The interplay of kinetic electron physics and atomic processes in ultrashort laser-plasma interactions provides a comprehensive understanding of electron energy distribution's impact on plasma properties. Notably, non-equilibrium electrons play a vital role in collisional ionization, influencing ionization degrees and spectra. This paper introduces a computational model that integrates the physics of kinetic electrons and atomic processes, utilizing a Boltzmann equation for non-equilibrium electrons and a collisional-radiative model for atomic state populations. The model is used to investigate the influence of non-equilibrium electrons on collisional ionization rates and their effect on population distribution, as demonstrated by L. Young et al. (Nature, 2010). The study reveals significant non-equilibrium electron presence during XFEL-matter interactions, profoundly affecting collisional ionization rates in the gas plasma, thereby necessitating careful consideration of the Collisional-Radiative (CR) model applied to such systems.
On December 5, 2022, an indirect drive fusion implosion on the National Ignition Facility (NIF) achieved a target gain G_{target} of 1.5. This is the first laboratory demonstration of exceeding "scientific breakeven" (or G_{target}>1) where 2.05 MJ of 351 nm laser light produced 3.1 MJ of total fusion yield, a result which significantly exceeds the Lawson criterion for fusion ignition as reported in a previous NIF implosion [H. Abu-Shawareb et al. (Indirect Drive ICF Collaboration), Phys. Rev. Lett. 129, 075001 (2022)PRLTAO0031-900710.1103/PhysRevLett.129.075001]. This achievement is the culmination of more than five decades of research and gives proof that laboratory fusion, based on fundamental physics principles, is possible. This Letter reports on the target, laser, design, and experimental advancements that led to this result.
The ionization dynamic of argon plasma irradiated by an intense laser is investigated to understand transient physics in dynamic systems. This study demonstrates that significant delayed ionization responses and stepwise ionization processes are crucial factors in determining the ionization state of such systems. When an intense laser begins to ionize an initially cold argon plasma, the conditions change rapidly, leading to a delayed response in ionization. Consequently, the dynamics do not reach a steady state, even if the electron temperature and density appear unchanged, particularly when the atomic transition process is not sufficiently rapid compared to the relevant time scales. Furthermore, in this case, numerous highly excited states are created primarily through collisional excitation. Thus, even low-energy photons can predominantly ionize plasmas, challenging the conventional belief that such photon energies insufficient to overcome the binding energy of bound electrons typically contribute less to the ionization. These findings underscore the necessity of incorporating these processes in ionization modeling within radiation hydrodynamic simulations for various laser-plasma experiments.
Time-gated Sc K-shell and Ge L-shell spectra are presented from a range of characterized thermodynamic states spanning ion densities of 1019–1020cm−3 and plasma temperatures around 2000 eV. For the higher densities studied and temperatures from 1000 to 3000 eV, the Sc and Ge x-ray emission spectra are consistent with steady-state calculations from the modern atomic kinetics model SCRAM. At the lower ion densities achieved through plasma expansion, however, the model calculations require a higher plasma temperature to reproduce the observed Ge spectrum. We attribute this to ionization disequilibrium of the Sc because the ionization time scales exceed the hydrodynamic timescale when the inferred temperatures diverge.
K-shell x-ray emission spectroscopy is a standard tool used to diagnose the plasma conditions created in high-energy-density physics experiments. In the simplest approach, the emissivity-weighted average temperature of the plasma can be extracted by fitting an emission spectrum to a single temperature condition. It is known, however, that a range of plasma conditions can contribute to the measured spectra due to a combination of the evolution of the sample and spatial gradients. In this work, we define a parameterized model of the temperature distribution and use Markov Chain Monte Carlo sampling of the input parameters, yielding uncertainties in the fit parameters to assess the uniqueness of the inferred temperature distribution. We present the analysis of time-integrated S and Fe x-ray spectroscopic data from the Orion laser facility and demonstrate that while fitting each spectral region to a single temperature yields two different temperatures, both spectra can be fit simultaneously with a single temperature distribution. We find that fitting both spectral regions together requires a maximum temperature of 1310-70 +90 eV with significant contributions from temperatures down to 200 eV.
Laser-accelerated proton beams are applicable to several research areas within high-energy density science, including warm dense matter generation, proton radiography, and inertial confinement fusion, which all involve transport of the beam through matter. We report on experimental measurements of intense proton beam transport through plastic foam blocks. The intense proton beam was accelerated by the 10ps, 700J OMEGA EP laser irradiating a curved foil target, and focused by an attached hollow cone. The protons then entered the foam block of density 0.38g/cm^{3} and thickness 0.55 or 1.00mm. At the rear of the foam block, a Cu layer revealed the cross section of the intense beam via proton- and hot electron-induced Cu-K_{α} emission. Images of x-ray emission show a bright spot on the rear Cu film indicative of a forward-directed beam without major breakup. 2D fluid-PIC simulations of the transport were conducted using a unique multi-injection source model incorporating energy-dependent beam divergence. Along with postprocessed calculations of the Cu-K_{α} emission profile, simulations showed that protons retain their ballistic transport through the foam and are able to heat the foam up to several keV in temperature. The total experimental emission profile for the 1.0mm foam agrees qualitatively with the simulated profile, suggesting that the protons indeed retain their beamlike qualities.
For more than half a century, researchers around the world have been engaged in attempts to achieve fusion ignition as a proof of principle of various fusion concepts. As recently reported, a burning plasma state, where the alpha-heating in the plasma is the primary source of heating, was achieved in laboratory experiments. Following the Lawson criterion, an ignited plasma is one where the fusion heating power is high enough to overcome all the physical processes that cool the fusion plasma, creating a positive thermodynamic feedback loop with rapidly increasing temperature. In inertially confined fusion, ignition is a state where the fusion plasma can begin ``burn propagation'' into surrounding cold fuel, enabling the possibility of high energy gain. While ``scientific breakeven'' (i.e. unity target gain) has not yet been achieved, this talk reports the first controlled fusion experiment on the National Ignition Facility to produce capsule gain greater than unity (here 5.8) and reach ignition by many different formulations of the Lawson criterion. In the talk, we will discuss some key basic physics inertial confinement fusion (ICF) principles behind the burning plasma and ignition results as well as discuss future challenges.
Non-local thermodyamic equilibrium (NLTE) atomic kinetics is necessary in inertial confinement fusion Hohlraum simulations for adequately modeling high-Z walls and dopants but is computationally very expensive. We present here an approach for tabulating NLTE material data in an economical manner. Material properties for an arbitrary radiation field are provided through tabulated data for a limited set of radiation fields plus derivatives with respect to components of those radiation fields. We have implemented this method in a radiation-hydrodynamics code and compare Hohlraum simulations done with inline NLTE calculations with those done with tables constructed from the same atomic data. The results demonstrate that NLTE tables can replace inline calculations in Hohlraum simulations without a significant loss of accuracy.
In this work, we present the measurement of L-band emission from buried Sc/V targets in experiments performed at the OMEGA laser facility. The goal of these experiments was to study non-local thermodynamic equilibrium plasmas and benchmark atomic physics codes. The L-band emission was measured simultaneously by the time resolved DANTE power diagnostic and the recently fielded time integrated Soreq-Transmission Grating Spectrometer (TGS) diagnostic. The TGS measurement was used to support the spectral reconstruction process needed for the unfolding of the DANTE data. The Soreq-TGS diagnostic allows for broadband spectral measurement in the 120 eV-2000 eV spectral band, covering L- and M-shell emission of mid- and high-Z elements, with spectral resolution λ/Δλ = 8-30 and accuracy better than 25%. The Soreq-TGS diagnostic is compatible with ten-inch-manipulator platforms and can be used for a wide variety of high energy density physics, laboratory astrophysics, and inertial confinement fusion experiments.
In a plasma of sufficient size and density, photons emitted within the system have a probability of being reabsorbed and reemitted multiple times---a phenomenon known in astrophysics as resonant scattering. This effect alters the ratio of optically thick to optically thin lines, depending on the plasma geometry and viewing angle, and has significant implications for the spectra observed in a number of astrophysical scenarios, but has not previously been studied in a controlled laboratory plasma. We demonstrate the effect in the x-ray spectra emitted by cylindrical plasmas generated by high power laser irradiation, and the results confirm the geometrical interpretation of resonant scattering.
We have produced high energy density iron plasmas at temperatures above 1 keV and electron densities exceeding 1023 cm-3 (~ 1 g/cm3 ) using the Orion laser at the Atomic Weapons Establishment. These plasmas were created by irradiating 50 µm diameter layered targets with frequency doubled (λ = 527 nm), 1 ps laser pulses focused to a 100 µm diameter producing an irradiance of ~ 2 x 1018 W/cm2 . The buried layer targets consist of 160 nm iron sulfide (FeS), 60 nm potassium chloride (KCl), and 15 nm carbon. The combined layers are tamped on both sides with 3 µm of parylene-N. The x-ray emission from the plasma was measured using two time-resolved, and four time-integrated Bragg crystal spectrometers, as well as one time-integrated imaging system. One time-resolved x-ray spectrometer measured emission from L-shell transitions in highly charged iron, the other from K-shell transitions in helium-like S14+ and hydrogen-like S15+. The time-integrated spectrometers are intensity-calibrated and measured emission from K-shell transitions in sulfur, potassium, chlorine, and both K-shell and L-shell transitions in iron. The density and temperature of the plasma were determined by modeling the x-ray spectra using different spectral and hydrodynamic modeling packages. A brief overview of the uncertainties associated with the measurements and models are presented. We also give an overview of our 1-D HYDRA-DCA radiation-hydrodynamics model and improvements for future work. Our results aid in assessing experimental uncertainties associated with plasma uniformity and with x-ray emission employed as diagnostics in opacity experiments at temperatures and densities not achievable elsewhere and represent a significant step in creating and diagnosing plasmas near LTE. These results are summarized as part of the completion requirements for milestone 7121
Proton beams driven by chirped pulse amplified lasers have multi-picosecond duration and can isochorically and volumetrically heat material samples, potentially providing an approach for creating samples of warm dense matter with conditions not present on Earth. Envisioned on a larger scale, they could heat fusion fuel to achieve ignition. We have shown in an experiment that a kilojoule-class, multi-picosecond short pulse laser is particularly effective for heating materials. The proton beam can be focussed via target design to achieve exceptionally high flux, important for the applications mentioned. The laser irradiated spherically curved diamond-like-carbon targets with intensity 4 × 1018 W/cm2, producing proton beams with 3 MeV slope temperature. A Cu witness foil was positioned behind the curved target, and the gap between was either empty or spanned with a structure. With a structured target, the total emission of Cu Kα fluorescence was increased 18 fold and the emission profile was consistent with a tightly focussed beam. Transverse proton radiography probed the target with ps order temporal and 10 μm spatial resolution, revealing the fast-acting focussing electric field. Complementary particle-in-cell simulations show how the structures funnel protons to the tight focus. The beam of protons and neutralizing electrons induce the bright Kα emission observed and heat the Cu to 100 eV.
Understanding the effects of radiative transfer in High Energy Density Physics experiments is critical for the characterization of the thermodynamic properties of highly ionized matter, in particular in Inertial Confinement Fusion (ICF). We report on non-Local Thermodynamic Equilibrium experiments on cylindrical targets carried out at the Omega Laser Facility at the Laboratory for Laser Energetics, Rochester NY, which aim to characterize these effects. In these experiments, a 50/50 mixture of iron and vanadium, with a thickness of 2000 Å and a diameter of 250 μm, is contained within a beryllium tamper, with a thickness of 10 μm and a diameter of 1000 μm. Each side of the beryllium tamper is then irradiated using 18 of the 60 Omega beams with an intensity of roughly 3 × 1014 W cm−2 per side, over a duration of 3 ns. Spectroscopic measurements show that a plasma temperature on the order of 2 keV was produced. Imaging data show that the plasma remains cylindrical, with geometrical aspect ratios (quotient between the height and the radius of the cylinder) from 0.4 to 2.0. The temperatures in this experiment were kept sufficiently low (∼1–2 keV) so that the optically thin Li-like satellite emission could be used for temperature diagnosis. This allowed for the characterization of optical-depth-dependent geometric effects in the vanadium line emission. Simulations present good agreement with the data, which allows this study to benchmark these effects in order to take them into account to deduce temperature and density in future ICF experiments, such as those performed at the National Ignition Facility.
Intense lasers can accelerate protons in sufficient numbers and energy that the resulting beam can heat materials to exotic warm (10 s of eV temperature) states. Here we show with experimental data that a laser-driven proton beam focused onto a target heated it in a localized spot with size strongly dependent upon material and as small as 35 μm radius. Simulations indicate that cold stopping power values cannot model the intense proton beam transport in solid targets well enough to match the large differences observed. In the experiment a 74 J , 670 fs laser drove a focusing proton beam that transported through different thicknesses of solid Mylar, Al, Cu or Au, eventually heating a rear, thin, Au witness layer. The XUV emission seen from the rear of the Au indicated a clear dependence of proton beam transport upon atomic number, Z, of the transport layer: a larger and brighter emission spot was measured after proton transport through the lower Z foils even with equal mass density for supposed equivalent proton stopping range. Beam transport dynamics pertaining to the observed heated spot were investigated numerically with a particle-in-cell (PIC) code. In simulations protons moving through an Al transport layer result in higher Au temperature responsible for higher Au radiant emittance compared to a Cu transport case. The inferred finding that proton stopping varies with temperature in different materials, considerably changing the beam heating profile, can guide applications seeking to controllably heat targets with intense proton beams.
K-shell x-ray spectra of Li- to H-like ions have long been used to determine plasma conditions. The ratio of integrated line intensities is used to determine the temperature. At the density of non-local thermal dynamic equilibrium (NLTE) plasmas (n e ≈ 1021 cm-3), the K-shell spectrum is not very sensitive to density. We propose using the L-shell emission of open L-shell ions (C- to Li-like) as an alternative to determine both temperature and density of NLTE plasmas. First, the L-shell models of a mid-Z material need to be verified against the temperatures obtained using a K-shell spectrum of a low-Z material. A buried layer platform is being developed at the OMEGA laser to study the open L-shell spectra of NLTE plasmas of mid-Z materials. Studies have been done using a 250 μm diameter dot composed of a layer of 1200 Å thick Zn between two 600 Å thick layers of Ti, in the center of a 1000 μm diameter, 13 μm thick beryllium tamper. Lasers heat the target from both sides for up to 3 ns. The size of the emitting volume vs time was measured with x-ray imaging (face-on and side-on) to determine the density. The temperature was measured from the Ti K-shell spectra. The use of this platform for the verification of atomic L-shell models is discussed.
Time resolved x-ray images with 7 ps resolution are recorded on relativistic short-pulse laser-plasma experiments using the dilation x-ray imager, a high-speed x-ray framing camera, sensitive to x-rays in the range of ≈1−17 keV. This capability enables a series of 2D x-ray images to be recorded at picosecond scales, which allows for the investigation of fast electron transport within the target with unprecedented temporal resolution. An increase in the Kα-emission spot size over time was found for targets thinner than the recirculation limit and is absent for thicker targets. Together with the observed polarization dependence of the spot size increase, this indicates that electron recirculation is relevant for the x-ray production in thin targets.
Short pulse laser heated buried layers experiments have been performed on the Orion laser facility to study the time-resolved emission characteristics of plasmas with mass densities >= 1 g/cc and electron temperatures > 500 eV. Our streak camera measurements focused on the K-shell emission lines of He-like and H-like aluminum from a buried aluminum layer. The data were analyzed by comparison to synthetic spectra generated with the non-local thermodynamic equilibrium (NLTE) radiation transfer code Cretin, which yielded maximum temperatures of nearly 800 eV at near solid density. The time precise history of the temperature evolution was reproduced with a 1-D radiation hydrodynamic code; however, the known effect of lateral transport of energy out of the focal spot made exacting agree with theory difficult. Thus, we have observed densities of >= 1 g/cc and temperatures of > 500 eV using the 1-D analysis, which supports the idea that the aluminum plasma is locally hotter than inferred from our spatially integrating measurements and that modeling requires the inclusion of 2-dimensional effects. (C) 2017 Elsevier B.V. All rights reserved.