Abstract—Spectral and temperature dependences of the magneto-optical transversal Kerr effect (TKE) of GaMnAs layers prepared by different methods are reported in this work. The GaMnAs layers prepared by pulsed laser sputtering at 300°С demonstrate a ferromagnetic behavior below 80 K, which is due to the presence of local ferromagnetic (Ga,Mn)As areas in the paramagnetic matrix. The Ga(In)MnAs layers prepared by ion implantation and subsequent pulsed laser annealing were found to exhibit a high TKE response at low temperatures. The presence of the characteristic band in the TKE spectrum in the range of transitions near the L point of the band structure of Ga(In)As confirms the intrinsic ferromagnetism. The temperature dependences of TKE measured for different spectrum ranges demonstrate nonmonotonic behavior, which indicates the magnetic inhomogeneity of the layers. The peculiarities of the magneto-optical spectra of GaMnAs, which were not observed previously, were explained by taking the magnetic and phase inhomogeneity of the layers into account. The sensitivity of TKE to the phase inhomogeneity of the Ga(In)MnAs layers and the efficiency of TKE in studying the electron spectrum and magnetic structure of diluted magnetic superconductors are demonstrated.
AbstractIn this paper, we present the results of studies of the spectral, temperature, and field dependences of the transversal Kerr effect in Ga_1 – _ x Mn_ x As ( x = 0.0066–0.033) layers produced by ion implantation and subsequent pulsed laser annealing. The complicated nonmonotonous nature of the temperature dependences of the transversal Kerr effect and its dependence on the measurement range indicate a magnetic inhomogeneity of the layers. The reasons for the inhomogeneity can be the Gaussian distribution of Mn over the thickness of the layers and the electron phase separation in them. The appearance of new features in the spectra of the transversal Kerr effect is explained by the presence in the doped semiconductor matrix of nanoregions with a higher carrier concentration and a higher Curie temperature and a shift of the Fermi level into the valence band leading to an increase in the energy of optical transitions.
In this paper, we present the results of studies of the spectral, temperature, and field dependences of the transversal Kerr effect in Ga1 – xMnxAs (x = 0.0066–0.033) layers produced by ion implantation and subsequent pulsed laser annealing. The complicated nonmonotonous nature of the temperature dependences of the transversal Kerr effect and its dependence on the measurement range indicate a magnetic inhomogeneity of the layers. The reasons for the inhomogeneity can be the Gaussian distribution of Mn over the thickness of the layers and the electron phase separation in them. The appearance of new features in the spectra of the transversal Kerr effect is explained by the presence in the doped semiconductor matrix of nanoregions with a higher carrier concentration and a higher Curie temperature and a shift of the Fermi level into the valence band leading to an increase in the energy of optical transitions.
GaMnAs layers grown by pulsed laser deposition were studied by magneto-optical transversal Kerr effect spectroscopy, spectral ellipsometry, resistivity and the Hall effect measurements, and magnetometry. The growth regimes for magnetically inhomogeneous layers containing Mn-enriched ferromagnetic regions with different composition and sizes were established. The layers grown at a temperature of 300°C exhibit a ferromagnetic behavior at temperatures below 80 K, which is conditioned by the presence of local ferromagnetic (Ga,Mn)As regions in the paramagnetic matrix. The nature of peculiarities in the TKE spectrum of these layers is discussed.
Ga-1 xMnxAs layers prepared by ion implantation and subsequent pulsed laser annealing with the planned Mn concentrations of x = 0.01-0.08 have been studied using the magneto-optical transversal Kerr effect (TKE) and spectral ellipsometry. The spectral dependences of the diagonal and nondiagonal components of the permittivity tensor (PT), as well as the spectrum of magnetic circular dichroism (MCD) have been calculated for the layers. The obtained spectra of the diagonal PT components show that the layers under study maintain the zinc-blende crystal structure of the parent GaAs semiconductor. All studied samples reveal a strong TKE response at low temperatures with a dependence of an effective Curie temperature (at which TKE appears) on the Mn concentration. A number of extrema in the low-temperature TKE and MCD spectra are close to the energies of transitions in the Gamma and L critical points of the parent semiconductor band structure that confirms the intrinsic ferromagnetism of the Ga-1 xMnxAs layers. The MCD spectra shape and its change with Mn concentration increasing are discussed on a base of the valence-band model of ferromagnetism in DMS. (C) 2017 Published by Elsevier B.V.
AbstractGaMnAs layers grown by pulsed laser deposition were studied by magneto-optical transversal Kerr effect spectroscopy, spectral ellipsometry, resistivity and the Hall effect measurements, and magnetometry. The growth regimes for magnetically inhomogeneous layers containing Mn-enriched ferromagnetic regions with different composition and sizes were established. The layers grown at a temperature of 300°C exhibit a ferromagnetic behavior at temperatures below 80 K, which is conditioned by the presence of local ferromagnetic (Ga,Mn)As regions in the paramagnetic matrix. The nature of peculiarities in the TKE spectrum of these layers is discussed.
The concentration, temperature, and magnetic-field dependences of the magnetoreflection and magnetotransmission of natural light in the infrared spectral range and the Kerr effect in single crystals of ferromagnetic Hg 1- x Cd x Cr 2 Se 4 (0 ⩽ x ⩽ 1) spinels have been studied. A relationship of the magneto-optical properties to the electronic band structure of spinels has been established. The most significant changes in the spectra of magnetoreflection, magnetotransmission, and the Kerr effect are shown to be observed for 0.1 < x < 0.25 and are attributable to a rearrangement of the band structure as the composition changes.
The research of magneto-optical properties has been conducted for the “Nanocomposite-bismuth telluride” (Co40Fe40B20)33.9(SiO2)66.1/[Te3Bi2] multilayer system at various thicknesses of each layer type. We report an enormous enhancement of magneto-optical (MO) response in this system. Besides, a good correlation between thickness dependences of transversal Kerr effect (TKE) and magneto-transport properties has been established. Such correlation was related to peculiarities of the interface forming process at the ferromagnetic (FM) granule boundaries. Moreover, this amplification of magneto-optical response is largest among the other spacer layers, such as Si, Cu, and C, therefore a comparison between them has been plotted.
GaMnAs layers fabricated on GaAs(001) substrates by laser ablation technique were studied using the magneto-optical transversal Kerr effect (TKE) (E = 0.5 - 4.0 eV) and spectral ellipsometry (E = 1.4 - 4.5 eV). Obtained spectral, temperature and magnetic field TKE dependences shown that the used technique allowed us to obtain ferromagnetic (Ga,Mn)As layers, whose composition was close to single-phase one (without MnAs inclusions). Spectral dependences of the off-diagonal components (e’ = e’1 - ie’2) of the permittivity tensor and also of the magnetic circular dichroism (MCD) were calculated for ferromagnetic (Ga,Mn)As sample. The calculated dependences were compared with the published magneto-optical spectra of (Ga,Mn)As layers grown by molecular beam epitaxy.
Magneto-optical spectra of polycrystalline samples of the Fe 48 Mn 24 Ga 28 Heusler alloy undergoing martensitic transformation from the high-temperature paramagnetic austenitic to ferromagnetic martensitic phase have been studied at 50–320 K in the transversal Kerr effect geometry. A comparison of magnetooptical spectra with data obtained in magnetic measurements has demonstrated that the martensitic transition on the surface of a sample and in its bulk takes place in the same temperature interval. Magnetic anisotropy has been found in the martensitic phase driven by large multidomain inclusions of martensite in austenite. The magneto-optical signal of Fe 48 Mn 24 Ga 28 differs strongly in spectral shape from that measured in Ni-Mn-Ga.
The presented work is devoted to the study of magneto-optical properties of «nanocomposite-semiconductor» ((Co40Fe40B20)33.9(SiO2)66.1/Te3Bi2)) multilayer structures. It has been found, that the adding of Te3Bi2 spacer regardless of composite’s compound increases a magneto-optical response and the amplification of it is the biggest among the other spacers such as Si, SiC and Cu. There has also been established a good correlation between thickness dependencies of magnetooptical (MO) and magnetotransport properties. This correlation is related to the peculiarities of interface forming at the «FM-granule - semiconductor» edge and to percolation process in multilayer structures.