A search for production of the superheavy elements with atomic numbers 119 and 120 was performed in the Ti-50 + Bk-249 and Ti-50 + Cf-249 fusion-evaporation reactions, respectively, at the gas-filled recoil separator TASCA at GSI Darmstadt, Germany. Over four months of irradiation, the Bk-249 target partially decayed into Cf-249, which allowed for a simultaneous search for both elements. Neither was detected at cross-section sensitivity levels of 65 and 200 fb for the Ti-50 + Bk-249 and Ti-50 + Cf-249 reactions, respectively, at a midtarget beam energy of E-lab = 281.5 MeV. The nonobservation of elements 119 and 120 is discussed within the concept of fusion-evaporation reactions including various theoretical predictions on the fission-barrier heights of superheavy nuclei in the region of the island of stability.
The neutron-deficient isotopes 254,255Rf were produced in the fusion-evaporation reaction 50Ti+206Pb at the gas-filled recoil separator TASCA. Decay properties of these nuclei were investigated by applying fast digital electronics. A search for isomeric states in both isotopes was performed by using the accompanying conversion electron emissions. Isomeric states with half-lives of 4(1) μs and >30 μs were measured for 254Rf and 255Rf, respectively, which confirm the findings at different separators. The present experimental results demonstrate the great potential of fast digital electronics for measurements of isomeric states in the heaviest nuclei, which are only producible in small quantities.
Fusion-evaporation reactions with the doubly magic projectile 48Ca were used to access neutron-deficient nuclei around neptunium at the velocity filter SHIP, and investigated using the COMPASS decay spectroscopy station. With the use of digital electronics, several isotopes produced via neutron, proton, and α evaporation channels were identified by establishing correlated α-decay chains with short-lived sub-μs members. Data are given on decay chains stemming from 225,226Np, 225U, and 222,223Pa. New information on the isotopes 225,226Np and 222Pa was obtained. Production cross sections of nuclei in the region using a variety of projectiles are discussed. The measured production cross-sections indicate that the usual advantages of using 48Ca as a beam projectile to produce nuclei Z>100 are absent in the production of these slightly lighter nuclei.
J. Khuyagbaatar,1,2,* A. Yakushev,2 Ch. E. Düllmann,1,2,3 D. Ackermann,2,† L.-L. Andersson,1 M. Asai,4 M. Block,2 R. A. Boll,5 H. Brand,2 D. M. Cox,6,‡ M. Dasgupta,7 X. Derkx,1,3 A. Di Nitto,3 K. Eberhardt,1,3 J. Even,1,§ M. Evers,7 C. Fahlander,8 U. Forsberg,8 J. M. Gates,9 N. Gharibyan,10 P. Golubev,8 K. E. Gregorich,9 J. H. Hamilton,11 W. Hartmann,2 R.-D. Herzberg,6 F. P. Heßberger,1,2 D. J. Hinde,7 J. Hoffmann,2 R. Hollinger,2 A. Hübner,2 E. Jäger,2 B. Kindler,2 J. V. Kratz,3 J. Krier,2 N. Kurz,2 M. Laatiaoui,2 S. Lahiri,12 R. Lang,2 B. Lommel,2 M. Maiti,12,‖ K. Miernik,5 S. Minami,2 A. Mistry,6,¶ C. Mokry,1,3 H. Nitsche,9,** J. P. Omtvedt,13 G. K. Pang,9 P. Papadakis,6,14 D. Renisch,3 J. Roberto,5 D. Rudolph,8 J. Runke,2 K. P. Rykaczewski,5 L. G. Sarmiento,8 M. Schädel,2,4 B. Schausten,2 A. Semchenkov,13 D. A. Shaughnessy,10 P. Steinegger,15,16 J. Steiner,2 E. E. Tereshatov,10,†† P. Thörle-Pospiech,1,3 K. Tinschert,2 T. Torres De Heidenreich,2 N. Trautmann,3 A. Türler,15,16 J. Uusitalo,14 D. E. Ward,8 M. Wegrzecki,17 N. Wiehl,1,3 S. M. Van Cleve,5 and V. Yakusheva1 1Helmholtz Institute Mainz, 55099 Mainz, Germany 2GSI Helmholtzzentrum für Schwerionenforschung, 64291 Darmstadt, Germany 3Johannes Gutenberg-Universität Mainz, 55099 Mainz, Germany 4Advanced Science Research Center, Japan Atomic Energy Agency, Tokai, Ibaraki 319-1195, Japan 5Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA 6University of Liverpool, Liverpool L69 7ZE, United Kingdom 7The Australian National University, Canberra, ACT 0200, Australia 8Lund University, 22100 Lund, Sweden 9Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA 10Lawrence Livermore National Laboratory, Livermore, California 94551, USA 11Vanderbilt University, Nashville, Tennessee 37235, USA 12Saha Institute of Nuclear Physics, Kolkata 700064, India 13University of Oslo, 0315 Oslo, Norway 14University of Jyväskylä, 40351 Jyväskylä, Finland 15Paul Scherrer Institute, 5232 Villigen, Switzerland 16University of Bern, 3012 Bern, Switzerland 17The Institute of Electron Technology, 02-668 Warsaw, Poland
Khuyagbaatar, J.; Yakushev, A.; Düllmann, Ch E.; Ackermann, D.; Andersson, L. L.; Asai, M.; Block, M.; Boll, R. A.; Brand, H.; Cox, D. M.; Dasgupta, M.; Derkx, X.; Di Nitto, A.; Eberhardt, K.; Even, J.; Evers, M.; Fahlander, C.; Forsberg, U.; Gates, J. M.; Gharibyan, N.; Golubev, P.; Gregorich, K. E.; Hamilton, J. H.; Hartmann, W.; Herzberg, R. D.; Heßberger, F. P.; Hinde, D. J.; Hoffmann, J.; Hollinger, R.; Hübner, A.; Jäger, E.; Kindler, B.; Kratz, J. V.; Krier, J.; Kurz, N.; Laatiaoui, M.; Lahiri, S.; Lang, R.; Lommel, B.; Maiti, M.; Miernik, K.; Minami, S.; Mistry, A.; Mokry, C.; Nitsche, H.; Omtvedt, J. P.; Pang, G. K.; Papadakis, P.; Renisch, D.; Roberto, J.
The heaviest currently known nuclei, which have up to 118 protons, have been produced in Ca-48 induced reactions with actinide targets. Among them, the element tennessine (Ts), which has 117 protons, has been synthesized by fusing Ca-48 with the radioactive target Bk-249, which has a half-life of 327 d. The experiment was performed at the gas-filled recoil separator TASCA. Two long and two short a decay chains were observed. The long chains were attributed to the decay of Ts-294. The possible origin of the short-decay chains is discussed in comparison with the known experimental data. They are found to fit with the decay chain patterns attributed to Ts-293. The present experimental results confirm the previous findings at the Dubna Gas-Filled Recoil Separator on the decay chains originating from the nuclei assigned to Ts.
The isotopic distribution of nuclei produced in the 50Ti + 249Cf reaction has been studied at the gas-filled recoil separator TASCA at GSI Darmstadt, which separates ions according to differences in magnetic rigidity. The bombardment was performed at an energy around the Bass barrier and with the TASCA magnetic fields set for collecting fusion-evaporation reaction products. Fifty-three isotopes located “north-east” of 208Pb were identified as recoiling products formed in non-fusion channels of the reaction. These recoils were implanted with energies in two distinct ranges; besides one with higher energy, a significant low-energy contribution was identified. The latter observation was not expected to occur according to kinematics of the known types of reactions, namely quasi-elastic, multi-nucleon transfer, deep-inelastic collisions or quasifission. The present observations are discussed within the framework of two-body kinematics passing through the formation of a composite system.
The isotopic distribution of nuclei produced in the 50 Ti + 249 Cf reaction has been studied at the gas- filled recoil separator TASCA at GSI Darmstadt, which separates ions according to differences in magnetic rigidity. The bombardment was performed at an energy around the Bass barrier and with the TASCA magnetic fields set for collecting fusion-evaporation reaction products. Fifty-three isotopes located “north-east” of 208 Pb were identified as recoiling products formed in non-fusion channels of the reaction. These recoils were implanted with energies in two distinct ranges; besides one with higher energy, a significant low-energy contribution was identified. The latter observation was not expected to occur according to kinematics collisions or quasifission. The present observations are discussed within the framework of two-body kinematics passing through the formation of a composite system.
The new COMPASS detection system designed and developed at GSI, Darmstadt was employed in the focal plane of the SHIP velocity filter online during a period of commissioning. The isotope No-254 was initially measured for control purposes, following which the nuclei, U-227,U-228,U-230, Np-229, and Pu-229,Pu-230 were synthesized. The obtained data from alpha-decay spectroscopy is evaluated and compared with previous measurements.
A compact silicon detector array with high spatial granularity and fast, fully digital data recording has been developed and commissioned for the investigation of heavy and superheavy nuclear species. The detector array can be combined in close geometry with large volume germanium detectors. It offers comprehensive particle and photon coincidence and correlation spectroscopy by highly efficient evaporation residue, α, γ, conversion electron and X-ray detection supported by the high granularity of the implantation chip. Access to fast decay events in the sub-microsecond region is made possible by the fast timing properties of the digital signal processing. A novel Si-chip support design allows direct cooling of the Si-chips and short signal transport. The compact and modular mechanical design equipped with a standard flange facilitates its transport and connection to different separators at different ion beam facilities. After initial tests, first α-γ coincidence spectroscopy experiments have been performed at the LISE separator of GANIL in Caen, France, in FULIS (velocity filter) mode and at the velocity filter SHIP of GSI in Darmstadt, Germany.
Abstract Online gas-solid adsorption studies with single-atom quantities of Hg, Tl, and Pb, the lighter homologs of the superheavy elements (SHE) copernicium (Cn, Z=112), nihonium (Nh, Z=113), and flerovium (Fl, Z=114), were carried out using short-lived radioisotopes. The interaction with Au and SiO2 surfaces was studied and the overall chemical yield was determined. Suitable radioisotopes were produced in fusion-evaporation reactions, isolated in the gas-filled recoil separator TASCA, and flushed rapidly to an adjacent setup of two gas chromatography detector arrays covered with SiO2 (first array) and Au (second array). While Tl and Pb adsorbed on the SiO2 surface, Hg interacts only weakly and reached the Au-covered array. Our results contribute to elucidating the influence of relativistic effects on chemical properties of the heaviest elements by providing experimental data on these lighter homologs.
The NeuRad neutron detector is constructed out of scintillation fibers and is aimed on measuring the neutron heavy fragment angular correlations from exotic neutron decays. The results of the first test of NeuRad prototype timing properties are presented in this report. The EXPERT (EXotic Particle Emission and Radioactivity by Tracking) is a part of the physics program of the Super-FRS Experiment Collaboration [1]. The EXPERT experiments are aimed at studies of the unknown exotic nuclear systems beyond the proton and neutron drip-lines. These experiments will use the first half of the Super-FRS as a radioactive beam separator and its second half as a high-resolution spectrometer. NeuRad detector will provide precise information on angular correlations between nuclear-decay neutrons and the charged decay products measured by the rest of EXPERT setup. An information on angular correlations will be used to determine the decay energy of the precursor, its life time and mode of the decay. The detector is designed in order to provide sufficient detection efficiency and fine position resolution for neutrons at expected energies about 200-800 MeV interacting with the material of fibers, in particular, via elastic scattering. The detector will be constructed of scintillating fibers (≈ 10 units) with 3x3 mm cross section and the length of 1 m each, which will be grouped into bundles. Two multianode PMT’s will be mounted on each side of bundle, each side of fiber will be read out by one pixel. Bundles will be oriented along beam axis meaning that the frontal PMT will be penetrated by neutrons. The detector will be placed at distance of ≈ 30 m from the focal plane FRF1. Such setup will ensure total angular acceptance of the detector up to ±6 mrad which reflects low transfer momentum, corresponding to the decay energy expected at the range of 0.1-100 keV. One of the significant NeuRad characteristics is the time resolution. The first neutron hit has to be determined in order to distinguish between one multi-scattered neutron and the event with multiple neutrons. The longitudinal (z) position, which enhances angular resolution, will be extracted from the time difference between the signals collected on both sides of the detector. In order to obtain required angular resolution, a position resolution about 6 cm is needed. This corresponds to the time-uncertainty of ∼ 0.5 ns. Test measurements of timing characteristics has been performed
The GEM-TPC described herein will be part of the standard beam-diagnostics equipment of the Super-FRS. This chamber will provide tracking information for particle identification at rates up to 1 MHz on an event-by-event basis. The key requirements of operation for these chambers are: close to 100% tracking efficiency under conditions of high counting rate, spatial resolution below 1 mm and a superb large dynamic range covering projectiles from Z=1 up to Z=92. The current prototype consists of two GEM-TPCs inside a single vessel, which are operating independently and have electrical drift fields in opposite directions. The twin configuration is done by flipping one of the GEM-TPCs on the middle plane with respect to the second one. In order to put this development in context, the evolution of previous prototypes will be described and its performances discussed. Finally, this chamber was tested at the University of Jyväskylä accelerator with proton projectiles and at GSI with Uranium, Xenon, fragments and Carbon beams. The results obtained have shown a position resolution between 120 to 300μm at moderate counting rate under conditions of full tracking efficiency.
The FAIR[1] facility is an international accelerator centre for research with ion and antiproton beams. It is being built at Darmstadt, Germany as an extension to the current GSI research institute. One major part of the facility will be the Super-FRS[2] separator, which will be include in phase one of the project construction. The NUSTAR experiments will benefit from the Super-FRS, which will deliver an unprecedented range of radioactive ion beams (RIB). These experiments will use beams of different energies and characteristics in three different branches; the high-energy which utilizes the RIB at relativistic energies 300-1500 MeV/u as created in the production process, the low-energy branch aims to use beams in the range of 0-150 MeV/u whereas the ring branch will cool and store beams in the NESR ring. The main tasks for the Super-FRS beam diagnostics chambers will be for the set up and adjustment of the separator as well as to provide tracking and event-by-event particle identification. The Helsinki Institute of Physics, and the Detector Laboratory and Experimental Electronics at GSI are in a joint R&D of a GEM-TPC detector which could satisfy the requirements of such tracking detectors, in terms of tracking efficiency, space resolution, count rate capability and momenta resolution. The current prototype, which is the generation four of this type, is two GEM-TPCs in twin configuration inside the same vessel. This means that one of the GEM-TPC is flipped on the middle plane w.r.t. the other one. This chamber was tested at Jyväskylä accelerator with protons projectiles and at GSI with Uranium, fragments and Carbon beams during this year 2016.
New experimental data for dissociation of relativistic 17Ne projectiles incident on targets of lead, carbon, and polyethylene targets at GSI are presented. Special attention is paid to the excitation and decay of narrow resonant states in 17Ne. Distributions of internal energy in the O15+p+p three-body system have been determined together with angular and partial-energy correlations between the decay products in different energy regions. The analysis was done using existing experimental data on 17Ne and its mirror nucleus 17N. The isobaric multiplet mass equation is used for assignment of observed resonances and their spins and parities. A combination of data from the heavy and light targets yielded cross sections and transition probabilities for the Coulomb excitations of the narrow resonant states. The resulting transition probabilities provide information relevant for a better understanding of the 17Ne structure.
The GEM-TPC detector will be part of the standard Super-FRS detection system, as tracker detectors at several focal stations along the separator and its three branches.