correlated state with strongly bound electrons and holes, in an angle-aligned monolayer WS 2 /bilayer WSe 2 moiré superlattice. The moiré coupling induces a flat miniband on the valence-band side only in the first WSe 2 layer interfacing WS 2 . The electrostatically introduced holes first fill this miniband and form a Mott insulator when the carrier density corresponds to one hole per moiré supercell. By applying a vertical electric field, we tune the valence band in the second WSe 2 layer to overlap with the moiré miniband in the first WSe 2 layer, realizing the coexistence of electrons and holes at equilibrium, which are bound as excitons due to a strong Coulomb interaction. We show that this new bound state is an excitonic insulator with a transition temperature as high as 90 K. Our study demonstrates a moiré system for the study of correlated many-body physics in two dimensions.
Contrary to a driven classical system that exhibits chaos phenomena and diffusive energy growth, a driven quantum system can exhibit dynamical localization that features energy saturation. However, the evolution of the dynamically localized state in the presence of many-body interactions has long remained an open question. Here we experimentally study an interacting 1D ultracold gas periodically kicked by a pulsed optical lattice, and observe the interaction-driven emergence of dynamical delocalization and many-body quantum chaos. The observed dynamics feature a sub-diffusive energy growth manifest over a broad parameter range of interaction and kick strengths, and shed light on an area where theoretical approaches are extremely challenging.
A vortex is a universal and significant phenomenon that has been known for centuries. However, creating vortices to the atomic limit has remained elusive. Very recently, it was demonstrated that intervalley scattering induced by the single carbon defect of graphene leads to phase winding over a closed path surrounding the defect. Motivated by this, we demonstrate that the single carbon defects at A and B sublattices of graphene can be regarded as pseudospin-mediated atomic-scale vortices with angular momenta l = +2 and -2, respectively. The quantum interference measurements of the vortices indicate that the vortices cancel each other, resulting in zero total angular momentum, in the |A| = |B| case, and they show aggregate chirality and angular momenta similar to a single vortex of the majority in the |A| ≠ |B| case, where |A| (|B|) is the number of vortices with angular momenta l = +2 (l = -2).
We demonstrate a generic mechanism to realize topological moir\'e minibands by considering a massive Dirac fermion moving in a moir\'e potential, which can be achieved in a heterobilayer of transition metal dichalcogenides. We take the MoTe$_2$/WSe$_2$ heterobilayer as an example and show that the topological phase can be driven by a vertical electric field due to the lattice corrugation. Thus a correlated Chern insulator can be stabilized by the Coulomb interaction that breaks the time-reversal symmetry spontaneously. Our work explains the recent experiment on the observation of Chern insulating state in the AB-stacked MoTe$_2$/WSe$_2$ and unveils a general strategy to design topological moir\'e materials.
Unusual magnetic textures can be stabilized in f -electron materials due to the interplay between competing magnetic interactions, complex Fermi surfaces, and crystalline anisotropy. Here we investigate CeAuSb 2 , an f -electron incommensurate antiferromagnet hosting both single- Q and double- Q spin textures as a function of magnetic fields ( H ) applied along the c axis. Experimentally, we map out the field-temperature phase diagram via electrical resistivity and thermal expansion measurements. Supported by calculations of a Kondo lattice model, we attribute the puzzling magnetoresistance enhancement in the double- Q phase to the localization of the electronic wave functions caused by the incommensurate magnetic texture.