Unconventional superconductivity is a hallmark of exotic quantum matter, where determining the pairing symmetry is essential for uncovering its microscopic origin. Kagome superconductors provide a fertile landscape for emergent phenomena arising from strong electronic correlations and nontrivial band topology, yet their superconducting pairing symmetry remains elusive. The superconducting gap structure is commonly probed via electrodynamic response, but such measurements are inapplicable to thin flakes due to their small volume and delicate nature. Superconducting microwave resonators offer a coherent and highly sensitive platform for probing electrodynamic responses, with versatile designs that enable incorporation of diverse materials and geometries. Here, we integrate flakes into microwave circuits, enabling noninvasive access to the superfluid response through contactless coupling that preserves structural integrity. By engineering the device geometry to suppress parasitic two-level-system losses that dominate dissipation in microwave circuits, we isolate the intrinsic material response. Remarkably, the temperature-dependent superfluid density exhibits linear behavior at low temperatures, consistent with a nodal gap structure. Our approach establishes a noninvasive platform for probing electrodynamic response of fragile superconducting flakes while advancing hybrid microwave architectures for quantum technologies.
We propose a superconducting circuit hosting d low-lying states, well separated from the rest of the spectrum, that naturally realizes a qudit system protected from leakage errors. The system represents a generalization of the fluxonium and the low-energy states are constituted by fractional fluxon states, that we call fraxons, localized in the minima of a suitably designed Josephson potential. The latter is tailored through a Fourier engineering approach, that employs multi-harmonic Josephson building block elements composed by a Josephson junction and an inductance connected in series. We present the spectrum of a d=4 and a d=5 qudit system and study in detail the qutrit case. We analyze the dipole matrix elements for coupling to radiation and propose a non-Abelian, stimulated Raman adiabatic passage (STIRAP) protocol for single-qutrit gates, that is particularly suited for the present system. The proposed platform opens novel perspectives in circuit engineering and quantum computing beyond the qubit paradigm.
Recent advances in the manipulation of complex oxide layers, particularly the fabrication of atomically thin cuprate superconducting films via molecular beam epitaxy, have revealed new ways in which nanoscale engineering can govern superconductivity and its interwoven electronic orders. In parallel, the creation of twisted cuprate heterostructures through cryogenic stacking techniques marks a pivotal step forward, exploiting cuprate superconductors to deepen our understanding of exotic quantum states and propel next‐generation quantum technologies. This review explores over three decades of research in the emerging field of cuprate twistronics, examining both experimental breakthroughs and theoretical progress. It also highlights the methodologies poised to surmount the outstanding challenges in leveraging these complex quantum materials, underscoring their potential to expand the frontiers of quantum science and technology.
The advent of two-dimensional van der Waals materials is a frontier of condensed matter physics and quantum devices. However, characterizing such materials remains challenging due to the limitations of bulk material techniques, necessitating the development of specialized methods. Here, we investigate the superconducting properties of Bi2Sr2CaCu2O8+x flakes by integrating them with a hybrid superconducting microwave resonator. The hybrid resonator is significantly modified by the interaction with the flake while maintaining a high quality factor (3 × 104). We also observe a significant upshift of the resonator frequency with increasing temperature, as well as a positive nonlinearity. These effects originate from a presently unknown microscopic mechanism within the flake, and can be modeled as a two-level system bath interacting with the resonant mode. Our findings open a path for high quality hybrid circuits with van der Waals flakes for exploring novel materials and developing new devices for quantum technology.
When materials are patterned in three dimensions, there exist opportunities to tailor and create functionalities associated with an increase in complexity, the breaking of symmetries, and the introduction of curvature and non-trivial topologies. For superconducting nanostructures, the extension to the third dimension may trigger the emergence of new physical phenomena, as well as advances in technologies. Here, we harness three-dimensional (3D) nanopatterning to fabricate and control the emergent properties of a 3D superconducting nanostructure. Not only are we able to demonstrate the existence and motion of superconducting vortices in 3D but, with simulations, we show that the confinement leads to a well-defined bending of the vortices within the volume of the structure. Moreover, we experimentally observe a strong geometrical anisotropy of the critical field, through which we achieve the reconfigurable coexistence of superconducting and normal states in our 3D superconducting architecture, and the local definition of weak links. In this way, we uncover an intermediate regime of nanosuperconductivity, where the vortex state is truly three-dimensional and can be designed and manipulated by geometrical confinement. This insight into the influence of 3D geometries on superconducting properties offers a route to local reconfigurable control for future computing devices, sensors, and quantum technologies.
Van der Waals assembly allows for the creation of Josephson junctions in an atomically sharp interface between two exfoliated Bi2Sr2CaCu2O8+δ (Bi-2212) flakes that are twisted relative to each other. In a narrow range of angles close to 45°, the junction exhibits a regime where time-reversal symmetry can be spontaneously broken, and it can be used to encode an inherently protected qubit called flowermon. In this work, we investigate the physics emerging when two such junctions are integrated in a superconducting quantum interference device circuit threaded by a magnetic flux. We show that the flowermon qubit regime is maintained up to a finite critical value of the magnetic field, and, under appropriate conditions, it is protected against both charge and flux noise. For larger external fluxes, the interplay between the inherent twisted d-wave nature of the order parameter and the external magnetic flux enables the implementation of different artificial atoms, including a flux-biased protected qubit and a supersymmetric quantum circuit.
Van-der-Waals (vdW) assembly enables the fabrication of novel Josephson junctions utilizing an atomically sharp interface between two exfoliated and relatively twisted $\rm{Bi_2Sr_2CaCu_2O_{8+x}}$ (Bi2212) flakes. In a range of twist angles around $45^\circ$, the junction provides a regime where the interlayer two-Cooper pair tunneling dominates the current-phase relation. Here we propose to employ this novel junction to realize a capacitively shunted qubit that we call flowermon. The $d$-wave nature of the order parameter endows the flowermon with inherent protection against charge-noise-induced relaxation and quasiparticle-induced dissipation. This inherently protected qubit paves the way to a new class of high-coherence hybrid superconducting quantum devices based on unconventional superconductors.
Josephson junctions enable dissipation-less electrical current through metals and insulators below a critical current. Despite being central to quantum technology based on superconducting quantum bits and fundamental research into self-conjugate quasiparticles, the spatial distribution of super current flow at the junction and its predicted evolution with current bias and external magnetic field remain experimentally elusive. Revealing the hidden current flow, featureless in electrical resistance, helps understanding unconventional phenomena such as the nonreciprocal critical current, i.e., Josephson diode effect. Here we introduce a platform to visualize super current flow at the nanoscale. Utilizing a scanning magnetometer based on nitrogen vacancy centers in diamond, we uncover competing ground states electrically switchable within the zero-resistance regime. The competition results from the superconducting phase re-configuration induced by the Josephson current and kinetic inductance of thin-film superconductors. We further identify a new mechanism for the Josephson diode effect involving the Josephson current-induced phase. The nanoscale super current flow emerges as a new experimental observable for elucidating unconventional superconductivity, and optimizing quantum computation and energy-efficient devices.
Hybrid systems represent one of the frontiers in the study of unconventional superconductivity and are a promising platform to realize topological superconducting states. Owing to their mesoscopic dimensions, these materials are challenging to probe using many conventional measurement techniques, and require new experimental probes to successfully characterize. In this work, we develop a probe that enables us to measure the superfluid density of micron-size superconductors using microwave techniques drawn from circuit quantum electrodynamics (cQED). We apply this technique to a paradigmatic hybrid system, the superconductor/ferromagnet bilayer, and find that the proximity-induced superfluid density is two-fold anisotropic within the plane of the sample and exhibits power law temperature-scaling which is indicative of a nodal superconducting state. These experimental results are consistent with the theoretically predicted signatures of induced triplet pairing with a nodal $p$-wave order parameter. Moreover, we unexpectedly observe drastic modifications to the microwave response at frequencies near the ferromagnetic resonance, suggesting a coupling between the spin dynamics and induced superconducting order in the ferromagnetic layer. Our results offer new insights into the unconventional superconducting states induced in superconductor/ferromagnet heterostructures and simultaneously establish a new avenue for the study of fragile unconventional superconductivity in low-dimensional materials such as van der Waals heterostructures.
In a hydrodynamic regime of electronic fluids, the electron scattering on impurities and phonons inhibits the development of oscillating preturbulent phenomena (such as the K\'arm\'an vortex shedding) and enforces a laminar flow. Working in a local generalization of the Navier-Stokes hydrodynamics of incompressible two-dimensional fluids, we show that the critical relaxation time separating these two regimes is described by a surprisingly simple fractional power function of the Reynolds number. The critical exponent, $\alpha \simeq 4/3$, sets particular experimental conditions for the observation of preturbulent effects in electronic fluids.
Magnetism in two-dimensional (2D) van der Waals (vdW) materials has recently emerged as one of the most promising areas in condensed matter research, with many exciting emerging properties and significant potential for applications ranging from topological magnonics to low-power spintronics, quantum computing, and optical communications. In the brief time after their discovery, 2D magnets have blossomed into a rich area for investigation, where fundamental concepts in magnetism are challenged by the behavior of spins that can develop at the single layer limit. However, much effort is still needed in multiple fronts before 2D magnets can be routinely used for practical implementations. In this comprehensive review, prominent authors with expertise in complementary fields of 2D magnetism (i.e., synthesis, device engineering, magneto-optics, imaging, transport, mechanics, spin excitations, and theory and simulations) have joined together to provide a genome of current knowledge and a guideline for future developments in 2D magnetic materials research.
Coupling qubits to a superconducting resonator provides a mechanism to enable long-distance entangling operations in a quantum computer based on spins in semiconducting materials. Here, we demonstrate a controllable spin-photon coupling based on a longitudinal interaction between a spin qubit and a resonator. We show that coupling a singlet-triplet qubit to a high-impedance superconducting resonator can produce the desired longitudinal coupling when the qubit is driven near the resonator's frequency. We measure the energy splitting of the qubit as a function of the drive amplitude and frequency of a microwave signal applied near the resonator antinode, revealing pronounced effects close to the resonator frequency due to longitudinal coupling. By tuning the amplitude of the drive, we reach a regime with longitudinal coupling exceeding 1 MHz. This mechanism for qubit-resonator coupling represents a stepping stone towards producing high-fidelity two-qubit gates mediated by a superconducting resonator.
Nitrogen-vacancy (NV) center in diamond is a promising quantum sensor with remarkably versatile sensing capabilities. While scanning NV magnetometry is well-established, NV electrometry has been so far limited to bulk diamonds. Here we demonstrate imaging external alternating (AC) and direct (DC) electric fields with a single NV at the apex of a diamond scanning tip under ambient conditions. A strong electric field screening effect is observed at low frequencies due to charge noise on the surface. We quantitatively measure its frequency dependence, and overcome this screening by mechanically oscillating the tip for imaging DC fields. Our scanning NV electrometry achieved an AC E-field sensitivity of 26 mV um^(-1) Hz^(-1/2), a DC E-field gradient sensitivity of 2 V um^(-2) Hz^(-1/2), and sub-100nm resolution limited by the NV-sample distance. Our work represents an important step toward building a scanning-probe-based multimodal quantum sensing platform.
In the presence of interactions, electrons in condensed-matter systems can behave hydrodynamically, exhibiting phenomena associated with classical fluids, such as vortices and Poiseuille flow. In most conductors, electron-electron interactions are minimized by screening effects, hindering the search for hydrodynamic materials; however, recently, a class of semimetals has been reported to exhibit prominent interactions. Here we study the current flow in the layered semimetal tungsten ditelluride by imaging the local magnetic field using a nitrogen-vacancy defect in a diamond. We image the spatial current profile within three-dimensional tungsten ditelluride and find that it exhibits non-uniform current density, indicating hydrodynamic flow. Our temperature-resolve current profile measurements reveal a non-monotonic temperature dependence, with the strongest hydrodynamic effects at approximately 20 K. We also report ab initio calculations showing that electron-electron interactions are not explained by the Coulomb interaction alone, but are predominantly mediated by phonons. This provides a promising avenue in the search for hydrodynamic flow and prominent electron interactions in high-carrier-density materials.
At non-zero temperatures, superconductors contain excitations known as Bogoliubov quasiparticles (QPs). The mesoscopic dynamics of QPs inform the design of quantum information processors, among other devices. Knowledge of these dynamics stems from experiments in which QPs are injected in a controlled fashion, typically at energies comparable to the pairing energy1–5. Here we perform tunnel spectroscopy of a mesoscopic superconductor under high electric fields. We observe QP injection due to field-emitted electrons with 106 times the pairing energy, an unexplored regime of QP dynamics. Upon application of a gate voltage, the QP injection decreases the critical current and, at sufficiently high electric field, a field-emission current (<0.1 nA in our device) switches the mesoscopic superconductor into the normal state, consistent with earlier observations6. We expect that high-energy injection will be useful for developing QP-tolerant quantum information processors, will allow rapid control of resonator quality factors and will enable the design of electric-field-controlled superconducting devices with new functionality. Typically, quasiparticles are injected into superconductors at energies comparable to the pairing energy in order to gain insights into quasiparticle dynamics. Tunnelling spectroscopy of a mesoscopic superconductor under high electric field now provides insights into a regime where electrons impinge with 106 times the pairing energy.
Quantum sensing exploits the strong sensitivity of quantum systems to measure small external signals. The nitrogen-vacancy (NV) center in diamond is one of the most promising platforms for real-world quantum sensing applications, predominantly used as a magnetometer. However, its magnetic field sensitivity vanishes when a bias magnetic field acts perpendicular to the NV axis. Here, we introduce a different sensing strategy assisted by the nitrogen nuclear spin that uses the entanglement between the electron and nuclear spins to restore the magnetic field sensitivity. This, in turn, allows us to detect small changes in the magnetic field angle relative to the NV axis. Furthermore, based on the same underlying principle, we show that the NV coupling strength to magnetic noise, and hence its coherence time, exhibits a strong asymmetric angle dependence. This allows us to uncover the directional properties of the local magnetic environment and to realize maximal decoupling from anisotropic noise.
High-impedance superconducting resonators are important tools for quantum information and quantum sensing, as their resilience to magnetic fields and their highly concentrated local electric fields allow for strong coupling to small defects.We propose to use this technique to study condensed-matter systems, and particularly the properties of graphene in the quantum Hall regime. In the dispersive regime, a change in the density-of-states of graphene will affect the resonator mode, allowing for RF detection.
The electron-hole plasma in charge-neutral graphene is predicted to realize a quantum critical system whose transport features a universal hydrodynamic description, even at room temperature. This quantum critical "Dirac fluid" is expected to have a shear viscosity close to a minimum bound, with an inter-particle scattering rate saturating at the Planckian time $\hbar/(k_B T)$. While electrical transport measurements at finite carrier density are consistent with hydrodynamic electron flow in graphene, a "smoking gun" of viscous behavior remains elusive. In this work, we directly image viscous Dirac fluid flow in graphene at room temperature via measurement of the associated stray magnetic field. Nanoscale magnetic imaging is performed using quantum spin magnetometers realized with nitrogen vacancy (NV) centers in diamond. Scanning single-spin and wide-field magnetometry reveals a parabolic Poiseuille profile for electron flow in a graphene channel near the charge neutrality point, establishing the viscous transport of the Dirac fluid. This measurement is in contrast to the conventional uniform flow profile imaged in an Ohmic conductor. Via combined imaging-transport measurements, we obtain viscosity and scattering rates, and observe that these quantities are comparable to the universal values expected at quantum criticality. This finding establishes a nearly-ideal electron fluid in neutral graphene at room temperature. Our results pave the way to study hydrodynamic transport in quantum critical fluids relevant to strongly-correlated electrons in high-$T_c$ superconductors. This work also highlights the capability of quantum spin magnetometers to probe correlated-electronic phenomena at the nanoscale.