The neutron-rich rare isotope 190W is discussed as a candidate for a prolate-oblate transitional nucleus with maximum γ-softness. The collectivity of this isotope is assessed for the first time by the measurement of the reduced E2 transition probability of its first 2+ state to the ground state. The experiment employed the FAst TIming Array (FATIMA), comprised of 36 LaBr3(Ce) scintillators, which was part of the DESPEC setup at GSI, Darmstadt. The 41+ and 21+ states of 190W were populated subsequently to the decay of its 127(12) μs isomeric Jπ=10− state. The mean lifetime of the 21+ state was determined to be τ=274(28) ps, which corresponds to a B(E2;21+→01+) value of 95(10) W.u. The results motivated a revision of previous calculations within an energy-density functional-based interacting boson model-2 approach, yielding E2 transition properties and spectroscopic quadrupole moments for tungsten isotopes. From comparison to theory, the new data suggest that 190W is at the transition from prolate to oblate structure along the W isotopic chain, which had previously been discussed as a nuclear shape-phase transition.
Reduced transition probabilities have been extracted between excited, yrast states in the N=Z+2 nucleus 94Pd. The transitions of interest were observed following decays of the Iπ=14+, Ex=2129-keV isomeric state, which was populated following the projectile fragmentation of a 124Xe primary beam at the GSI Helmholtzzentrum für Schwerionenforschung accelerator facility as part of FAIR Phase-0. Experimental information regarding the reduced E2 transition strengths for the decays of the yrast 8+ and 6+ states was determined following isomer-delayed Eγ1−Eγ2−△T2,1 coincidence method, using the LaBr3(Ce)-based FATIMA fast-timing coincidence gamma-ray array, which allowed direct determination of lifetimes of states in 94Pd using the Generalized Centroid Difference (GCD) method. The experimental value for the half-life of the yrast 8+ state of 755(106) ps results in a reduced transition probability of B(E2:8→+6+) = 205−25+34 e2 fm4, which enables a precise verification of shell-model calculations for this unique system, lying directly between the N=Z line and the N=50 neutron shell closure. The determined B(E2) value provides an insight into the purity of (g9/2)n configurations in competition with admixtures from excitations between the (lower) N=3pf and (higher) N=4gds orbitals for the first time. The results indicate weak collectivity expected for near-zero quadrupole deformation and an increasing importance of the T=0 proton-neutron interaction at N=48.
Lifetime measurements of low-lying excited states in the semimagic (N=50) nucleus Rh95 have been performed by means of the fast-timing technique. The experiment was carried out using γ-ray detector arrays consisting of LaBr3(Ce) scintillators and germanium detectors integrated into the DESPEC experimental setup commissioned for the Facility for Antiproton and Ion Research () Phase-0, Darmstadt, Germany. The excited states in Rh95 were populated primarily via the β decays of Pd95 nuclei, produced in the projectile fragmentation of a 850 MeV/nucleon Xe124 beam impinging on a 4g/cm2Be9 target. The deduced electromagnetic E2 transition strengths for the γ-ray cascade within the multiplet structure depopulating from the isomeric Iπ=21/2+ state are found to exhibit strong deviations from predictions of standard shell model calculations which feature approximately conserved seniority symmetry. In particular, the observation of a strongly suppressed E2 strength for the 13/2+→9/2+ ground state transition cannot be explained by calculations employing standard interactions. This remarkable result may require revision of the nucleon-nucleon interactions employed in state-of-the-art theoretical model calculations, and might also point to the need for including three-body forces in the Hamiltonian. Published by the American Physical Society 2024
Direct lifetime measurements via gamma-gamma coincidences using the FATIMA fast-timing LaBr3(Ce) array were performed for the excited states below previously reported isomers. In the N = 50 semi-magic 96Pd nucleus, lifetimes below the I pi = 8+ seniority isomer were addressed as a benchmark for further analysis. The results for the I pi = 2+ and 4+ states confirm the published values. Increased accuracy for the lifetime value was achieved for the 4+ state.
Direct lifetime measurements via gamma -gamma coincidences using a fast timing detector array consisting of LaBr3(Ce) scintillators has been applied to determine the lifetime of low-lying states in the semimagic (N = 50) nucleus Ru-94. The experiment was carried out as the first in a series of "FAIR-0" experiments with the DESPEC experimental setup at the Facility for Antiproton and Ion Research (FAIR). Excited states in Ru-94 were populated primarily via the beta-delayed proton emission of Pd-95 nuclei, produced in the projectile fragmentation of an 850 MeV/nucleon Xe-124 beam impinging on a 4 g/cm(2) Be-9 target. While the deduced E2 strength for the 2(+) -> 0(+) transition in the yrast cascade follows the expected behavior for conserved seniority symmetry, the intermediate 4(+) -> 2(+) transition exhibits a drastic enhancement of transition strength in comparison with pure-seniority model predictions as well as standard shell model predictions in the f pg proton hole space with respect to doubly magic Sn-100. The anomalous behavior is ascribed to a subtle interference between the wave function of the lowest seniority v = 2, I-pi = 4(+) state and that of a close-lying v = 4 state that exhibits partial dynamic symmetry. In addition, the observed strongly prohibitive 6(+) -> 4(+) transition can be attributed to the same mechanism but with a destructive interference. It is noted that such effects may provide stringent tests of the nucleon-nucleon interactions employed in state-of-the-art theoretical model calculations.
The HISPEC-DESPEC collaboration aims at investigating the struc-ture of exotic nuclei formed in fragmentation reactions with decay spectroscopymeasurements, as part of the FAIR Phase-0 campaign at GSI. This paper reportson first results of an experiment performed in spring 2021, with a focus on beta-decaystudies in the Po-Fr nuclei in the 220 < A <230 island of octupole deformationexploiting the DESPEC setup. Ion-beta correlations and fast-timing techniques arebeing employed, giving an insight into this difficult-to-reach region.
The HISPEC/DESPEC collaboration envisages long experimental campaigns exploiting the expected beam performances of Super-FRS. The experiments will be performed at the Low-Energy Branch of the upcoming FAIR and will focus on the physics of exotic isotopes, primarily in the heavy neutron-rich region. The goal of the HISPEC/DESPEC experimental campaigns is to explore the excitation and decay properties of rare isotopes produced via fragmentation and fission. First rare-isotope beam simulations of representative future HISPEC/DESPEC experimental cases are presented. The simulations provide an insight into the forthcoming state-of-art experiments in the future FAIR facility.
The DEcay SPECtroscopy (DESPEC) setup for nuclear structure investigations was developed and commissioned at GSI, Germany in preparation for a full campaign of experiments at the FRS and Super-FRS. In this paper, we report on the first employment of the setup in the hybrid configuration with the AIDA implanter coupled to the FATIMA LaBr3(Ce) fast-timing array, and high-purity germanium detectors. Initial results are shown from the first experiments carried out with the setup. An overview of the setup and function is discussed, including technical advancements along the path.
Summary. — This paper reports preliminary results of the DESPEC campaign at GSI, focused on the study of neutron-deficient nuclei approaching 100 Sn. The results presented show the isomeric decays of excited states with I π = 14 + and 8 + in 96 Pd and 94 Pd, respectively. The detailed characterisation of the DESPEC set-up and analysis methodologies, proven in this experimental run, are crucial for the future campaigns.
Received 23 November 2017DOI:https://doi.org/10.1103/PhysRevC.97.019901©2018 American Physical SocietyPhysics Subject Headings (PhySH)Research AreasElectromagnetic transitionsIsomer decaysLifetimes & widthsNuclear structure & decaysProperties59 ≤ A ≤ 8990 ≤ A ≤ 149TechniquesShell modelNuclear Physics
The neutron-rich 213Pb isotope was produced in the fragmentation of a primary 1 GeV A 238U beam, separated in FRS in mass and atomic number, and then implanted for isomer decay γ-ray spectroscopy with the RISING setup at GSI. A newly observed isomer and its measured decay properties indicate that states in 213Pb are characterized by the seniority quantum number that counts the nucleons not in pairs coupled to angular momentum J=0. The conservation of seniority is a consequence of a geometric phase associated with particle-hole conjugation, which becomes observable in semi-magic nuclei where nucleons half-fill the valence shell. The γ-ray spectroscopic observables in 213Pb are thus found to be driven by two mechanisms, particle-hole conjugation and seniority conservation, which are intertwined through a Berry phase.
In a high-energy fragmentation experiment at GSI an I=π(6+) isomer and its γ-decay are identified in 102Sn, the two-neutron neighbour of the doubly-magic 100Sn. Its half-life is measured to be T=1/2367(11) ns. The possible existence of further isomers is discussed in the framework of large-scale shell model (LSSM) calculations including up to five particle-hole excitations of the 100Sn core. From the precise B(E2; 6+→4+) strength and the recently remeasured value for B(E2; 8+→6+) in the two-proton hole neighbour 98Cd effective E2 polarization charges for protons and neutrons were inferred including LSSM corrections within the full N=4 0ħω space. The results are discussed in comparison to predicted and empirically determined effective operators.
We report on new γ-ray spectroscopy results from β decays of In99 and Sn101. 30 new γ rays were observed following the β decay of In99, and inconsistencies in the literature with respect to the γ rays following the β decay of Sn101 were addressed with two confirmed cases and two new transitions. The experimental γ-ray energies, intensities, and coincidence relationships are discussed with shell model calculations, where theoretical β-decay branching ratios from the parent nuclei and γ-ray cascades of excited states from the daughter nuclei were combined to generate hypothetical βγ spectra and βγγ coincidence matrices. The most intense β-delayed γ-ray branches in both Cd99 and In101 were well reproduced with this approach, and several γ rays were assigned to new excited states based on their good agreement with shell model predictions.
We report on new gamma-ray spectroscopy results from beta decays of In-99 and Sn-101. 30 new gamma rays were observed following the beta decay of In-99, and inconsistencies in the literature with respect to the gamma rays following the beta decay of Sn-101 were addressed with two confirmed cases and two new transitions. The experimental gamma-ray energies, intensities, and coincidence relationships are discussed with shell model calculations, where theoretical beta-decay branching ratios from the parent nuclei and gamma-ray cascades of excited states from the daughter nuclei were combined to generate hypothetical beta gamma spectra and beta gamma gamma coincidence matrices. The most intense beta-delayed gamma-ray branches in both Cd-99 and In-101 were well reproduced with this approach, and several gamma rays were assigned to new excited states based on their good agreement with shell model predictions.
A first performance test of the Coulomb excitation multipolarimetry (Coulex-multipolarimetry) method is presented. It is based on a $$^{85}\hbox {Br}\,\pi p_{3/2}\rightarrow \pi p_{1/2}$$ spin-flip experiment performed as part of the PreSPEC-AGATA campaign at the GSI Helmholtzzentrum für Schwerionenforschung (GSI). Via determination of background levels around the expected $$^{85}\hbox {Br}$$ excitations as well as measured $$^{197}\hbox {Au}$$ excitations, an upper limit for the M1 transition strength of the $$1/2_1^-\rightarrow 3/2_\text {g.s.}^-$$ transition in $$^{85}\hbox {Br}$$ and a lower beam time limit for upcoming experimental campaigns utilizing Coulex-multipolarimetry have been inferred. The impact of the use of AGATA in its anticipated $$1\pi $$ configuration on these estimates is deduced via Geant4 simulations.
first performance test of the Coulomb excitation multipolarimetry ( Coulex-multipolarimetry ) method is presented. It is based on a ^85Br π p_3/2→π p_1/2 spin-flip experiment performed as part of the PreSPEC-AGATA campaign at the GSI Helmholtzzentrum für Schwerionenforschung (GSI). Via determination of background levels around the expected ^85Br excitations as well as measured ^197Au excitations, an upper limit for the M 1 transition strength of the 1/2_1^-→ 3/2_g.s.^- transition in ^85Br and a lower beam time limit for upcoming experimental campaigns utilizing Coulex-multipolarimetry have been inferred. The impact of the use of AGATA in its anticipated 1π configuration on these estimates is deduced via Geant4 simulations.
We report on new $\ensuremath{\gamma}$-ray spectroscopy results from $\ensuremath{\beta}$ decays of $^{99}\mathrm{In}$ and $^{101}\mathrm{Sn}$. 30 new $\ensuremath{\gamma}$ rays were observed following the $\ensuremath{\beta}$ decay of $^{99}\mathrm{In}$, and inconsistencies in the literature with respect to the $\ensuremath{\gamma}$ rays following the $\ensuremath{\beta}$ decay of $^{101}\mathrm{Sn}$ were addressed with two confirmed cases and two new transitions. The experimental $\ensuremath{\gamma}$-ray energies, intensities, and coincidence relationships are discussed with shell model calculations, where theoretical $\ensuremath{\beta}$-decay branching ratios from the parent nuclei and $\ensuremath{\gamma}$-ray cascades of excited states from the daughter nuclei were combined to generate hypothetical $\ensuremath{\beta}\ensuremath{\gamma}$ spectra and $\ensuremath{\beta}\ensuremath{\gamma}\ensuremath{\gamma}$ coincidence matrices. The most intense $\ensuremath{\beta}$-delayed $\ensuremath{\gamma}$-ray branches in both $^{99}\mathrm{Cd}$ and $^{101}\mathrm{In}$ were well reproduced with this approach, and several $\ensuremath{\gamma}$ rays were assigned to new excited states based on their good agreement with shell model predictions.
Electric quadrupole matrix elements, Mp, for the Jπ=2+→0+, ΔT=0, T=1 transitions across the A=46 isobaric multiplet 46Cr-46V-46Ti have been measured at GSI with the FRS-LYCCA-AGATA setup. This allows direct insight into the isospin purity of the states of interest by testing the linearity of Mp with respect to Tz. Pairs of nuclei in the T=1 triplet were studied using identical reaction mechanisms in order to control systematic errors. The Mp values were obtained with two different methodologies: (i) a relativistic Coulomb excitation experiment was performed for 46Cr and 46Ti; (ii) a "stretched target" technique was adopted here, for the first time, for lifetime measurements in 46V and 46Ti. A constant value of Mp across the triplet has been observed. Shell-model calculations performed within the fp shell fail to reproduce this unexpected trend, pointing towards the need of a wider valence space. This result is confirmed by the good agreement with experimental data achieved with an interaction which allows excitations from the underlying sd shell. A test of the linearity rule for all published data on complete T=1 isospin triplets is presented.
A record number of ^{100}Sn nuclei was detected and new isotopic species toward the proton dripline were discovered at the RIKEN Nishina Center. Decay spectroscopy was performed with the high-efficiency detector arrays WAS3ABi and EURICA. Both the half-life and the β-decay end point energy of ^{100}Sn were measured more precisely than the literature values. The value and the uncertainty of the resulting strength for the pure 0^{+}→1^{+} Gamow-Teller decay was improved to B_{GT}=4.4_{-0.7}^{+0.9}. A discrimination between different model calculations was possible for the first time, and the level scheme of ^{100}In is investigated further.