We show how the phase profile of Bose-Einstein condensates can be engineered through its interaction with localized Rydberg excitations. The interaction is made controllable and long range by off-resonantly coupling the condensate to another Rydberg state with laser light. Our technique allows the mapping of entanglement generated in systems of few strongly interacting Rydberg atoms onto much larger atom clouds in hybrid setups. As an example we discuss the creation of a spatial mesoscopic superposition state from a bright soliton. Additionally, the phase imprinted onto the condensate using the Rydberg excitations is a diagnostic tool for the latter. For example, a condensate time-of-flight image would permit reconstructing the pattern of an embedded Rydberg crystal.

We explore trapped ions as a setting to investigate nonequilibrium phases in a generalized Dicke model of dissipative spins coupled to phonon modes. We find a rich dynamical phase diagram including superradiantlike regimes, dynamical phase coexistence, and phonon-lasing behavior. A particular advantage of trapped ions is that these phases and transitions among them can be probed in situ through fluorescence. We demonstrate that the main physical insights are captured by a minimal model and consider an experimental realization with Ca+ ions trapped in a linear Paul trap with a dressing scheme to create effective two-level systems with a tunable dissipation rate.

We consider a dense one-dimensional laser-driven Rydberg lattice gas with perfect nearest-neighbor blockade. The ground state of this system can be found analytically in certain parameter regimes even when the applied fields are inhomogeneous in space. We will use this unique feature to investigate the effect of an impurity-introduced by the local variation of the laser parameters-on the correlations of the many-body ground state. Moreover, we explore the role of a staggered laser field which alternates from site to site thereby breaking the sublattice symmetry. We demonstrate that this technique, which can be applied experimentally, reveals insights into the role of long-range interactions on the critical properties of a Rydberg gas. Our work highlights possibilities for the exploration of many-body physics in Rydberg lattice gases based on locally tunable laser fields.

Received 4 February 2014DOI:https://doi.org/10.1103/PhysRevLett.112.099901© 2014 American Physical Society

The dynamics of excitons in a one-dimensional ensemble with partial spatial order are studied. During optical excitation, cold Rydberg atoms spontaneously organize into regular spatial arrangements due to their mutual interactions. This emergent lattice is used as the starting point to study resonant energy transfer triggered by driving a $nS$ to ${n}^{\ensuremath{'}}P$ transition using a microwave field. The dynamics are probed by detecting the survival probability of atoms in the $nS$ Rydberg state. Experimental data qualitatively agree with our theoretical predictions including the mapping onto the $XXZ$ spin model in the strong-driving limit. Our results suggest that emergent Rydberg lattices provide an ideal platform to study coherent energy transfer in structured media without the need for externally imposed potentials.

The laser excitation of Rydberg atoms in ultracold gases is often described assuming that the atomic motion is frozen during the excitation time. We show that this frozen gas approximation can break down for atoms that are held in optical lattices or microtraps. In particular, we show that the excitation dynamics is in general strongly affected by mechanical forces among the Rydberg atoms as well as the spread of the atomic wave packet in the confining potential. This causes decoherence in the excitation dynamics---resulting in a dissipative blockade effect---that renders the Rydberg excitation inefficient even in the antiblockade regime. For a strongly off-resonant laser excitation---usually considered in the context of Rydberg dressing---these motional effects compromise the applicability of the Born-Oppenheimer approximation. In particular, our results indicate that they can also lead to decoherence in the dressing regime.

We present a fast and quasideterministic protocol for the production of single ions and electrons from a cloud of laser-cooled atoms. The approach is based on a two-step process where first a single Rydberg atom is photoexcited from a dipole-blockade configuration and subsequently ionized by an electric field pulse. We theoretically describe these excitation-ionization cycles via dynamical quantum maps and observe a rich behavior of the ionization dynamics as a function of laser Rabi frequency, pulse duration, and particle number. Our results show that a fast sequential heralded production of single charged particles is achievable even from an unstructured and fluctuating atomic ensemble.

We study the out-of-equilibrium evolution of a strongly interacting quantum spin chain which is mapped on a system of hard rods that are coherently deposited on and removed from a lattice. We show that this closed quantum system approaches an equilibrium steady state which strongly resembles a microcanonical ensemble of classical hard rods. Starting from the fully coherent evolution equation we derive a master equation for the evolution of the number of hard rods on the lattice. This equation not only captures properties of the equilibrium state but also describes the dynamical non-equilibrium evolution into it for the majority of initial conditions. We analyze this in detail for hard rods of varying size.

In a laser-driven Rydberg gas the strong interaction between atoms excited to Rydberg states results in the formation of collective excitations. Atoms within a so-called blockade volume share a single Rydberg excitation, which is dynamically created and annihilated. For sufficiently long times this driven system approaches a steady state, which lends its properties from a maximum entropy state of a Tonks gas. Using this connection we show that spatial correlations between Rydberg atoms are controlled by the number of atoms contained within a blockade volume. For a small number the system favors a disordered arrangement of Rydberg atoms, whereas in the opposite limit Rydberg atoms tend to arrange in an increasingly ordered configuration. We argue that this is an entropic effect which is observable in current experiments.

We show that in a gas of ultracold atoms distance selective two-body loss can be engineered via the resonant laser excitation of atom pairs to interacting electronic states. In an optical lattice this leads to a dissipative master equation dynamics with Lindblad jump operators that annihilate atom pairs with a specific interparticle distance. In conjunction with coherent hopping between lattice sites this unusual dissipation mechanism leads to the formation of coherent long-lived complexes that can even exhibit an internal level structure which is strongly coupled to their external motion. We analyze this counterintuitive phenomenon in detail in a system of hard-core bosons. While current research has established that dissipation in general can lead to the emergence of coherent features in many-body systems our work shows that strong nonlocal dissipation can effectuate a binding mechanism for particles.

Thermalization has been shown to occur in a number of closed quantum many-body systems, but the description of the actual thermalization dynamics is prohibitively complex. Here, we present a model - in one and two dimensions - for which we can analytically show that the evolution into thermal equilibrium is governed by a Fokker-Planck equation derived from the underlying quantum dynamics. Our approach does not rely on a formal distinction of weakly coupled bath and system degrees of freedom. The results show that transitions within narrow energy shells lead to a dynamics which is dominated by entropy and establishes detailed balance conditions that determine both the eventual equilibrium state and the non-equilibrium relaxation to it.

We employ the concept of a dynamical, activity order parameter to study the Ising model in a transverse magnetic field coupled to a Markovian bath. For a certain range of values of the spin-spin coupling, magnetic field and dissipation rate, we identify a first order dynamical phase transition between active and inactive {\em dynamical phases}. We demonstrate that dynamical phase-coexistence becomes manifest in an intermittent behavior of the bath quanta emission. Moreover, we establish the connection between the dynamical order parameter that quantifies the activity, and the longitudinal magnetization that serves as static order parameter. The system we consider can be implemented in current experiments with Rydberg atoms and trapped ions.

We show how to create long range interactions between alkali-atoms in different hyper-fine ground states, allowing coherent electronic quantum state migration. The scheme uses off resonant dressing with atomic Rydberg states, exploiting the dipole-dipole excitation transfer that is possible between those. Actual population in the Rydberg state is kept small. Dressing offers large advantages over the direct use of Rydberg levels: It reduces ionisation probabilities and provides an additional tuning parameter for life-times and interaction-strengths. We present an effective Hamiltonian for the ground-state manifold and show that it correctly describes the full multi-state dynamics for up to 5 atoms.

We develop an efficient Monte-Carlo approach to describe the optical response of cold three-level atoms in the presence of EIT and strong atomic interactions. In particular, we consider a "Rydberg-EIT medium" where one involved level is subject to large shifts due to strong van der Waals interactions with surrounding Rydberg atoms. We find excellent agreement with much more involved quantum calculations and demonstrate its applicability over a wide range of densities and interaction strengths. The calculations show that the nonlinear absorption due to Rydberg-Rydberg atom interactions exhibits universal behavior.

We present the direct measurements of electric dipole moments for 5P3/2 → nD5/2 transitions with 20 < n < 48 for rubidium atoms. The measurements were carried out in an ultracold sample via observation of the Autler–Townes splitting in a three-level ladder scheme, commonly used for twophoton excitation of Rydberg states. To the best of our knowledge, this is the first systematic measurement of the electric dipole moments for transitions from low excited states of rubidium to Rydberg states. Due to its simplicity and versatility, this method can be easily extended to other transitions and other atomic species with few constraints. The good agreement seen between the experimental results and the theory proves the reliability of the measurement method. 3 Author to whom any correspondence should be addressed. New Journal of Physics 13 (2011) 093012 1367-2630/11/093012+11$33.00 © IOP Publishing Ltd and Deutsche Physikalische Gesellschaft

We study a two-dimensional lattice gas of atoms that are photoexcited to Rydberg states in which they interact via the van der Waals interaction. We explore the regime of dominant nearest-neighbor interaction where this system is intimately connected with a quantum version of Baxter's hard-squares model. We show that the strongly correlated ground state of the Rydberg gas can be analytically described by a projected entangled pair state that constitutes the ground state of the quantum hard-squares model. This correspondence allows us to identify a phase boundary where the Rydberg gas undergoes a transition from a disordered (liquid) phase to an ordered (solid) phase.

Thermalization has been shown to occur in a number of closed quantum many-body systems, but the description of the actual thermalization dynamics is prohibitively complex. Here, we present a model - in one and two dimensions - for which we can analytically show that the evolution into thermal equilibrium is governed by a Fokker-Planck equation derived from the underlying quantum dynamics. Our approach does not rely on a formal distinction of weakly coupled bath and system degrees of freedom. The results show that transitions within narrow energy shells lead to a dynamics which is dominated by entropy and establishes detailed balance conditions that determine both the eventual equilibrium state and the non-equilibrium relaxation to it.

We consider the interplay between excitonic and atomic motion in a regular, flexible chain of Rydberg atoms, extending our recent results on entanglement transport in Rydberg chains [W\"uster et al., Phys.Rev.Lett 105 053004 (2010)]. In such a Rydberg chain, similar to molecular aggregates, an electronic excitation is delocalised due to long range dipole-dipole interactions among the atoms. The transport of an exciton that is initially trapped by a chain dislocation is strongly coupled to nuclear dynamics, forming a localised pulse of combined excitation and displacement. This pulse transfers entanglement between dislocated atoms adiabatically along the chain. Details about the interaction and the preparation of the initial state are discussed. We also present evidence that the quantum dynamics of this complex many-body problem can be accurately described by selected quantum-classical methods, which greatly simplify investigations of excitation transport in flexible chains.

In this paper, we consider the effects of strong dipole-dipole interactions on three-level interference phenomena such as coherent population trapping and electromagnetically induced transparency. Experiments are performed on laser cooled rubidium atoms and the results compared to a many-body theory based on either a reduced many-body density matrix expansion or Monte Carlo simulations of many-body rate equations. We show that these approaches permit quantitative predictions of the experimentally observed excitation and transmission spectra. Based on the calculations, we moreover predict a universal scaling of the nonlinear response of cold Rydberg gases.

We present an analytical theory for the nonlinear optical response of a strongly interacting Rydberg gas under conditions of electromagnetically induced transparency. Simple formulas for the third-order optical susceptibility are derived and shown to be in excellent agreement with recent experiments. The obtained expressions reveal strong nonlinearities, which in addition are of highly nonlocal character. This property together with the enormous strength of the Rydberg-induced nonlinearities is shown to yield a unique laboratory platform for nonlinear wave phenomena, such as collapse-arrested modulational instabilities in a self-defocusing medium.