The energy dependence of the light output for secondary charged particles (protons and alpha-particles) was measured in the neutron energy range of 1.5-14.0 MeV for an array of scintillation detectors based on a EJ-200 scintillator. The scattering of a tagged neutron beam with an energy of 14.1 MeV on graphite and polyethylene samples was used to obtain neutrons with known energies at different angles. Based on the obtained data, both the response function and the intrinsic efficiency of the detectors used were simulated in GEANT4. To verify the simulated efficiency a method based on the measurement of elastically scattered neutrons from the 1H(n,n0)1H reaction was implemented.
The excitation functions of ^nat Mo( α , x) ^97 Ru and ^nat Mo( α , x) ^103 Ru reactions in the energy range of 10–22 MeV are determined using the stacked foil activation technique and offline γ -ray spectrometry. The correction for γ -self attenuation is performed in the present measurement. The theoretical predictions of cross-section for ^nat Mo( α , x) ^97 Ru and ^nat Mo( α , x) ^103 Ru reactions are calculated by TALYS. The results of the experiment are compared with the existing cross-section data available in the EXFOR database and different level density models by TALYS code. The uncertainty propagation in the measured cross-sections and correlation matrix using covariance analysis has been studied in this work.
In this study, we measured the 58 Ni( n , p ) 58 Co reaction cross section with neutron energies of 1.06, 1.86, and 2.85 MeV. The cross section was measured using neutron activation techniques and γ -ray spectroscopy, and it was compared with cross section data available in the EXFOR. Furthermore, we calculated the covariance matrix of the measured cross section for the aforementioned nuclear reaction. The uncertainties of the theoretical calculation for 58 Ni( n , p ) 58 Co reaction cross section were calculated via Monte Carlo method. In this study, we used uncertainties in the optical model and level density parameters to calculate uncertainties in the theoretical cross sections. The theoretical calculations were performed by using TALYS-1.96. In this study, we aim to analyze the effect of uncertainties of the nuclear model input as well as different experimental variables used to obtain the values of reaction cross section.
Within the TANGRA project framework, a new experimental setup has been constructed for the measurement of reaction cross sections (n, X, γ) in the interaction of 14.1 MeV neutrons with nuclei. The facility has a special feature: the use of the tagged neutron method. This method enables efficient separation of background and useful events, as well as accurate tracking of neutron flux. Test measurements were performed on 28Si, 12C, and 16O nuclei, and the results showed satisfactory agreement with available experimental data. This paper presents the features of the setup design and the methodology for processing the obtained experimental data
Most gamma-ray scintillation detectors currently in use are made from inorganic materials that have a relatively high electron density. Quite often they are used to build multidetector systems that provide high scintillation light output. The performance of a gamma radiation detector (its detection efficiency) depends on the shape and size of the crystal, as well as on the source-to-detector geometry used. The NaI(Tl) gamma detector exhibits moderate energy resolution but relatively high gamma-ray detection efficiency and fast time response. In this work, the efficiency and resolution of a scintillation hexagonal detector are studied to optimize its response function. This type and size of scintillator were selected to construct a budget-friendly, reconfigurable, easy-to-maintain multidetector system for registering gamma-rays following fission, capture, and inelastic neutron scattering reactions, with reasonably good energy and time resolutions The research results made it possible to establish a geometric solid angle that increases the efficiency of recording gamma-ray radiation of the hexagonal NaI(Tl) scintillation probe under study.
A study of the inelastic scattering of neutrons with an energy of 14.1 MeV on the nuclei of oxygen, phosphorus and sulfur was carried out at the TANGRA facility at JINR (Dubna). The purpose of the experiment was to refine existing and obtain new data on the yields and angular distributions of γ-quanta emitted by the studied nuclei as a result of neutron-induced nuclear reactions using the tagged neutron method. Two types of detector systems were used to register γ-quanta. The γ-ray yields were measured using a high-purity germanium (HPGe) detector. The angular distributions of γ-rays were obtained using a system of 18 scintillation detectors based on bismuth germanite Bi 4 Ge 3 O 12 (BGO) located around the sample. As a result of the studies carried out, the yields of two transitions for the reaction of tagged neutrons with 16 O, nine transitions for the reaction with 31 P, and nine transitions for the reaction with 32 S were measured for the first time. The angular anisotropy of the γ-radiation accompanying the inelastic scattering of neutrons with an energy of 14.1 MeV on 31 P nuclei was also measured for the first time.
In this paper, we describe an experimental setup designed to investigate double and triple angular correlations, specifically (n-gamma) and (n-n 'gamma)-correlations. The experiment was conducted by the TAgged Neutrons and Gamma-RAys (TANGRA) group at the Frank Laboratory of Neutron Physics, Joint Institute for Nuclear Research. A key feature of this experiment is the implementation of the tagged neutron method, which enables the determination of the emission direction and propagation of neutrons tagged with alpha-particles (He-4) resulting from the T(D,n)He-4 reaction. The deuterium-tritium reaction releases approximately 80% of its energy through the emission of 14MeV neutrons. Neutrons scattered by the irradiated target sample were detected using long plastic scintillation detectors, each equipped with fast photomultipliers at both ends. The dual photomultiplier configuration enhanced the position sensitivity of these detectors and improved their angular resolution.
Tagged neutrons with an initial energy of 14.1 MeV scattered on a carbon sample are measured within the framework of the TANGRA project. Angular distributions of neutrons are obtained for elastic scattering and scattering to the first excited state of 12 C with an energy of 4.44 MeV. Results are compared to experimental data from other authors and model calculations performed using a coupled channels model with a deformed optical potential.
Tagged neutrons are used to perform an experimental investigation of the inelastic scattering of 14.1 MeV neutrons on 23Na and 35Cl nuclei as part of the TANGRA project at the Frank Laboratory of Neutron Physics, Joint Institute for Nuclear Research. The energies and yields of γ quanta for transitions observed in the experiment are measured, and the γ angular distribution coefficients for the highest intensity γ transitions are obtained. The experimental data are compared to others in the literature.
In the framework of TANGRA-project at the Frank Laboratory of Neutron Physics of the Joint Institute for Nuclear research in Dubna (Russia), two experimental setups (Fig. 1) have been designed and tested for investigation of 14-MeV neutron-induced nuclear reactions on a number of important for nuclear science and engineering isotopes. As a source of 14-MeV “tagged” neutrons we are using the VNIIA ING-27 steady-state portable neutron generator with embedded in its vacuum tube 64-pixel charge-particle detector. The “Romashka” system is an array of up-to 24 hexagonal NaI(Tl)-crystal scintillation probes, while the “Romasha” array consists of 18 cylindrical BGO-crystal detectors of neutrons and gamma-rays. In addition to these detectors there is a HPGe gamma-ray spectrometer and a number of Stilbene detectors that can be added for high-resolution gamma-ray spectrometry and neutron-gamma detection. The main characteristics of the neutron-induced nuclear reaction products can be investigated by commissioning the detectors in suitable for these experiments’ geometries. Both setups can be used for doing basic and applied scientific research, because they permit simultaneously to measure the energy, angle and multiplicity distributions of gamma-rays and neutrons, produced in the competitive neutron-induced nuclear reactions (n, n’γ), (n,2n), (n, xnγ) and (n, f) in pure or complex substances.
The response function of the BGO, NaI (Tl) and LaBr3(Ce) scintillation detectors to monoenergetic gamma quanta was built on the basis of Monte Carlo simulations using the GEANT4 toolkit and calibration measurements with gamma radiation sources of different energies. The response function consists of seven components: the first six constitute the detector’s response to a direct hit of monoenergetic gamma radiation and depend on the properties of the detector (size, material, energy resolution, etc.), and the seventh component represents the effect of surrounding materials on the measured gamma spectrum. For each component of the function, the analytical form of the energy dependence is determined and its parameters are found when registering gamma quanta with energies in the range from 0.3 MeV to 10 MeV.
Scintillation NaI(Tl) crystals are typically utilized at room temperature for detection of energetic photons in high energy and nuclear physics research, non-destructive analysis of materials testing, safeguards, verification of nuclear treaty, geological exploration and therapeutic imaging. The present work provides a new geometry for the source-to-detector combination. A special order cubic detector with rectangular cavity was used. The mathematical expressions of the path-lengths traveled by the incident photon as well as the geometrical solid angle were derived. The detector efficiency was determined for an axially positioned standard point-like gamma-ray source using the analytical efficiency transfer technique. Geant4 Monte Carlo simulation code was also used to predict the detector response under the calibration geometry. The analytical efficiency transfer and Geant4 simulation results were compared with those obtained experimentally and a good agreement between them was shown.
A study of the reaction of inelastic scattering of 14.1 MeV neutrons by 23 Na nuclei was carried out at the TANGRA facility using the tagged neutron method. In this work, the energies of visible g-transitions are determined, the yields of g -quanta are obtained, the angular distributions of g -quanta for 23 Na are measured. The results obtained are in good agreement with the data of other published experimental works.
In the frame of TANGRA-project at JINR-FLNP (Dubna) we measured the gamma-rays resulting from the inelastic scattering of 14.1 MeV neutrons on magnesium. As a source of neutrons we used ING-27 portable neutron generator of VNIIA (Moscow) where the neutrons are produced in a d-t fusion-fission nuclear reaction, H(d,n)He. The α-particles were registered by a 64-pixel Si charge particle detector embedded in ING-27 vacuum chamber. The sample tested was a 10cm-thick plastic cube filled with MgO powder. The gamma-rays from the interaction of neutrons with the sample we registered by a Romashka-type Fe-protected array, consisted of 22 hexagonal NaI(Tl) scintillator prisms. The analog signals form all the αand γdetectors were collected in list-mode, simultaneously, by a computerized 32-channel data acquisition system (DAQ) from JINR AFI-electronics, which was used, also, for digitizing and storing the waveforms on the computer hard-drive for further off-line analysis with CERN-ROOT modular scientific software toolkit. Using the time-correlated associated particle method (TCAPM), also known as tagged neutron method (TNM), the influence of the background radiation on the collected gamma-ray spectra was
Low cost scintillation detectors as compared with HPGe detectors are considered to be one of most important radiation detection tools. Therefore, these detectors can be manufactured in different shapes and work at room temperature without any cooling systems, which added an extra advantage to it. This work presents a study of a cubic detector with a rectangular cavity in different experimental setup geometries, using standard point-like gamma-ray sources, where the efficiency of the detector in these geometries was the target to be studied. According to this aim, the data from the experimental measurements was used to determine the detector efficiency. An analytical calculation of the detector efficiency was done by using a new mathematical expression, this mathematical expression depends on the efficiency transfer technique and effective solid angle calculations. To support the mathematical model, the source-to-detector arrangement was simulated by Geant4 Monte Carlo code. All the compared efficiency results were found to be promising and trusted based on the calculated deviation percentages.
The fast and thermal neutron attenuation properties through polymer composites based on high density polyethylene (HDPE) reinforced by micro-sized and nano-sized Cadmium Oxide (CdO) particles with weight fractions of 10% and 40% have been investigated. This study was carried out to present a new composite material based on HDPE filled with CdO in the form of micro and nano particles to be used as a promising neutron radiation shielding material. The composites were fabricated by compression molding technique and characterized by a scanning electron microscope (SEM). The composites were subjected to fast neutrons generated from Pu-238-Be neutron source with activity 12 x 10(9) Bq and detected by a Stilbene scintillator. The fast neutron shielding properties were determined in terms of the fast neutron transmission fractions of the composites. The neutron activation method was applied by using Indium foils and Indium foils covered with Cadmium as a detector to study the properties of the thermal and epithermal neutron fluxes of the composites upon exposure to neutron flux generated from Am-241-Be neutron source. It is clear from this study that the transmitted fractions for fast neutron in case of nano CdO/HDPE composites are less than the case of micro CdO/HDPE composites, however, the capture of thermal neutrons inside the micro CdO/HDPE composites is more probable than that in nano CdO/HDPE composites at the same weight fraction. Tensile mechanical testing has been conducted and showed that particle addition percentage and size have significant effect on the mechanical properties of composites. Nano CdO/HDPE composites showed more superior mechanical properties compared to micro CdO/HPDE composites at the same particle addition level.
The reaction induced by the inelastic scattering of 14.1-MeV neutrons on chromium nuclei is studied by means of the tagged-neutron method at the TANGRA (TAgged Neutrons and Gamma RAys) facility deployed at Frank Laboratory of Neutron Physics, Joint Institute for Nuclear Research, and based on the ING-27 standard neutron generator. The energies of visible gamma transitions occurring in various reactions of neutron interaction with chromium nuclei and their partial cross sections are determined. The results obtained by measuring the angular distribution of gamma rays for $${}^{52}$$Cr are analyzed and are compared with respective results of other experimental studies available in the literature.
This paper is dedicated to n+C-12, n+Mg-24, n+Cr-52 -reactions investigation at 14.1 MeV neutron energy. Characteristics of these reactions have been calculated using TALYS code to estimate perspectives of using of this code in data interpretation in the TANGRA project. This project is performed in Frank Laboratory of Neutron Physics (FLNP JINR) to investigate properties of (n,xy)-type reactions, important for fundamental and practical applications.