A direct measurement of the ground-state-to-ground-state electron-capture decay Q (QEC) value of 97Tc has been conducted employing the high-resolving-power phase-imaging ion-cyclotron-resonance technique with the double Penning trap mass spectrometer JYFLTRAP. The resulting QEC value for 97Tc is 324.82(21) keV, exhibiting a precision approximately 19 times higher than the value adopted in the newest Atomic Mass Evaluation (AME2020) and differing by 1.2 sigma. Furthermore, by combining this refined Q value with nuclear energy-level data for the decay-daughter 97Mo, a potential ultralow Q-value transition 97Tc (9/2+, ground state) -> 97Mo & lowast; [320(1) keV] was detected. The ground-state-to-excited-state electron-capture decay Q value (Q & lowast;EC) of this transition was determined to be 4.8(10) keV, confirming it to be energetically allowed with a confidence level of exceeding 4 sigma. The captures of electrons occupying the L and higher shells for this transition are energetically allowed, giving a value of 2.0(10) keV for the closest distance of Q & lowast; EC to the allowed binding energy of the L1 shell. To predict partial half-lives and energy-release distributions for this transition, the atomic self-consistent many-electron Dirac-Hartree-Fock-Slater method and the nuclear shell model have been employed. Dominant correction terms such as exchange and overlap corrections, as well as shake-up and shake-off effects, were included in the final results. Moreover, in the case of a possible allowed transition, the normalized distribution of released energy in the electron-capture decay of 97Tc to the excited 320-keV state of 97Mo, is compared with that of 163Ho, which is being used for electron-neutrino-mass determination. A pseudoexperiment technique was introduced to calculate error propagation in half-life and the 68% confidence interval for normalized energy distributions.
High-precision mass measurements of exotic ^{95-97}Ag isotopes close to the N=Z line have been conducted with the JYFLTRAP double Penning trap mass spectrometer, with the silver ions produced using the recently commissioned inductively heated hot cavity catcher laser ion source at the Ion Guide Isotope Separator On-Line facility. The atomic mass of ^{95}Ag was directly determined for the first time. In addition, the atomic masses of β-decaying 2^{+} and 8^{+} states in ^{96}Ag have been identified and measured for the first time, and the precision of the ^{97}Ag mass has been improved. The newly measured masses, with a precision of ≈1 keV/c^{2}, have been used to investigate the N=50 neutron shell closure, confirming it to be robust. Empirical shell-gap and pairing energies determined with the new ground-state mass data are compared with the state-of-the-art ab initio calculations with various chiral effective field theory Hamiltonians. The precise determination of the excitation energy of the ^{96m}Ag isomer in particular serves as a benchmark for ab initio predictions of nuclear properties beyond the ground state, specifically for odd-odd nuclei situated in proximity to the proton dripline below ^{100}Sn. In addition, density functional theory calculations and configuration-interaction shell-model calculations are compared with the experimental results. All theoretical approaches face challenges to reproduce the trend of nuclear ground-state properties in the silver isotopic chain across the N=50 neutron shell and toward the proton dripline.
We report on new precision mass measurements of neutron-rich $^{137}$Sb and $^{136-142}$I isotopes from the JYFLTRAP double Penning trap mass spectrometer. We confirm the value from the previous Penning-trap measurement of $^{137}$Sb at the Canadian Penning Trap and therefore rule out the conflicting result from the Experimental Storage Ring. The ground state and isomer in $^{136}$I were resolved and measured directly for the first time. The isomer excitation energy, $E_x = 215.1(43)$ keV, agrees with the literature but is three times more precise. The measurements have improved the precision of the mass values and confirmed previous results in the majority of cases. However, for $^{138,140}$I the results differ by 17(6) keV and 23(12) keV, respectively. This could be explained by an unresolved contamination or different ratio of unresolved isomeric states in the case of $^{140}$I.
Superconducting (SC) tokamak JT-60SA plays an essential role in fusion research and development by supporting and complementing the ITER project, providing directions to the DEMO design activity and fostering next generation scientists and engineers. Since the short circuit incident at the terminal joints of equilibrium field coil #1 during the integrated commissioning (IC) in March 2021, both EU and JA implementing agencies (IAs) have examined how to ensure safe operation of JT-60SA by mitigating the risk of possible discharge occurrence inside the cryostat. Based on the experience of the global Paschen tests, the IAs have established a strategy of risk mitigation measures, which is a combination of (i) reinforcement of insulation, (ii) avoiding unnecessary voltage application to the coil systems and (iii) immediate de-energization of the coils when deteriorated vacuum conditions are detected. Thanks to the considerable efforts of the Integrated Project Team members, the IC restarted in May 2023. After confirmation of the SC state of the coil systems (TF, EF and CS), the coil energization test and the plasma operation phase 1 (OP-1) started. The first plasma was successfully achieved on 23 October 2023 with a limited value of voltage and current applied to the coils. The plasma configuration control was also confirmed with low plasma current and low auxiliary heating power conditions. Based on the IO-F4E-QST collaboration, activities of JT-60SA have been shared with the IO and provided an important lesson for ITER assembly and commissioning, and will provide an outstanding contribution to fusion research at large. After OP-1, maintenance & enhancement phase 1 (M/E-1) starts from January 2024, in which in-vessel components are installed, and heating and diagnostic systems are extensively upgraded to allow a high power heating experiment planned in OP-2. In order to make the best use of JT-60SA, a newly organized JT-60SA experiment team will refine the research plan for the future high heating power operation phase.
The absolute mass of ^84Sr was determined using the phase-imaging ion-cyclotron-resonance technique with the JYFLTRAP double Penning trap mass spectrometer. A more precise value for the mass of ^84Sr is essential for providing potential indications of physics beyond the Standard Model through high-precision isotope shift measurements of Sr atomic transition frequencies. The mass excess of ^84Sr was refined to be -80649.229(37) keV/c^2 from high-precision cyclotron-frequency-ratio measurements with a relative precision of 4.8× 10^-10 . The obtained mass-excess value is in agreement with the adopted value in the Atomic Mass Evaluation 2020, but is 30 times more precise. With this new value, we confirm the previously observed nonlinearity in the study of the isotope shift of strontium. Moreover, the double-beta ( 2β ^+ ) decay Q value of ^84Sr was directly determined to be 1790.115(37) keV, and the precision was improved by a factor of 30.
Isomers close to the doubly magic nucleus 78Ni (Z=28, N=50) provide essential information on the shell evolution and shape coexistence far from stability. The existence of a long-lived isomeric state in 76Cu has been debated for a long time. We have performed high-precision mass measurements of 76Cu with the JYFLTRAP double Penning trap mass spectrometer at the Ion Guide Isotope Separator On-Line facility and confirm the existence of such an isomeric state with an excitation energy Ex=64.8(25) keV. Based on the ratio of detected ground- and isomeric-state ions as a function of time, we show that the isomer is the shorter-living state previously considered as the ground state of 76Cu. The result can potentially change the conclusions made in previous works related to the spin-parity and charge radius of the 76Cu ground state. Additionally, the new 76Cu(n,γ) reaction Q-value has an impact on the astrophysical rapid neutron-capture process.
The first direct determination of the ground-state-to-ground-state β ^- -decay Q-value of ^77 As to ^77 Se was performed by measuring their atomic mass difference utilizing the double Penning trap mass spectrometer, JYFLTRAP. The resulting Q-value is 684.463(70) keV, representing a remarkable 24-fold improvement in precision compared to the value reported in the most recent Atomic Mass Evaluation (AME2020). With the significant reduction of the uncertainty of the ground-state-to-ground-state Q-value and knowledge of the excitation energies in ^77 Se from γ -ray spectroscopy, the ground-state-to-excited-state Q-value of the transition ^77 As (3/2 ^- , ground state) → ^77 Se ^* (5/2 ^+ , 680.1035(17) keV) was refined to be 4.360(70) keV. We confirm that this potential low Q-value β ^- -decay transition for neutrino mass determination is energetically allowed at a confidence level of about 60 σ . Nuclear shell-model calculations with two well-established effective Hamiltonians were used to estimate the partial half-life for the low Q-value transition. The half-life was found to be of the order of 10 ^9 years for this first-forbidden non-unique transition. Since the half-life of ^77 As is only ≈ 2 days, usage of it as source for rare-event experiments searching for the electron antineutrino mass would be challenging.
The multinucleon transfer (MNT) reaction approach was successfully employed for the first time to measure the isomeric ratios (IRs) of 211Po isomer (25/2+) and its ground state (9/2+) at the IGISOL facility using a 945 MeV 136Xe beam impinged on 209Bi and natPb targets. The dominant production of isomers compared to the corresponding ground states was consistently revealed in the α-decay spectra. Deduced IR of 211Po populated through the 136Xe+natPb reaction was found to have an enhancement of ≈1.8-times than that observed for the 136Xe+209Bi. State-of-the-art Langevin-type model calculations have been utilized to estimate the spin distribution of an MNT residue. The computations qualitatively corroborate with the considerable increase in the IRs of 211Po produced from 136Xe+natPb compared to 136Xe+209Bi. Theoretical investigations indicate a weak dependence of target spin on the IRs. The enhancement of the 211Po isomer in the 136Xe+natPb over 136Xe+209Bi can be attributed to the different proton (p)-transfer production routes. Estimations demonstrate an increment in the angular momentum transfer, favorable for isomer production, with increasing projectile energy. Comparative analysis reveals the two entrance channel parameters, projectile mass and p-transfer channels, strongly influencing the population of the high-spin isomer of 211Po (25/2+). This letter reports the first experimental and theoretical study on the IRs of nuclei formed via two different channels of MNT reactions.
A direct measurement of the ground-state-to-ground-state electron-capture decay Q value of 95 Tc has been performed utilizing the double Penning trap mass spectrometer JYFLTRAP. The Q value was determined to be 1695.92(13) keV by taking advantage of the high resolving power of the phase-imaging ion-cyclotron-resonance technique to resolve the low-lying isomeric state of 95 Tc (excitation energy of 38.910(40) keV) from the ground state. The mass excess of 95 Tc was measured to be -86015.95(18) keV/c2, exhibiting a precision of about 28 times higher and in agreement with the value from the newest Atomic Mass Evaluation (AME2020). Combined with the nuclear energy-level data for the decay-daughter 95 Mo, two potential ultra-low Q-value transitions are identified for future long-term neutrino-mass determination experiments. The atomic self-consistent many-electron Dirac- Hartree-Fock-Slater method and the nuclear shell model have been used to predict the partial half-lives and energy-release distributions for the two transitions. The dominant correction terms related to those processes are considered, including the exchange and overlap corrections, and the shake-up and shake-off effects. The normalized distribution of the released energy in the electron-capture decay of 95 Tc to excited states of 95 Mo is compared to that of 163 Ho currently being used for electron-neutrino-mass determination.
Collinear laser spectroscopy was performed on the isomer of the aluminium isotope $^{26m}$Al. The measured isotope shift to $^{27}$Al in the $3s^{2}3p\;^{2}\!P^\circ_{3/2} \rightarrow 3s^{2}4s\;^{2}\!S_{1/2}$ atomic transition enabled the first experimental determination of the nuclear charge radius of $^{26m}$Al, resulting in $R_c$=\qty{3.130\pm.015}{\femto\meter}. This differs by 4.5 standard deviations from the extrapolated value used to calculate the isospin-symmetry breaking corrections in the superallowed $\beta$ decay of $^{26m}$Al. Its corrected $\mathcal{F}t$ value, important for the estimation of $V_{ud}$ in the CKM matrix, is thus shifted by one standard deviation to \qty{3071.4\pm1.0}{\second}.
Isomers close to doubly magic _{28}^{78}Ni_{50} provide essential information on the shell evolution and shape coexistence near the Z=28 and N=50 double shell closure. We report the excitation energy measurement of the 1/2^{+} isomer in _{30}^{79}Zn_{49} through independent high-precision mass measurements with the JYFLTRAP double Penning trap and with the ISOLTRAP multi-reflection time-of-flight mass spectrometer. We unambiguously place the 1/2^{+} isomer at 942(10) keV, slightly below the 5/2^{+} state at 983(3) keV. With the use of state-of-the-art shell-model diagonalizations, complemented with discrete nonorthogonal shell-model calculations which are used here for the first time to interpret shape coexistence, we find low-lying deformed intruder states, similar to other N=49 isotones. The 1/2^{+} isomer is interpreted as the bandhead of a low-lying deformed structure akin to a predicted low-lying deformed band in ^{80}Zn, and points to shape coexistence in ^{79,80}Zn similar to the one observed in ^{78}Ni. The results make a strong case for confirming the claim of shape coexistence in this key region of the nuclear chart.
As an essential part of the Super-FRS particle identification, the GEM-TPC detector in a twin field-cage configuration will provide position information at up to 1 MHz counting rate with a spatial resolution < 1 mm and with tracking efficiency >95 %. This detector is designed to provide particle-beam tracking information of projectiles ranging from protons to uranium. The performance of the GEM-TPC detector in a single field-cage configuration and newly integrated AWAGS readout electronics with a differential output was studied at the FRS for the response to the uranium beam at 850 MeV/u with intensity up to 1000 ions/spill. The result shows that a clusterization algorithm developed for this analysis works properly. The spatial resolution of 0.74–0.81 mm, a detection efficiency >99 %, and a tracking efficiency >96 % were found. This work describes the methodology used to achieve such results in detail.
The accurate determination of reactor antineutrino spectra remains a very hot research topic, where new questions have emerged in recent years. Indeed, after the “reactor anomaly” – a deficit of measured antineutrinos at short baseline reactor experiments with respect to spectral predictions – the three international reactor neutrino experiments Double Chooz, Daya Bay and Reno have evidenced spectral distortions in their measurements with respect to the same spectral predictions. This puzzle is called the “shape anomaly”. Recently summation calculations of reactor antineutrino spectra based on the use of nuclear data have obtained the best agreement to date with the reactor neutrino flux measurements at the level of 2% thanks to a decade of Total Absorption Gamma-ray Spectroscopy (TAGS) measurements at the radioactive beam facility of the University of Jyväskylä in two experimental campaigns. A selection of the results obtained so far is presented.
The observation of a weak proton-emission branch in the decay of the 3174-keV 53mCo isomeric state marked the discovery of proton radioactivity in atomic nuclei in 1970. Here we show, based on the partial half-lives and the decay energies of the possible proton-emission branches, that the exceptionally high angular momentum barriers, [Formula: see text] and [Formula: see text], play a key role in hindering the proton radioactivity from 53mCo, making them very challenging to observe and calculate. Indeed, experiments had to wait decades for significant advances in accelerator facilities and multi-faceted state-of-the-art decay stations to gain full access to all observables. Combining data taken with the TASISpec decay station at the Accelerator Laboratory of the University of Jyväskylä, Finland, and the ACTAR TPC device on LISE3 at GANIL, France, we measured their branching ratios as bp1 = 1.3(1)% and bp2 = 0.025(4)%. These results were compared to cutting-edge shell-model and barrier penetration calculations. This description reproduces the order of magnitude of the branching ratios and partial half-lives, despite their very small spectroscopic factors.
The β-delayed neutron emission in the 85,86As β-decays has been measured at the IGISOL facility of the Accelerator Laboratory of the University of Jyväskylä (JYFL-ACCLAB). The complete β-decays have been studied with a complex setup that consists of a plastic scintillator, the MOdular Neutron time-of-flight SpectromeTER (MONSTER), and two types of γ-ray detectors—an HPGe clover and four LaBr3 crystals. The β-delayed neutron energy distributions have been determined by unfolding the TOF spectra with an innovative methodology based on the iterative Bayesian unfolding method and accurate Monte Carlo simulations.
The beta- decay Q value of 136Cs (J pi = 5+, t1/2 approximate to 13 d) was measured with the JYFLTRAP Penning trap setup at the Ion Guide Isotope Separator On-Line facility of the University of Jyvaskyla, Finland. The monoisotopic samples required in the measurements were prepared with a new scheme utilized for the cleaning, based on the coupling of dipolar excitation with Ramsey's method of time-separated oscillatory fields and the phase-imaging ion-cyclotron-resonance technique. The Q value is determined to be 2536.83(45) keV, which is approximate to 4 times more precise and 11.4(20) keV (approximate to 6 sigma) smaller than the adopted value in the most recent Atomic Mass Evaluation AME2020. The daughter, 136Ba, has a 4+ state at 2544.481(24) keV and a 3- state at 2532.653(23) keV, both of which can potentially be ultralow Q-value end states for the 136Cs decay. With our new ground-to-ground state Q value, the decay energies to these two states become -7.65(45 ) keV and 4.18(45) keV, respectively. The former is confirmed to be negative at the level of approximate to 17 sigma, which verifies that this transition is not a suitable candidate for neutrino mass determination. On the other hand, the slightly negative Q value makes this transition an interesting candidate for the study of virtual beta-gamma transitions. The decay to the 3- state is validated to have a positive low Q value which makes it a viable candidate for neutrino mass determination. For this transition, we obtained a shell-model-based half-life estimate of 2.1+1.6 reaction threshold of 79.08(54) keV for the charged-current nu e + 136Xe (0+) -> 136Cs* + e- neutrino capture process is used to update the cross sections for a set of neutrino energies relevant to solar 7Be, pep, and CNO neutrinos. Based on our shell-model calculations, the new lower threshold shows event rates of 2-4 percent higher than the old threshold for several final states reached by the different species of solar neutrinos.
Collinear laser spectroscopy was performed on the isomer of the aluminium isotope ^{26m}Al. The measured isotope shift to ^{27}Al in the 3s^{2}3p ^{2}P_{3/2}^{○}→3s^{2}4s ^{2}S_{1/2} atomic transition enabled the first experimental determination of the nuclear charge radius of ^{26m}Al, resulting in R_{c}=3.130(15) fm. This differs by 4.5 standard deviations from the extrapolated value used to calculate the isospin-symmetry breaking corrections in the superallowed β decay of ^{26m}Al. Its corrected Ft value, important for the estimation of V_{ud} in the Cabibbo-Kobayashi-Maskawa matrix, is thus shifted by 1 standard deviation to 3071.4(1.0) s.
The ss decays of more than twenty fission fragments were measured in the first experiments with radioactive-ion beams employing the Decay Total Absorption.-ray Spectrometer. In this work, we summarize the main results obtained so far from this experimental campaign carried out at the Ion Guide Isotope Separator On-Line facility. The advances introduced for these studies represent the state-of-the-art of our analysis methodology for segmented spectrometers.
The β-delayed neutron emission in the 85 As β-decay has been measured at the IGISOL facility of the Accelerator Laboratory of the University of Jyväskylä (JYFL). The complete β-decay has been studied with a setup which consists of a plastic scintillator, the MO dular N eutron time-of-flight S pectrome TER (MONSTER), and two types of γ-rays detectors (HPGe and LaBr 3 ). The, β-delayed neutron energy distribution has been determined by unfolding the TOF spectrum with the iterative Bayesian unfolding method.