The PROSPECT-I detector has several features that enable measurement of the direction of a compact neutrino source. In this paper, a detailed report on the directional measurements made on electron antineutrinos emitted from the High Flux Isotope Reactor is presented. With an estimated true neutrino (reactor to detector) direction of % = 40.8 degrees + 0.7 degrees and theta = 98.6 degrees + 0.4 degrees, the PROSPECT-I detector is able to reconstruct an average neutrino direction of % = 39.4 degrees + 2.9 degrees and theta = 97.6 degrees + 1.6 degrees. This measurement is made with approximately 48 000 inverse beta decay signal events and is the most precise directional reconstruction of reactor antineutrinos to date.

The PROSPECT experiment is designed to perform precise searches for antineutrino disappearance at short distances (7-9 m) from compact nuclear reactor cores. This Letter reports results from a new neutrino oscillation analysis performed using the complete data sample from the PROSPECT-I detector operated at the High Flux Isotope Reactor in 2018. The analysis uses a multiperiod selection of inverse beta decay neutrino interactions with reduced backgrounds and enhanced statistical power to set limits on electron neutrino disappearance caused by mixing with sterile neutrinos with 0.2-20  eV^{2} mass splittings. Inverse beta decay positron energy spectra from six different reactor-detector distance ranges are found to be statistically consistent with one another, as would be expected in the absence of sterile neutrino oscillations. The data excludes at 95% confidence level the existence of sterile neutrinos in regions above 3  eV^{2} previously unexplored by terrestrial experiments, including all space below 10  eV^{2} suggested by the recently strengthened Gallium Anomaly. The best-fit point of the Neutrino-4 reactor experiment's claimed observation of short-baseline oscillation is ruled out at more than 5 standard deviations.

Nuclear reactors are uniquely powerful, abundant, and flavor-pure sources of antineutrinos that have played a central role in the discovery of the neutrinos and in elucidation of their properties. This continues through a broad range of experiments investigating topics including Standard Model and short-baseline oscillations, beyond-the-Standard-Model physics searches, and reactor flux and spectrum modelling. This Report will survey the state of the reactor antineutrino physics field and summarize the ways in which current and future reactor antineutrino experiments can play a critical role in advancing the field of particle physics in the next decade.

A 6 Li-doped plastic scintillator with pulse-shape discrimination capabilities, commercially identified as EJ-299- 50, has been developed and produced at the kilogram-scale. A total of 44 bars of dimensions 5.5 cm x 5.5 cm x 50 cm of this material have been characterized. Optical properties like light output and effective attenuation length have been found to be comparable to 6 Li-doped liquid scintillators. The scintillator EJ-299-50 shows good neutron detection capabilities with an effective efficiency for capture on 6 Li of approximately 85%. Stability tests performed on two formulation variations showed no intrinsic degradation in the material or optical properties during several months of observations.

This white paper provides a comprehensive review of our present understanding of experimental neutrino anomalies that remain unresolved, charting the progress achieved over the last decade at the experimental and phenomenological level, and sets the stage for future programmatic prospects in addressing those anomalies. It is purposed to serve as a guiding and motivational "encyclopedic" reference, with emphasis on needs and options for future exploration that may lead to the ultimate resolution of the anomalies. We see the main experimental, analysis, and theory-driven thrusts that will be essential to achieving this goal being: 1) Cover all anomaly sectors -- given the unresolved nature of all four canonical anomalies, it is imperative to support all pillars of a diverse experimental portfolio, source, reactor, decay-at-rest, decay-in-flight, and other methods/sources, to provide complementary probes of and increased precision for new physics explanations; 2) Pursue diverse signatures -- it is imperative that experiments make design and analysis choices that maximize sensitivity to as broad an array of these potential new physics signatures as possible; 3) Deepen theoretical engagement -- priority in the theory community should be placed on development of standard and beyond standard models relevant to all four short-baseline anomalies and the development of tools for efficient tests of these models with existing and future experimental datasets; 4) Openly share data -- Fluid communication between the experimental and theory communities will be required, which implies that both experimental data releases and theoretical calculations should be publicly available; and 5) Apply robust analysis techniques -- Appropriate statistical treatment is crucial to assess the compatibility of data sets within the context of any given model.

One of the two detector material choices now being considered for the Mobile Antineutrino Demonstrator (MAD) project is 6 Li-doped pulse shape discriminating (PSD) plastic scintillator. This new material, manufactured by Eljen and designated EJ-299-50, continues the development of PSD plastic materials by the materials science group at LLNL, which invented PSD plastic in 2012. At present EJ-299-50 can be manufactured in multi-liter volumes with attenuation lengths approaching ~1 m. The MAD project is considering the use of this material in the form of 1 m long segments at 6 cm x 6 cm cross section. A 2D array of scintillator segments was shown to be an effective technique for above-ground reactor antineutrino detection by PROSPECT. For MAD, plastic material is considered a requirement for truly mobile above-ground detection systems suited to reactor monitoring for safeguards. In this presentation, we will summarize a set of key performance criteria, including attenuation length, stability, pulse shape sensitivity, and fast and slow neutron efficiency measurements and discuss how those performance criteria might translate to the overall performance of MAD.

Plastic scintillators that can discriminate between gamma rays, fast neutrons, and thermal neutrons were synthesized and characterized while considering the performance at the kilogram scale. The synthesis and processing of these plastic scintillators on the kilogram scale required examination of several factors. The examination of these factors was necessitated by the inclusion of 0.1 wt.% lithium-6 to enable detection of thermal neutrons. First, methacrylic acid was used as an additive to solubilize salts of lithium-6, which allow for a thermal-neutron capture reaction that produces scintillation light following energy transfer. Second, a trade-off between scintillation performance and processability was considered because the increasing content of the methacrylic acid that aided processability resulted in a sharp decrease in the light output. The use of small amounts of methacrylic acid (≤3 wt.%) resulted in better performance but required high processing temperatures. At large scales, these high temperatures could initiate exothermic polymerization that results in premature curing and/or defects. The deleterious effects of the methacrylic acid may be mitigated by using m-terphenyl as a primary dye rather than 2,5-diphenyloxazole (PPO), which has been traditionally used in organic scintillators. Finally, the curing environment was controlled to avoid defects like cracking and discolouration​ while maintaining solubility of dopants during curing. For scintillators that were produced from kilogram-scale batches of precursors, the effective attenuation of scintillation light was characterized.

The precise modeling of the de-excitation of Gd isotopes is of great interest for experimental studies of neutrinos using Gd-loaded organic liquid scintillators. The FIFRELIN code was recently used within the purposes of the STEREO experiment for the modeling of the Gd de-excitation after neutron capture in order to achieve a good control of the detection efficiency. In this work, we report on the recent additions in the FIFRELIN de-excitation model with the purpose of enhancing further the de-excitation description. Experimental transition intensities from the EGAF database are now included in the FIFRELIN cascades, in order to improve the description of the higher energy part of the spectrum. Furthermore, the angular correlations between γ rays are now implemented in FIFRELIN, to account for the relative anisotropies between them. In addition, conversion electrons are now treated more precisely in the whole spectrum range, while the subsequent emission of X rays is also accounted for. The impact of the aforementioned improvements in FIFRELIN is tested by simulating neutron captures in various positions inside the STEREO detector. A repository of up-to-date FIFRELIN simulations of the Gd isotopes is made available for the community, with the possibility of expanding for other isotopes which can be suitable for different applications.

This paper presents an energy calibration scheme for an upgraded reactor antineutrino detector for the Precision Reactor Oscillation and Spectrum Experiment (PROSPECT). The PROSPECT collaboration is preparing an upgraded detector, PROSPECT-II (P-II), to advance capabilities for the investigation of fundamental neutrino physics, fission processes and associated reactor neutrino flux, and nuclear security applications. P-II will expand the statistical power of the original PROSPECT (P-I) dataset by at least an order of magnitude. The new design builds upon previous P-I design and focuses on improving the detector robustness and long-term stability to enable multi-year operation at one or more sites. The new design optimizes the fiducial volume by elimination of dead space previously occupied by internal calibration channels, which in turn necessitates the external deployment. In this paper, we describe a calibration strategy for P-II. The expected performance of externally deployed calibration sources is evaluated using P-I data and a well-benchmarked simulation package by varying detector segmentation configurations in the analysis. The proposed external calibration scheme delivers a compatible energy scale model and achieves comparable performance with the inclusion of an additional AmBe neutron source, in comparison to the previous internal arrangement. Most importantly, the estimated uncertainty contribution from the external energy scale calibration model meets the precision requirements of the P-II experiment.

The paper describes preparation of 6Li-loaded liquid scintillators by methods involving direct dissolution of 6Li salts in the commercial diisopropylnaphthalene (DIPN) solvent, without the formation of water-in-oil emulsions. Methods include incorporation of 6Li that, unlike previously reported formulations, does not require additions of water or a strong acid such as hydrochloric acid (HCl). Results of the conducted experiments show that dissolution of aromatic , aliphatic 6Li salts in DIPN can be easily achieved at 0.1%-0.3% by weight of atomic 6Li, using small additions of waterless surfactants, or mild carboxylic acids. An alternative way suggests incorporation of 6Li as a part of a surfactant molecule that can be dissolved in DIPN without any solubilizing additions. Proposed methods enable preparation of efficient 6Li-loaded liquid scintillators that, at a large scale of 50 cm, exhibit good pulse shape discrimination (PSD) properties combined with up to 107% of light output and up to 115% of the attenuation length measured relative to standard undoped EJ-309 liquid scintillator.

This Letter reports one of the most precise measurements to date of the antineutrino spectrum from a purely ^{235}U-fueled reactor, made with the final dataset from the PROSPECT-I detector at the High Flux Isotope Reactor. By extracting information from previously unused detector segments, this analysis effectively doubles the statistics of the previous PROSPECT measurement. The reconstructed energy spectrum is unfolded into antineutrino energy and compared with both the Huber-Mueller model and a spectrum from a commercial reactor burning multiple fuel isotopes. A local excess over the model is observed in the 5-7 MeV energy region. Comparison of the PROSPECT results with those from commercial reactors provides new constraints on the origin of this excess, disfavoring at 2.0 and 3.7 standard deviations the hypotheses that antineutrinos from ^{235}U are solely responsible and noncontributors to the excess observed at commercial reactors, respectively.

Nuclear reactors are uniquely powerful, abundant, and flavor-pure sources of antineutrinos that continue to play a vital role in the US neutrino physics program. The US reactor antineutrino physics community is a diverse interest group encompassing many detection technologies and many particle physics topics, including Standard Model and short-baseline oscillations, BSM physics searches, and reactor flux and spectrum modeling. The community's aims offer strong complimentary with numerous aspects of the wider US neutrino program and have direct relevance to most of the topical sub-groups composing the Snowmass 2021 Neutrino Frontier. Reactor neutrino experiments also have a direct societal impact and have become a strong workforce and technology development pipeline for DOE National Laboratories and universities. This white paper, prepared as a submission to the Snowmass 2021 community organizing exercise, will survey the state of the reactor antineutrino physics field and summarize the ways in which current and future reactor antineutrino experiments can play a critical role in advancing the field of particle physics in the next decade.

Different extensions of the standard model of particle physics, such as braneworld or mirror matter models, predict the existence of a neutron sterile state, possibly as a dark matter candidate. This Letter reports a new experimental constraint on the probability p for neutron conversion into a hidden neutron, set by the STEREO experiment at the high flux reactor of the Institut Laue-Langevin. The limit is p<3.1×10^{-11} at 95% C.L. improving the previous limit by a factor of 13. This result demonstrates that short-baseline neutrino experiments can be used as competitive passing-through-walls neutron experiments to search for hidden neutrons.

The PROSPECT and STEREO collaborations present a combined measurement of the pure ^{235}U antineutrino spectrum, without site specific corrections or detector-dependent effects. The spectral measurements of the two highest precision experiments at research reactors are found to be compatible with χ^{2}/ndf=24.1/21, allowing a joint unfolding of the prompt energy measurements into antineutrino energy. This ν[over ¯]_{e} energy spectrum is provided to the community, and an excess of events relative to the Huber model is found in the 5-6 MeV region. When a Gaussian bump is fitted to the excess, the data-model χ^{2} value is improved, corresponding to a 2.4σ significance.

The PROSPECT experiment has substantially addressed the original 'Reactor Antineutrino Anomaly' by performing a high-resolution spectrum measurement from an enriched compact reactor core and a reactor model-independent sterile neutrino oscillation search based on the unique spectral distortions the existence of eV$^2$-scale sterile neutrinos would impart. But as the field has evolved, the current short-baseline (SBL) landscape supports many complex phenomenological interpretations, establishing a need for complementary experimental approaches to resolve the situation. While the global suite of SBL reactor experiments, including PROSPECT, have probed much of the sterile neutrino parameter space, there remains a large region above 1 eV$^2$ that remains unaddressed. Recent results from BEST confirm the Gallium Anomaly, increasing its significance to $\sim 5\sigma$, with sterile neutrinos providing a possible explanation of this anomaly. Separately, the MicroBooNE exclusion of electron-like signatures causing the MiniBooNE low-energy excess does not eliminate the possibility of sterile neutrinos as an explanation. Focusing specifically on the future use of reactors as a neutrino source for beyond-the-standard-model physics and applications, higher-precision spectral measurements still have a role to play. These recent results have created a confusing landscape which requires new data to disentangle the seemingly contradictory measurements. To directly probe $\overline{\nu}_{e}$ disappearance from high $\Delta m^2$ sterile neutrinos, the PROSPECT collaboration proposes to build an upgraded and improved detector, PROSPECT-II. It features an evolutionary detector design which can be constructed and deployed within one year and have impactful physics with as little as one calendar year of data.

This article reports the measurement of the $^{235}$U-induced antineutrino spectrum shape by the STEREO experiment. 43'000 antineutrinos have been detected at about 10 m from the highly enriched core of the ILL reactor during 118 full days equivalent at nominal power. The measured inverse beta decay spectrum is unfolded to provide a pure $^{235}$U spectrum in antineutrino energy. A careful study of the unfolding procedure, including a cross-validation by an independent framework, has shown that no major biases are introduced by the method. A significant local distortion is found with respect to predictions around $E_\nu \simeq 5.3$ MeV. A gaussian fit of this local excess leads to an amplitude of $A = 12.1 \pm 3.4\%$ (3.5$\sigma$).

We report a measurement of the antineutrino rate from the fission of ^{235}U with the STEREO detector using 119 days of reactor turned on. In our analysis, we perform several detailed corrections and achieve the most precise single measurement at reactors with highly enriched ^{235}U fuel. We measure an IBD cross section per fission of σ_{f}=(6.34±0.06[stat]±0.15[sys]±0.15[model])×10^{-43}  cm^{2}/fission and observe a rate deficit of (5.2±0.8[stat]±2.3[sys]±2.3[model])% compared to the model, consistent with the deficit of the world average. Testing ^{235}U as the sole source of the deficit, we find a tension between the results of lowly and highly enriched ^{235}U fuel of 2.1 standard deviations.

We comment on the claimed observation [arXiv:arXiv:2005.05301] of sterile neutrino oscillations by the Neutrino-4 collaboration. Such a claim, which requires the existence of a new fundamental particle, demands a level of rigor commensurate with its impact. The burden lies with the Neutrino-4 collaboration to provide the information necessary to prove the validity of their claim to the community. In this note, we describe aspects of both the data and analysis method that might lead to an oscillation signature arising from a null experiment and describe additional information needed from the Neutrino-4 collaboration to support the oscillation claim. Additionally, as opposed to the assertion made by the Neutrino-4 collaboration, we also show that the method of 'coherent summation' using the $L/E$ parameter produces similar results to the methods used by the PROSPECT and the STEREO collaborations.

The STEREO experiment is a very short baseline reactor antineutrino experiment. It is designed to test the hypothesis of light sterile neutrinos being the cause of a deficit of the observed antineutrino interaction rate at short baselines with respect to the predicted rate, known as the reactor antineutrino anomaly. The STEREO experiment measures the antineutrino energy spectrum in six identical detector cells covering baselines between 9 and 11 m from the compact core of the ILL research reactor. In this article, results from 179 days of reactor turned on and 235 days of reactor turned off are reported at a high degree of detail. The current results include improvements in the modelling of detector optical properties and the gamma-cascade after neutron captures by gadolinium, the treatment of backgrounds, and the statistical method of the oscillation analysis. Using a direct comparison between antineutrino spectra of all cells, largely independent of any flux prediction, we find the data compatible with the null oscillation hypothesis. The best-fit point of the reactor antineutrino anomaly is rejected at more than 99.9% C.L.