Reduced transition probabilities have been extracted between excited, yrast states in the N=Z+2 nucleus 94Pd. The transitions of interest were observed following decays of the Iπ=14+, Ex=2129-keV isomeric state, which was populated following the projectile fragmentation of a 124Xe primary beam at the GSI Helmholtzzentrum für Schwerionenforschung accelerator facility as part of FAIR Phase-0. Experimental information regarding the reduced E2 transition strengths for the decays of the yrast 8+ and 6+ states was determined following isomer-delayed Eγ1−Eγ2−△T2,1 coincidence method, using the LaBr3(Ce)-based FATIMA fast-timing coincidence gamma-ray array, which allowed direct determination of lifetimes of states in 94Pd using the Generalized Centroid Difference (GCD) method. The experimental value for the half-life of the yrast 8+ state of 755(106) ps results in a reduced transition probability of B(E2:8→+6+) = 205−25+34 e2 fm4, which enables a precise verification of shell-model calculations for this unique system, lying directly between the N=Z line and the N=50 neutron shell closure. The determined B(E2) value provides an insight into the purity of (g9/2)n configurations in competition with admixtures from excitations between the (lower) N=3pf and (higher) N=4gds orbitals for the first time. The results indicate weak collectivity expected for near-zero quadrupole deformation and an increasing importance of the T=0 proton-neutron interaction at N=48.

Lifetime measurements of low-lying excited states in the semimagic (N=50) nucleus Rh95 have been performed by means of the fast-timing technique. The experiment was carried out using γ-ray detector arrays consisting of LaBr3(Ce) scintillators and germanium detectors integrated into the DESPEC experimental setup commissioned for the Facility for Antiproton and Ion Research () Phase-0, Darmstadt, Germany. The excited states in Rh95 were populated primarily via the β decays of Pd95 nuclei, produced in the projectile fragmentation of a 850 MeV/nucleon Xe124 beam impinging on a 4g/cm2Be9 target. The deduced electromagnetic E2 transition strengths for the γ-ray cascade within the multiplet structure depopulating from the isomeric Iπ=21/2+ state are found to exhibit strong deviations from predictions of standard shell model calculations which feature approximately conserved seniority symmetry. In particular, the observation of a strongly suppressed E2 strength for the 13/2+→9/2+ ground state transition cannot be explained by calculations employing standard interactions. This remarkable result may require revision of the nucleon-nucleon interactions employed in state-of-the-art theoretical model calculations, and might also point to the need for including three-body forces in the Hamiltonian. Published by the American Physical Society 2024

Nuclei in the vicinity of 78Ni are important benchmarks for nuclear structure, which can reveal changes in the shell structure far from stability. Spectroscopy of the odd-odd isotope 78Cu was performed for the first time in an experiment with the EURICA setup at the Radioactive Isotope Beam Factory at RIKEN Nishina Center. Excited states in the neutron-rich isotope were populated following the beta decay of 78Ni produced by in-flight fission and

Isomeric states were observed in nuclei produced in an experiment at the RIKEN Nishina Center Radioactive Isotope Beam Factory following the in-flight fission of a 345 MeV/nucleon ^238 U beam. Isomers reported in nuclei spanning a predicted prolate-oblate shape change boundary, ^111 Zr ( E=283.1 keV; τ =0.326(63) s), ^112 Nb ( E=44.2 keV; τ =0.094(26) s), ^113 Nb ( E=135.4 keV; τ =0.846(80) s), and ^115 Mo ( E=198.6 keV; τ =63(4) s), are compared to potential-energy surface calculations which gave a selection of low-lying configurations for each nucleus. Tentative assignments of ground and excited states were made based on energy similarities to the calculations, reduced transition probabilities of the decays, and constraints of transition multipolarities from γ -ray coincidence measurements. These assignments are suggestive of significant deformation being persistent for N>70 in this region. In addition, isomers in ^108 Nb, ^109 Nb, ^113 Tc, ^117 Ru, ^119 Ru, ^120 Rh, and ^122 Rh, not spanning the prolate-oblate transition discussed, are presented.

The Zirconium (Z = 40) isotopic chain has attracted interest for more than four decades. The abrupt lowering of the energy of the first 2^+ state and the increase in the transition strength B(E2; 2^+_1→ 0^+_1) going from ^98 Zr to ^100 Zr has been the first example of “quantum phase transition” in nuclear shapes, which has few equivalents in the nuclear chart. Although a multitude of experiments have been performed to measure nuclear properties related to nuclear shapes and collectivity in the region, none of the measured lifetimes were obtained using the Recoil Distance Doppler Shift method in the γγ -coincidence mode where a gate on the direct feeding transition of the state of interest allows a strict control of systematical errors. This work reports the results of lifetime measurements for the first yrast excited states in ^98-104 Zr carried out to extract reduced transition probabilities. The new lifetime values in γγ -coincidence and γ -single mode are compared with the results of former experiments. Recent predictions of the Interacting Boson Model with Configuration Mixing, the Symmetry Conserving Configuration Mixing model based on the Hartree–Fock–Bogoliubov approach and the Monte Carlo Shell Model are presented and compared with the experimental data.

Excited states in Cu-78 were observed for the first time following the ss decay of Ni-78 created by in-flight fission of U-238. Based on the coincidence relationships between the observed gamma-ray transitions, it was possible to construct a level scheme comprising eight excited states with tentative spin assignments for 5 of them. In addition to the gamma-decaying states, an isomeric state with a lifetime of 3.8(4) ms was found to decay by internal conversion.

Isomeric states of the neutron-rich isotope 189 73 Ta 116 were populated via fragmentation of a primary beam of 208 Pb ions at 1 GeV/u impinging on a 9 Be target at GSI, Darmstadt, Germany. The isotopes of interest were separated, identified and delivered to the DESPEC setup. Two isomers were deduced in 189 Ta 116 and their lifetimes were measured based on the γ-ray time distributions.

The Monte-Carlo simulated response for gamma-ray detection of the FAst TIMing Array (FATIMA) for exploitation within the DEcay SPECtroscopy (DESPEC) experimental system at the FAIR Phase-0 facility at Darmstadt, Germany is presented. In this configuration, FATIMA consisted of 36 LaBr3(Ce) detectors surrounding the AIDA, position-sensitive charged-particle active stopper. The decay of the I-pi=8(+) isomer-fed decay cascade in Pd-96, measured in the first DESPEC experiment at the FAIR-0 facility was used to validate the simulations. The experimental data yielded in-situ full-energy peak efficiency values for FATIMA of 11.2(11)%, 6.8(7)%, 3.8(4)% and 2.1(4)% at 106, 325, 684 and 1415 keV respectively, consistent with the values derived from the simulated response.

Direct lifetime measurements via gamma-gamma coincidences using the FATIMA fast-timing LaBr3(Ce) array were performed for the excited states below previously reported isomers. In the N = 50 semi-magic 96Pd nucleus, lifetimes below the I pi = 8+ seniority isomer were addressed as a benchmark for further analysis. The results for the I pi = 2+ and 4+ states confirm the published values. Increased accuracy for the lifetime value was achieved for the 4+ state.

We report on gamma-ray spectroscopy of low-lying excited states in the neutron-rich Kr-94,Kr-95,Kr-96 isotopes measured as part of the "Shell Evolution And Search for Two-plus energies At RIBF" (SEASTAR) campaign at the RIKEN Radioactive Isotope Beam Factory. Excited yrast and non-yrast states were observed, and half-lives extracted via GEANT4 simulations. In Kr-94,Kr-96 candidates for the 3-1 state were identified. For Kr-95, the prompt SEASTAR data were combined with delayed spectroscopic data measured with the EURICA array to observe transitions on top of the known (7/2)(+) isomer at a level energy of 195.5(3) keV. The comparison of the new experimental results with five-dimensional collective Hamiltonian (5DCH) and mapped interacting boson model (IBM) calculations, both using the Gogny D1M interaction, could suggest oblate-prolate shape coexistence already in Kr-96.

Direct lifetime measurements via gamma -gamma coincidences using a fast timing detector array consisting of LaBr3(Ce) scintillators has been applied to determine the lifetime of low-lying states in the semimagic (N = 50) nucleus Ru-94. The experiment was carried out as the first in a series of "FAIR-0" experiments with the DESPEC experimental setup at the Facility for Antiproton and Ion Research (FAIR). Excited states in Ru-94 were populated primarily via the beta-delayed proton emission of Pd-95 nuclei, produced in the projectile fragmentation of an 850 MeV/nucleon Xe-124 beam impinging on a 4 g/cm(2) Be-9 target. While the deduced E2 strength for the 2(+) -> 0(+) transition in the yrast cascade follows the expected behavior for conserved seniority symmetry, the intermediate 4(+) -> 2(+) transition exhibits a drastic enhancement of transition strength in comparison with pure-seniority model predictions as well as standard shell model predictions in the f pg proton hole space with respect to doubly magic Sn-100. The anomalous behavior is ascribed to a subtle interference between the wave function of the lowest seniority v = 2, I-pi = 4(+) state and that of a close-lying v = 4 state that exhibits partial dynamic symmetry. In addition, the observed strongly prohibitive 6(+) -> 4(+) transition can be attributed to the same mechanism but with a destructive interference. It is noted that such effects may provide stringent tests of the nucleon-nucleon interactions employed in state-of-the-art theoretical model calculations.

This paper reports results of the first experiment of the DESPEC Phase-0 campaign at GSI, which focused on the study of neutron-deficient nuclei approaching 100Sn. These data provide the first extended commissioning experiment for the DESPEC collaboration within NuSTAR. We present results on electromagnetic transition rates associated with the decays from excited states populated following the formation of I pi = 8+ proton 'seniority -isomer' states in the N = 50 isotones 94Ru and 96Pd. Direct half-life measurements via gamma-gamma coincidences using the FATIMA detector array consisting of 36 LaBr3(Ce) scintillators have determined the reduced matrix elements associated with decays between low-lying states in these semi-magic nuclei. The extracted half-lives for yrast I pi = 6+ and 4+ states in 96Pd and the 6+ state in 94Ru are consistent with the published, highest-precision values for these nuclei.

The HISPEC-DESPEC collaboration aims at investigating the struc-ture of exotic nuclei formed in fragmentation reactions with decay spectroscopymeasurements, as part of the FAIR Phase-0 campaign at GSI. This paper reportson first results of an experiment performed in spring 2021, with a focus on beta-decaystudies in the Po-Fr nuclei in the 220 < A <230 island of octupole deformationexploiting the DESPEC setup. Ion-beta correlations and fast-timing techniques arebeing employed, giving an insight into this difficult-to-reach region.

The DEcay SPECtroscopy (DESPEC) setup for nuclear structure investigations was developed and commissioned at GSI, Germany in preparation for a full campaign of experiments at the FRS and Super-FRS. In this paper, we report on the first employment of the setup in the hybrid configuration with the AIDA implanter coupled to the FATIMA LaBr3(Ce) fast-timing array, and high-purity germanium detectors. Initial results are shown from the first experiments carried out with the setup. An overview of the setup and function is discussed, including technical advancements along the path.

Neutron spectrum unfolding using activation foils is currently the primary technique planned for measuring the neutron energy spectrum at the first wall of power-generating fusion reactors. Room for improvement in the effectiveness of current foil selection was identified, and a program produced to select foils procedurally in order to maximise the accuracy of the unfolding procedure. Using Kullback–Leibler Divergence to quantify the accuracy, the spectrum unfolded by the procedurally selected set of foils is found to be more accurate than the spectrum unfolded by a set of foils used in the literature.

The nucleus 212Po has been produced through the fragmentation of a 238U primary beam at 1 GeV/nucleon at GSI, separated with the FRagment Separator, FRS, and studied via isomer γ-decay spectroscopy with the RISING setup. Two delayed previously unknown γ rays have been observed. One has been attributed to the E3 decay of a 21− isomeric state feeding the α-emitting 45-s (18+) high-spin isomer. The other γ-ray line has been assigned to the decay of a higher-lying 23+ metastable state. These are the first observations of high-spin states above the 212Po (18+) isomer, by virtue of the selectivity obtained via ion-by-ion identification of 238U fragmentation products. Comparison with shell-model calculations points to shortfalls in the nuclear interactions involving high-j proton and neutron orbitals, to which the region around Z∼100 is sensitive.

Among the most important physical observables in nuclear structure are the lifetimes of nuclear excited states. Nuclei of Pd-114, predicted by spectroscopic signatures to be candidates for gamma-rigid triaxiality, were populated in the spontaneous fission of Cf-252 and the lifetimes of the 2(1)(+), 4(1)(+) and 6(1)(+) states were measured via the fast-timing technique. The obtained lifetimes of tau(2+) = 103(10) ps, tau(4+) = 21(11) ps, and tau(6+) <= 10 ps, and the corresponding deduced B(E2; I -> I-2) transition probabilities, indicate these to be collective states and also suggest the triaxial shape of Pd-114 to be more gamma-rigid than its even-even neighbours in the Z = 46 isotopic chain.

Summary. — This paper reports preliminary results of the DESPEC campaign at GSI, focused on the study of neutron-deficient nuclei approaching 100 Sn. The results presented show the isomeric decays of excited states with I π = 14 + and 8 + in 96 Pd and 94 Pd, respectively. The detailed characterisation of the DESPEC set-up and analysis methodologies, proven in this experimental run, are crucial for the future campaigns.

The neutron-rich 213Pb isotope was produced in the fragmentation of a primary 1 GeV A 238U beam, separated in FRS in mass and atomic number, and then implanted for isomer decay γ-ray spectroscopy with the RISING setup at GSI. A newly observed isomer and its measured decay properties indicate that states in 213Pb are characterized by the seniority quantum number that counts the nucleons not in pairs coupled to angular momentum J=0. The conservation of seniority is a consequence of a geometric phase associated with particle-hole conjugation, which becomes observable in semi-magic nuclei where nucleons half-fill the valence shell. The γ-ray spectroscopic observables in 213Pb are thus found to be driven by two mechanisms, particle-hole conjugation and seniority conservation, which are intertwined through a Berry phase.

Neutron-rich radioactive isotope (RI) beams in the vicinity of Zr-110 were produced using the in-flight fission of a 345-MeV/nucleon U-238 beam at the RIKEN Radioactive Isotope Beam Factory. The RI beams were separated in flight by the large-acceptance two-stage fragment separator BigRIPS. Isotopes were clearly identified in a low-background particle-identification plot, which was obtained from the measurements of time of flight, magnetic rigidity, and energy loss using beam-line detectors placed in the BigRIPS separator and the ZeroDegree spectrometer. Nine new isotopes, Br-101, Kr-102, Rb-105,Rb-106, Sr-108, Y-110,Y-111, Zr-114, and Nb-117, are reported for the first time, with their measured production cross sections compared with the extrapolations of lighter isotopes down to the femtobarn regime.