Ghost phonon polaritons (g-PhPs), a unique class of phonon polaritons in the infrared, feature ultralong diffractionless propagation (>20 μm) across the surface and tilted wavefronts in the bulk. Here, we study hybrid g-PhPs in a heterostructure of calcite and an ultrathin film of the phase change material (PCM) In3SbTe2, where the optical field is bound in the PCM film with enhanced confinement compared with conventional g-PhPs. Near-field optical images for hybrid g-PhPs reveal a lemniscate pattern in the momentum distribution. We fabricated In3SbTe2 gratings and investigated how different orientations and periodicities of gratings impact the propagation of hybrid g-PhPs. As the grating period decreases to zero, the wavefront of hybrid g-PhPs can be dynamically steered by varying the grating orientation. Our results highlight the promise of hybrid g-PhPs with tunable functionalities for nanophotonic studies.
An ultra-compact lithium niobate phase modulator based on the plasmonic slot waveguide is demonstrated with a length of ~16 μm, featuring a bandwidth exceeding 110 GHz and a high-rate operation beyond 90 Gbaud.
In recent years, the concept of hyperbolic phonon polaritons (HPPs) has revolutionized the field of nanophotonic, enabling unprecedented control over light-matter interactions at the nanoscale. Here, we theoretically propose and study the lateral optical forces in twisted mixed-dimensional MoO3 homostructures. Assisted with the low-symmetry HPPs, we realize a lateral optical force exerted on the Au nanoparticles near the surface of mixed-dimensional MoO3 homostructures with a linear polarized incident light. By controlling the polarization state, incident angle of light and the twisted angle of MoO3, the amplitude and direction of the lateral optical forces can be tailored in the mid-infrared range. Our findings provide a new platform for engineering lateral optical forces to manipulate diverse objects in a flexible and efficient manner.
Hyperbolic polaritons that originate from the extreme optical anisotropy in van der Waals (vdW) crystals have gained much attention for their potential in controlling nanolight. For practical use, there has been a strong interest to develop various manipulation strategies to customize the propagation of hyperbolic polaritons on a deeply sub-diffractional scale. In this regard, phase-change materials (PCMs) that possess two phases with different refractive indices offer suitably a tunable dielectric environment. Here, we report on the tuning of hyperbolic phonon polaritons in natural vdW crystals, hexagonal boron nitride (hBN), and alpha-phase molybdenum trioxide (α-MoO3), using the plasmonic phase-change material In3SbTe2 (IST). Unlike conventional PCMs whose both phases are dielectric, IST features a metallic crystalline phase that is stable at room temperature. The coupling between polaritons with their mirror charges in the underneath crystalline IST triggers an even stronger field confinement for polaritons. Moreover, benefited from the metallicity of laser-writable crystalline IST, we show an all-optical material platform in which crystalline IST boundaries efficiently excite and focus hyperbolic phonon polaritons in α-MoO3. Our experiments highlight the possibility to obtain new degrees of freedom in polariton engineering with plasmonic PCMs, thereby expanding the toolkit of tunable nanophotonics with flexible, on-demand fabrication and reconfiguration capabilities.
In conventional thin materials, the diffraction limit of light constrains the number of waveguide modes that can exist at a given frequency. However, layered van der Waals (vdW) materials, such as hexagonal boron nitride (hBN), can surpass this limitation due to their dielectric anisotropy, exhibiting positive permittivity along one optic axis and negativity along the other. This enables the propagation of hyperbolic rays within the material bulk and an unlimited number of subdiffractional modes characterized by hyperbolic dispersion. By employing time-domain near-field interferometry to analyze ultrafast hyperbolic ray pulses in thin hBN, we showed that their zigzag reflection trajectories bound within the hBN layer create an illusion of backward-moving and leaping behavior of pulse fringes. These rays result from the coherent beating of hyperbolic waveguide modes but could be mistakenly interpreted as negative group velocities and backward energy flow. Moreover, the zigzag reflections produce nanoscale (60 nm) and ultrafast (40 fs) spatiotemporal optical vortices along the trajectory, presenting opportunities to chiral spatiotemporal control of light–matter interactions. Supported by experimental evidence, our simulations highlight the potential of hyperbolic ray reflections for molecular vibrational absorption nanospectroscopy. The results pave the way for miniaturized, on-chip optical spectrometers, and ultrafast optical manipulation.
The discovery of ultraconfined polaritons with extreme anisotropy in a number of van der Waals (vdW) materials has unlocked new prospects for nanophotonic and optoelectronic applications. However, the range of suitable materials for specific applications remains limited. Here we introduce tellurite molybdenum quaternary oxides—which possess non-centrosymmetric crystal structures and extraordinary nonlinear optical properties—as a highly promising vdW family of materials for tunable low-loss anisotropic polaritonics. By employing chemical flux growth and exfoliation techniques, we successfully fabricate high-quality vdW layers of various compounds, including MgTeMoO 6 , ZnTeMoO 6 , MnTeMoO 6 and CdTeMoO 6 . We show that these quaternary vdW oxides possess two distinct types of in-plane anisotropic polaritons: slab-confined and edge-confined modes. By leveraging metal cation substitutions, we establish a systematic strategy to finely tune the in-plane polariton propagation, resulting in the selective emergence of circular, elliptical or hyperbolic polariton dispersion, accompanied by ultraslow group velocities (0.0003 c ) and long lifetimes (5 ps). Moreover, Reststrahlen bands of these quaternary oxides naturally overlap that of α-MoO 3 , providing opportunities for integration. As an example, we demonstrate that combining α-MoO 3 (an in-plane hyperbolic material) with CdTeMoO 6 (an in-plane isotropic material) in a heterostructure facilitates collimated, diffractionless polariton propagation. Quaternary oxides expand the family of anisotropic vdW polaritons considerably, and with it, the range of nanophotonics applications that can be envisioned.
Phonon polaritons (PhPs), collective modes hybridizing photons with lattice vibrations in polar insulators, enable nanoscale control of light. In recent years, the exploration of in-plane anisotropic PhPs has yielded new levels of confinement and directional manipulation of nano-light. However, the investigation of in-plane anisotropic PhPs at the atomic layer limit is still elusive. Here, we report the optical nanoimaging of highly-confined phonon polaritons in atomically-thin nanoribbons of α-MoO3 (5 atomic layers). We show that narrow α-MoO3 nanoribbons as thin as a few atomic layers can support anisotropic PhPs modes with a high confinement ratio (∼133 times smaller wavelength than that of light). The anisotropic PhPs interference fringe patterns in atomic layers are tunable depending on the PhP wavelength via changing the illumination frequency. Moreover, spatial control over the PhPs interference patterns is also achieved by varying the nanostructures' shape or nanoribbon width of atomically-thin α-MoO3. Our work may serve as an empirical reference point for other anisotropic PhPs that approach the thickness limit and pave the way for applications such as atomically integrated nano-photonics and sensing.
Polariton pulses—transient light-matter hybrid excitations—traveling through anisotropic media can lead to unusual optical phenomena in space and time. However, studying these pulses presents challenges with their anisotropic, ultrafast, and nanoscale field variations. Here, we demonstrate the creation, observation, and control of polariton pulses, with in-plane hyperbolic dispersion, on anisotropic crystal surfaces by using a time-resolved nanoimaging technique and our developed high-dimensional data processing. We capture and analyze movies of distinctive pulse spatiotemporal dynamics, including curved ultraslow energy flow trajectories, anisotropic dissipation, and dynamical misalignment between phase and group velocities. Our approach enables analysis of polariton pulses in the wave vector time domain, demonstrating a time-domain polaritonic topological transition from lenticular to hyperbolic dispersion contours and the ability to study the polariton-induced time-varying optical forces. Our findings promise to facilitate the study of diverse space-time phenomena at extreme scales and drive advances in ultrafast nanoimaging.
We theoretically propose and study in-plane anisotropic acoustic phonon polaritons (APhPs) based on a layered structure consisting of a monolayer (or few layers) α-phase molybdenum trioxide (α-MoO3) sandwiched between two metal layers. We find that the APhPs in the proposed sandwiched structures are a canalization (highly directional) electromagnetic mode propagating along with the layers and at the same time exhibit extreme electromagnetic-field confinement surpassing any other type of phonon-polariton modes. When a double layer of α-MoO3 is sandwiched by two Au layers, twisting the two α-MoO3 layers can adjust the interlayer polaritonic coupling and thus manipulate the in-plane propagation of the highly confined APhPs. Our results illustrate that the metal-MoO3-metal sandwiched structures are a promising platform for light guiding and manipulation at ultimate scale.
Integrated silicon-based plasmonic photodetectors have attracted more and more attention recently, due to their potential applications in THz bandwidth. In this paper, by utilizing a simplified two-step lithography process, the photoconductive detector is fabricated with the core structure of plasmonic slot waveguide in two symmetric metallic slabs as microwave electrodes to integrate with mechanically exfoliated graphene. The 3-dB bandwidth of the graphene-on-plasmonic slot waveguide photodetector is exceeded 120 GHz under the theoretical calculation, and the measured bandwidth is still beyond 70 GHz due to the lack of larger-bandwidth equipment. High-speed data reception is demonstrated for 72 Gbit/s NRZ and 64 Gbit/s PAM-4 signals with a BER below 15% soft-decision FEC threshold. Based on the enhanced interactions of light and graphene induced by the subwavelength confinement from the plasmonic structure, the responsivity of 0.13 A/W is achieved under the condition of the 7-mu m long detection zone and the 0.4-V bias voltage. With the advantages of ultra-compact, high-speed, large-bandwidth and compatible with the CMOS process, our photodetector has the potential to be used in high-speed optical interconnection, terahertz transmission and terahertz communication.
Polarization multiplexing technology is widely adopted for increasing the capacity in optical communication systems. Especially, silicon‐based integrated polarization division multiplexing (PDM) optical receivers with large bandwidth therein play an important role, which are crucial for on‐chip large‐capacity optical interconnection. Here, a silicon‐based PDM optical receiving chip is enabled by two‐dimensional grating couplers and graphene‐on‐plasmonic slot waveguide photodetectors. Utilizing the advantages of the designed focusing two‐dimensional grating couplers and plasmonic‐slot‐waveguide‐enhanced graphene–light interaction, the optical receiving chip is achieved with an ultra‐small footprint, a bandwidth exceeding 70 GHz and a reception of PDM signals in a line rate of 128 Gbit s −1 non‐return‐to‐zero and 224 Gbit s −1 four‐level pulse‐amplitude‐modulation at 1550 nm, accompanied by the bit error rates lower than the KP4 forward error correction threshold and 15% soft‐decision forward error correction threshold, respectively. Comparing with receiving the single‐polarization state, simultaneous receiving dual‐polarization state introduces about 1 dB additional power penalty because of inter‐polarization crosstalk. The graphene‐plasmonic PDM optical receiving chip can greatly improve the line rate of the system, showing its unique advantages of small footprint, high speed, large bandwidth, low crosstalk and complementary metal–oxide–semiconductor compatibility, which can be potentially used in the next generation silicon‐based high‐speed optical communication.
Photo-mixing with its advantages of ultra-large bandwidth and precise tunability has emerged as an important technique for terahertz (THz) wave generation. Recently, graphene photodetectors exhibiting a large bandwidth are expected to further boost the development of integrated THz emitters. Here, we fabricate a sub-THz emitter based on a large-bandwidth silicon–plasmonic graphene (SPG) photodetector integrated with a broadband rounded bow-tie THz antenna. The SPG sub-THz emitter is experimentally demonstrated to emit sub-THz waves with a radiation spectrum from 50 to 300 GHz. A maximum sub-THz emission power of 5.4 nW is obtained at 145 GHz with only 3 mW input light power. The SPG sub-THz emitter can be fabricated by a CMOS-compatible process, which offers enormous opportunities for its use in a variety of THz applications.
目的:探讨小儿珠珀散治疗感冒的药物效应,为临床应用提供参考.方法:针对感冒过程中儿童可能出现的发热、咳嗽、痰多、消化不良等症状,分别利用脂多糖(LPS)致热家兔,氨水诱发小鼠咳嗽,酚红排泌法、半固体营养糊小鼠肠推进实验探讨小儿珠珀散对症治疗的作用.结果:小儿珠珀散可降低小鼠耳肿胀程度、家兔体温上升幅度;延长小鼠咳嗽潜伏期,减少咳嗽次数,减少小鼠气管酚红排出量;促进小鼠胃排空,增加小鼠小肠推进率(P均<0.05).结论:小儿珠珀散可缓解感冒过程中的多种症状.
We report high-data rate reception of polarization division multiplexing signals using graphene-on-plasmonic slot waveguide photodetectors with bandwidth exceeding 70 GHz. 128 Gbps NRZ and 224 Gbps PAM-4 signals reception are experimentally demonstrated at 1550 nm with high quality.
We present an ultra-compact graphene-on-plasmonic slot waveguide photodetector with active size of 90 nm × 100 nm × 6 μm, which shows a responsivity of 300 mA/W, a 1.5-dB bandwidth exceeding 70 GHz and 72 GBd high-data rate reception for communication band of 1550 nm.