We show that intervalley coupling can be induced in twisted bilayer graphene (TBG) by aligning the bottom graphene layer with either of two types of commensurate insulating triangular Bravais lattice substrate. The intervalley coupling folds the ±K valleys of TBG to the Γ-point and hybridizes the original TBG flat bands into a four-band model equivalent to the p_{x}-p_{y} orbital honeycomb lattice model, in which the second conduction and valence bands have quadratic band touchings and can become flat due to geometric frustration. The spin-orbit coupling from the substrate opens gaps between the bands, yielding topological bands with spin Chern numbers C up to ±4. For realistic substrate potential strengths, the minimal bandwidths of the hybridized flat bands are still achieved around the TBG magic angle θ_{M}=1.05°, and their quantum metrics are nearly ideal. We identify two candidate substrate materials Sb_{2}Te_{3} and GeSb_{2}Te_{4}, which nearly perfectly realize the commensurate lattice constant ratio of sqrt[3] with graphene. These systems provide a promising platform for exploring strongly correlated topological states driven by geometric frustration.
We describe a semidefinite relaxation method which finds lower bounds to the ground state energy of a quantum Hamiltonian subject to Hermitian linear constraints along with approximations of ground state expectation values. We show that symmetry can be used to significantly reduce the computational requirements, and we include unitary, antiunitary, discrete, and continuous symmetries in our analysis. We demonstrate our method using the 1D Hubbard model and find quantitative agreement with both exact diagonalization and the Bethe ansatz.
Hofstadter's butterfly, the predicted energy spectrum for non-interacting electrons confined to a two-dimensional lattice in a magnetic field, is one of the most remarkable fractal structures in nature1. At rational ratios of magnetic flux quanta per lattice unit cell, this spectrum shows self-similar distributions of energy levels that reflect its recursive construction. For most materials, Hofstadter's butterfly is predicted under experimental conditions that are unachievable using laboratory-scale magnetic fields1-3. More recently, electrical transport studies have provided evidence for Hofstadter's butterfly in materials engineered to have artificially large lattice constants4-6, such as those with moiré superlattices7-10. Yet, so far, direct spectroscopy of the fractal energy spectrum predicted by Hofstadter nearly 50 years ago has remained out of reach. Here we use high-resolution scanning tunnelling microscopy/spectroscopy (STM/STS) to investigate the flat electronic bands in twisted bilayer graphene (TBG) near the predicted second magic angle11,12, an ideal setting for spectroscopic studies of Hofstadter's spectrum. Our study shows the fractionalization of flat moiré bands into discrete Hofstadter subbands and discerns experimental signatures of self-similarity of this spectrum. Moreover, our measurements uncover a spectrum that evolves dynamically with electron density, showing phenomena beyond that of Hofstadter's original model owing to the combined effects of strong correlations, Coulomb interactions and the quantum degeneracy of electrons in TBG.
Flat bands and nontrivial topological physics are two important topics of condensed matter physics. With a unique stacking configuration analogous to the Su-Schrieffer-Heeger model, rhombohedral graphite (RG) is a potential candidate for realizing both flat bands and nontrivial topological physics. Here, we report experimental evidence of topological flat bands (TFBs) on the surface of bulk RG, which are topologically protected by bulk helical Dirac nodal lines via the bulk-boundary correspondence. Moreover, upon in situ electron doping, the surface TFBs show a splitting with exotic doping evolution, with an order-of-magnitude increase in the bandwidth of the lower split band, and pinning of the upper band near the Fermi level. These experimental observations together with Hartree-Fock calculations suggest that correlation effects are important in this system. Our results demonstrate RG as a platform for investigating the rich interplay between nontrivial band topology, correlation effects, and interaction-driven symmetry-broken states.
Kekul\'e-O order in graphene, which has recently been realized experimentally, induces Dirac electron masses on the order of $m \sim 100 \text{meV}$. We show that twisted bilayer graphene in which one or both layers have Kekul\'e-O order exhibits nontrivial flat electronic bands on honeycomb and kagome lattices. When only one layer has Kekul\'e-O order, there is a parameter regime for which the lowest four bands at charge neutrality form an isolated two-orbital honeycomb lattice model with two flat bands. The bandwidths are minimal at a magic twist angle $\theta \approx 0.7^\circ$ and Dirac mass $m \approx 100 \text{meV}$. When both layers have Kekul\'e-O order, there is a large parameter regime around $\theta\approx 1^\circ$ and $m\gtrsim 100 \text{meV}$ in which the lowest three valence and conduction bands at charge neutrality each realize isolated kagome lattice models with one flat band, while the next three valence and conduction bands are flat bands on triangular lattices. These flat band systems may provide a new platform for strongly correlated phases of matter.
Modeling the behavior of superconducting electronic circuits containing Josephson junctions is crucial for the design of superconducting information processors and devices. In this paper, we introduce DEC-QED, a computational approach for modeling the electrodynamics of superconducting electronic circuits containing Josephson junctions in arbitrary three-dimensional electromagnetic environments. DEC-QED captures the nonlinear response and induced currents in BCS superconductors and accurately captures phenomena such as the Meissner effect, flux quantization, and Josephson effects. Using a spatial coarse-graining formulation based on discrete exterior calculus (DEC), DEC-QED can accurately simulate transient and long-time dynamics in superconductors. The expression of the entire electrodynamic problem in terms of the gauge-invariant flux field and charges makes the resulting classical field theory suitable for second quantization.
We propose a class of graphene-based moire systems hosting flat bands on kagome and honeycomb moire superlattices. These systems are formed by stacking a graphene layer on a 2D substrate with lattice constant N/ approximately 3 times that of graphene. When the moire potentials are induced by a 2D irreducible corep-resentation in the substrate, the model shows a rich phase diagram of low-energy bands including eigenvalue fragile phases as well as kagome and honeycomb flat bands. Spin-orbit coupling in the substrate can lift symmetry-protected degeneracies and create spin Chern bands, and we observe spin Chern numbers up to three. We additionally propose a moire system formed by stacking two graphene-like layers with similar lattice constants and Fermi energies but with Dirac Fermi velocities of opposite sign. This system exhibits multiple kagome and honeycomb flat bands simultaneously. Both models we propose resemble the hypermagic model of [Scheer et al., Phys. Rev. B 106, 115418 (2022)] and may provide ideal platforms for the realization of strongly correlated topological phases.
Modeling the behavior of superconducting electronic circuits containing Josephson junctions is crucial for the design of superconducting information processors and devices. In this paper, we introduce DEC-QED, a computational approach for modeling the electrodynamics of superconducting electronic circuits containing Josephson junctions in arbitrary three-dimensional electromagnetic environments. DEC-QED captures the non-linear response and induced currents in BCS superconductors and accurately captures phenomena such as the Meissner effect, flux quantization and Josephson effects. Using a spatial coarse-graining formulation based on Discrete Exterior Calculus (DEC), DEC-QED can accurately simulate transient and long-time dynamics in superconductors. The expression of the entire electrodynamic problem in terms of the gauge-invariant flux field and charges makes the resulting classical field theory suitable for second quantization.
The Bistritzer-MacDonald continuum model (BM model) describes the low-energy moir\'e bands for twisted bilayer graphene (TBG) at small twist angles. We derive a generalized continuum model for TBG near any commensurate twist angle, which is characterized by complex interlayer hoppings at commensurate $AA$ stackings (rather than the real hoppings in the BM model), a real interlayer hopping at commensurate $AB/BA$ stackings, and a global energy shift. The complex phases of the $AA$ stacking hoppings and the twist angle together define a single angle parameter $\phi_0$. We compute the model parameters for the first six distinct commensurate TBG configurations, among which the $38.2^\circ$ configuration may be within experimentally observable energy scales. We identify the first magic angle for any $\phi_0$ at a condition similar to that of the BM model. At this angle, the lowest two moir\'e bands at charge neutrality become flat except near the $\boldsymbol\Gamma_M$ point and retain fragile topology but lose particle-hole symmetry. We further identify a hypermagic parameter regime centered at $\phi_0 = \pm\pi/2$ where many moir\'e bands around charge neutrality (often $8$ or more) become flat simultaneously. Many of these flat bands resemble those in the kagome lattice and $p_x$, $p_y$ 2-orbital honeycomb lattice tight-binding models.
We present a framework for modeling superconducting circuits that integrates classical microwave analysis with circuit quantization. Our framework enables the calculation of the lossy eigenmodes of superconducting circuits, and we demonstrate the method by analyzing several circuits relevant to multiplexed, Purcell filtered transmon readout architectures. We show that the transmon relaxation times obtained by our method agree with the established approximation $T_1 \approx C/\text{Re}[Y(i\omega_q)]$ away from environmental resonances and do not vanish on resonance. We also show that the hybridization of the modes in the readout circuit is highly sensitive to the bandwidth of the Purcell filter.
We describe and implement a family of entangling gates activated by radio-frequency flux modulation applied to a tunable transmon that is statically coupled to a neighboring transmon. The effect of this modulation is the resonant exchange of photons directly between levels of the two-transmon system, obviating the need for mediating qubits or resonator modes and allowing for the full utilization of all qubits in a scalable architecture. The resonance condition is selective in both the frequency and amplitude of modulation and thus alleviates frequency crowding. We demonstrate the use of three such resonances to produce entangling gates that enable universal quantum computation: one iSWAP gate and two distinct controlled Z gates. We report interleaved randomized benchmarking results indicating gate error rates of 6% for the iSWAP (duration 135ns) and 9% for the controlled Z gates (durations 175 ns and 270 ns), limited largely by qubit coherence.
We show that parametric coupling techniques can be used to generate selective entangling interactions for multi-qubit processors. By inducing coherent population exchange between adjacent qubits under frequency modulation, we implement a universal gate set for a linear array of four superconducting qubits. An average process fidelity of ℱ = 93% is estimated for three two-qubit gates via quantum process tomography. We establish the suitability of these techniques for computation by preparing a four-qubit maximally entangled state and comparing the estimated state fidelity with the expected performance of the individual entangling gates. In addition, we prepare an eight-qubit register in all possible bitstring permutations and monitor the fidelity of a two-qubit gate across one pair of these qubits. Across all these permutations, an average fidelity of ℱ = 91.6 ± 2.6% is observed. These results thus offer a path to a scalable architecture with high selectivity and low cross-talk.
We present a framework for modeling superconducting circuits that integrates classical microwave analysis with circuit quantization. Our framework enables the calculation of the lossy eigenmodes of superconducting circuits, and we demonstrate the method by analyzing several circuits relevant to multiplexed, Purcell filtered transmon readout architectures. We show that the transmon relaxation times obtained by our method agree with the established approximation $T_1 \approx C/\text{Re}[Y(i\omega_q)]$ away from environmental resonances and do not vanish on resonance. We also show that the hybridization of the modes in the readout circuit is highly sensitive to the bandwidth of the Purcell filter.
Machine learning techniques have led to broad adoption of a statistical model of computing. The statistical distributions natively available on quantum processors are a superset of those available classically. Harnessing this attribute has the potential to accelerate or otherwise improve machine learning relative to purely classical performance. A key challenge toward that goal is learning to hybridize classical computing resources and traditional learning techniques with the emerging capabilities of general purpose quantum processors. Here, we demonstrate such hybridization by training a 19-qubit gate model processor to solve a clustering problem, a foundational challenge in unsupervised learning. We use the quantum approximate optimization algorithm in conjunction with a gradient-free Bayesian optimization to train the quantum machine. This quantum/classical hybrid algorithm shows robustness to realistic noise, and we find evidence that classical optimization can be used to train around both coherent and incoherent imperfections.